Advanced Materials, volume 32, issue 23, pages 2001093

Scalable Manufacturing of Free‐Standing, Strong Ti 3 C 2 T x MXene Films with Outstanding Conductivity

ZHANG JIZHEN ¹

Kong Na ²

Uzun Simge ³

Levitt Ariana ³

Seyedin Shayan ¹

Lynch Peter A. ¹

Qin Si ¹

Han Meikang ³

Yang Wen-Rong ²

Liu Jingquan ⁴

Wang Xungai ¹

Gogotsi Yury ³

Razal Joselito M. ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Institute for Frontier Materials Deakin University Geelong Victoria 3216 Australia |

School of Life and Environmental Sciences Deakin University Geelong Victoria 3216 Australia |

A.J. Drexel Nanomaterials Institute and Department of Materials Science and Engineering Drexel University Philadelphia PA 19104 USA |

⁴

College of Materials Science and Engineering Institute for Graphene Applied Technology Innovation Qingdao University Qingdao 266071 China |

Publication type: Journal Article

Publication date: 2020-04-20

Wiley

Journal: Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor: 29.4

ISSN: 09359648, 15214095

DOI: 10.1002/adma.202001093

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General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

Free-standing films that display high strength and high electrical conductivity are critical for flexible electronics, such as electromagnetic interference (EMI) shielding coatings and current collectors for batteries and supercapacitors. 2D Ti3C2Tx flakes are ideal candidates for making conductive films due to their high strength and metallic conductivity. It is, however, challenging to transfer those outstanding properties of single MXene flakes to macroscale films as a result of the small flake size and relatively poor flake alignment that occurs during solution-based processing. Here, a scalable method is shown for the fabrication of strong and highly conducting pure MXene films containing highly aligned large MXene flakes. These films demonstrate record tensile strength up to ≈570 MPa for a 940 nm thick film and electrical conductivity of ≈15 100 S cm−1 for a 214 nm thick film, which are both the highest values compared to previously reported pure Ti3C2Tx films. These films also exhibit outstanding EMI shielding performance (≈50 dB for a 940 nm thick film) that exceeds other synthetic materials with comparable thickness. MXene films with aligned flakes provide an effective route for producing large-area, high-strength, and high-electrical-conductivity MXene-based films for future electronic applications.

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Citations by journals

	5 10 15 20 25 30 35
Chemical Engineering Journal	Chemical Engineering Journal, 35, 5.85% Chemical Engineering Journal 35 publications, 5.85%
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Journal of Materials Chemistry A	Journal of Materials Chemistry A, 15, 2.51% Journal of Materials Chemistry A 15 publications, 2.51%
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Citations by publishers

	20 40 60 80 100 120 140 160 180
Wiley	Wiley, 175, 29.26% Wiley 175 publications, 29.26%
Elsevier	Elsevier, 122, 20.4% Elsevier 122 publications, 20.4%
American Chemical Society (ACS)	American Chemical Society (ACS), 107, 17.89% American Chemical Society (ACS) 107 publications, 17.89%
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Cambridge University Press	Cambridge University Press, 4, 0.67% Cambridge University Press 4 publications, 0.67%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 4, 0.67% American Association for the Advancement of Science (AAAS) 4 publications, 0.67%
The Electrochemical Society	The Electrochemical Society, 2, 0.33% The Electrochemical Society 2 publications, 0.33%
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World Scientific	World Scientific, 1, 0.17% World Scientific 1 publication, 0.17%
SAGE	SAGE, 1, 0.17% SAGE 1 publication, 0.17%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.17% Frontiers Media S.A. 1 publication, 0.17%
Higher Education Press	Higher Education Press, 1, 0.17% Higher Education Press 1 publication, 0.17%
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Taylor & Francis	Taylor & Francis, 1, 0.17% Taylor & Francis 1 publication, 0.17%
Walter de Gruyter	Walter de Gruyter, 1, 0.17% Walter de Gruyter 1 publication, 0.17%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.17% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.17%
Wolters Kluwer Health	Wolters Kluwer Health, 1, 0.17% Wolters Kluwer Health 1 publication, 0.17%
American Physical Society (APS)	American Physical Society (APS), 1, 0.17% American Physical Society (APS) 1 publication, 0.17%
Materials Research Society	Materials Research Society, 1, 0.17% Materials Research Society 1 publication, 0.17%
	20 40 60 80 100 120 140 160 180

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ZHANG J. et al. Scalable Manufacturing of Free‐Standing, Strong Ti 3 C 2 T x MXene Films with Outstanding Conductivity // Advanced Materials. 2020. Vol. 32. No. 23. p. 2001093.

GOST all authors (up to 50) Copy

ZHANG J., Kong N., Uzun S., Levitt A., Seyedin S., Lynch P. A., Qin S., Han M., Yang W., Liu J., Wang X., Gogotsi Y., Razal J. M. Scalable Manufacturing of Free‐Standing, Strong Ti 3 C 2 T x MXene Films with Outstanding Conductivity // Advanced Materials. 2020. Vol. 32. No. 23. p. 2001093.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adma.202001093

UR - https://doi.org/10.1002%2Fadma.202001093

TI - Scalable Manufacturing of Free‐Standing, Strong Ti 3 C 2 T x MXene Films with Outstanding Conductivity

T2 - Advanced Materials

AU - Kong, Na

AU - Razal, Joselito M.

AU - ZHANG, JIZHEN

AU - Uzun, Simge

AU - Levitt, Ariana

AU - Seyedin, Shayan

AU - Lynch, Peter A.

AU - Qin, Si

AU - Han, Meikang

AU - Yang, Wen-Rong

AU - Liu, Jingquan

AU - Wang, Xungai

AU - Gogotsi, Yury

PY - 2020

DA - 2020/04/20 00:00:00

PB - Wiley

SP - 2001093

IS - 23

VL - 32

SN - 0935-9648

SN - 1521-4095

ER -

BibTex |

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BibTex Copy

@article{2020_ZHANG,

author = {Na Kong and Joselito M. Razal and JIZHEN ZHANG and Simge Uzun and Ariana Levitt and Shayan Seyedin and Peter A. Lynch and Si Qin and Meikang Han and Wen-Rong Yang and Jingquan Liu and Xungai Wang and Yury Gogotsi},

title = {Scalable Manufacturing of Free‐Standing, Strong Ti 3 C 2 T x MXene Films with Outstanding Conductivity},

journal = {Advanced Materials},

year = {2020},

volume = {32},

publisher = {Wiley},

month = {apr},

url = {https://doi.org/10.1002%2Fadma.202001093},

number = {23},

pages = {2001093},

doi = {10.1002/adma.202001093}

}

MLA

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MLA Copy

ZHANG, JIZHEN, et al. “Scalable Manufacturing of Free‐Standing, Strong Ti 3 C 2 T x MXene Films with Outstanding Conductivity.” Advanced Materials, vol. 32, no. 23, Apr. 2020, p. 2001093. https://doi.org/10.1002%2Fadma.202001093.

Found error?

Publisher

Wiley

Journal

Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor

29.4

ISSN

09359648 (Print)
15214095 (Electronic)