Ethylene/10-Undecenoic Acid Copolymers Prepared with Different Metallocene Catalysts
Maria L. Cerrada
1
,
R. Benavente
2
,
Ernesto Pérez
2
,
Jorge Moniz-Santos
3
,
João M Campos
3
,
Maria do Rosário Ribeiro
3
2
Publication type: Journal Article
Publication date: 2007-04-19
scimago Q2
wos Q3
SJR: 0.569
CiteScore: 4.5
Impact factor: 2.7
ISSN: 10221352, 15213935
Materials Chemistry
Organic Chemistry
Physical and Theoretical Chemistry
Condensed Matter Physics
Polymers and Plastics
Abstract
The synthesis and characterisation of several functionalised polyethylenes, obtained by direct copolymerisation of ethylene with 10-undecenoic acid (UA), have been carried out. Two metallocene complexes of C s symmetry with different bridges were used: a dimethylsilyl bridge complex Me 2 Si(Cp)(Flu)ZrCl 2 and a phenylidene bridge complex Ph 2 C(Cp)(Flu)ZrCl 2 . For comparison, results obtained with the Cp 2 ZrCl 2 / MAO system are also reported. The copolymerisation activity depends strongly on the metallocene complex and on the added amount of the UA comonomer. High incorporation levels of up to 7.3 mol-% are achieved when using the phenylidene bridged catalyst presenting a rigid structure and a wide bite angle. The effect of comonomer content and catalyst geometry on the crystalline structure and mechanical behaviour of the different copolymers are comprehensively discussed.
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14
Total citations:
14
Citations from 2024:
2
(14%)
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GOST
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Cerrada M. L. et al. Ethylene/10-Undecenoic Acid Copolymers Prepared with Different Metallocene Catalysts // Macromolecular Chemistry and Physics. 2007. Vol. 208. No. 8. pp. 841-850.
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Cerrada M. L., Benavente R., Pérez E., Moniz-Santos J., Campos J. M., Ribeiro M. D. R. Ethylene/10-Undecenoic Acid Copolymers Prepared with Different Metallocene Catalysts // Macromolecular Chemistry and Physics. 2007. Vol. 208. No. 8. pp. 841-850.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/macp.200600575
UR - https://doi.org/10.1002/macp.200600575
TI - Ethylene/10-Undecenoic Acid Copolymers Prepared with Different Metallocene Catalysts
T2 - Macromolecular Chemistry and Physics
AU - Cerrada, Maria L.
AU - Benavente, R.
AU - Pérez, Ernesto
AU - Moniz-Santos, Jorge
AU - Campos, João M
AU - Ribeiro, Maria do Rosário
PY - 2007
DA - 2007/04/19
PB - Wiley
SP - 841-850
IS - 8
VL - 208
SN - 1022-1352
SN - 1521-3935
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2007_Cerrada,
author = {Maria L. Cerrada and R. Benavente and Ernesto Pérez and Jorge Moniz-Santos and João M Campos and Maria do Rosário Ribeiro},
title = {Ethylene/10-Undecenoic Acid Copolymers Prepared with Different Metallocene Catalysts},
journal = {Macromolecular Chemistry and Physics},
year = {2007},
volume = {208},
publisher = {Wiley},
month = {apr},
url = {https://doi.org/10.1002/macp.200600575},
number = {8},
pages = {841--850},
doi = {10.1002/macp.200600575}
}
Cite this
MLA
Copy
Cerrada, Maria L., et al. “Ethylene/10-Undecenoic Acid Copolymers Prepared with Different Metallocene Catalysts.” Macromolecular Chemistry and Physics, vol. 208, no. 8, Apr. 2007, pp. 841-850. https://doi.org/10.1002/macp.200600575.