Modeling of the lithium-air battery cathodes with broad pore size distribution
Publication type: Journal Article
Publication date: 2016-09-01
scimago Q2
wos Q2
SJR: 0.546
CiteScore: 5.9
Impact factor: 3.1
ISSN: 00092614, 18734448
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract
Abstract Achieving theoretical promises of 1000 W h/kg specific energy for lithium-air batteries is quite challenging due to limited transport in the cathode along with electrode passivation. Transport can be enhanced in the electrodes with complex hierarchical pore architecture. Here, using computer simulations we analyze the effects of cathode pore size distribution (PSD) on capacity and discharge curve shape. Calculations considering a broad PSD revealed that even small discharge product resistivity prevents larger pores from accumulating the discharge product and thus turning them into non-clogging oxygen supply channels. Thus optimization of cathode architecture by adding of large-scale cavities enables cell capacity enhancement.
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18
Total citations:
18
Citations from 2024:
1
(5%)
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Sergeev A. V., Chertovich A. V., Itkis D. Modeling of the lithium-air battery cathodes with broad pore size distribution // Chemical Physics Letters. 2016. Vol. 660. pp. 149-154.
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Sergeev A. V., Chertovich A. V., Itkis D. Modeling of the lithium-air battery cathodes with broad pore size distribution // Chemical Physics Letters. 2016. Vol. 660. pp. 149-154.
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TY - JOUR
DO - 10.1016/j.cplett.2016.08.012
UR - https://doi.org/10.1016/j.cplett.2016.08.012
TI - Modeling of the lithium-air battery cathodes with broad pore size distribution
T2 - Chemical Physics Letters
AU - Sergeev, Artem V.
AU - Chertovich, Alexander V.
AU - Itkis, Daniil
PY - 2016
DA - 2016/09/01
PB - Elsevier
SP - 149-154
VL - 660
SN - 0009-2614
SN - 1873-4448
ER -
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BibTex (up to 50 authors)
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@article{2016_Sergeev,
author = {Artem V. Sergeev and Alexander V. Chertovich and Daniil Itkis},
title = {Modeling of the lithium-air battery cathodes with broad pore size distribution},
journal = {Chemical Physics Letters},
year = {2016},
volume = {660},
publisher = {Elsevier},
month = {sep},
url = {https://doi.org/10.1016/j.cplett.2016.08.012},
pages = {149--154},
doi = {10.1016/j.cplett.2016.08.012}
}