Structurally uniform 1-hexene, 1-octene, and 1-decene oligomers: Zirconocene/MAO-catalyzed preparation, characterization, and prospects of their use as low-viscosity low-temperature oil base stocks
Publication type: Journal Article
Publication date: 2018-01-01
scimago Q2
wos Q2
SJR: 1.000
CiteScore: 8.6
Impact factor: 4.8
ISSN: 0926860X, 18733875
Catalysis
Process Chemistry and Technology
Abstract
Abstract An original approach to α-olefin oligomerization as well as novel thermally stable zirconocene catalysts for use in such reactions has been elaborated. The method reported allows the achievement of fractions of lightweight α-olefin oligomers up to 90% yields without considerable formation of byproducts like internal alkenes, alkanes, and higher oligomers. Trimers, tetramers, and pentamers of 1-hexene, 1-octene, and 1-decene were isolated as individual compounds and were hydrogenated. Viscosity characteristics of the isolated saturated and unsaturated hydrocarbons have been studied at various temperatures. The isolated saturated oligomers of 1-octene and 1-decene outperform the traditional electrophilic oligomerization products in terms of viscosity indexes, pour points, and low-temperature viscosity.
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69
Total citations:
69
Citations from 2024:
18
(26%)
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Nifant'ev I. E. et al. Structurally uniform 1-hexene, 1-octene, and 1-decene oligomers: Zirconocene/MAO-catalyzed preparation, characterization, and prospects of their use as low-viscosity low-temperature oil base stocks // Applied Catalysis A: General. 2018. Vol. 549. pp. 40-50.
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Nifant'ev I. E., Vinogradov A. A., Vinogradov A. A., Sedov I. V., Dorokhov V. G., Lyadov A. S., Ivchenko P. V. Structurally uniform 1-hexene, 1-octene, and 1-decene oligomers: Zirconocene/MAO-catalyzed preparation, characterization, and prospects of their use as low-viscosity low-temperature oil base stocks // Applied Catalysis A: General. 2018. Vol. 549. pp. 40-50.
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TY - JOUR
DO - 10.1016/j.apcata.2017.09.016
UR - https://linkinghub.elsevier.com/retrieve/pii/S0926860X17304453
TI - Structurally uniform 1-hexene, 1-octene, and 1-decene oligomers: Zirconocene/MAO-catalyzed preparation, characterization, and prospects of their use as low-viscosity low-temperature oil base stocks
T2 - Applied Catalysis A: General
AU - Nifant'ev, Ilya E.
AU - Vinogradov, Alexander A.
AU - Vinogradov, Alexey A.
AU - Sedov, Igor V
AU - Dorokhov, Viktor G
AU - Lyadov, A S
AU - Ivchenko, Pavel V
PY - 2018
DA - 2018/01/01
PB - Elsevier
SP - 40-50
VL - 549
SN - 0926-860X
SN - 1873-3875
ER -
Cite this
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@article{2018_Nifant'ev,
author = {Ilya E. Nifant'ev and Alexander A. Vinogradov and Alexey A. Vinogradov and Igor V Sedov and Viktor G Dorokhov and A S Lyadov and Pavel V Ivchenko},
title = {Structurally uniform 1-hexene, 1-octene, and 1-decene oligomers: Zirconocene/MAO-catalyzed preparation, characterization, and prospects of their use as low-viscosity low-temperature oil base stocks},
journal = {Applied Catalysis A: General},
year = {2018},
volume = {549},
publisher = {Elsevier},
month = {jan},
url = {https://linkinghub.elsevier.com/retrieve/pii/S0926860X17304453},
pages = {40--50},
doi = {10.1016/j.apcata.2017.09.016}
}