XPS study of the electron structure of heterometallic trinuclear complexes Fe2M(μ3-O)(μ-Piv)6(HPiv)3 (MMn, Co, Ni)
3
Lomonosov Moskow State University, Moscow, Russia
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Publication type: Journal Article
Publication date: 2015-11-01
scimago Q2
wos Q3
SJR: 0.601
CiteScore: 3.6
Impact factor: 1.5
ISSN: 03682048, 18732526
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
Spectroscopy
Atomic and Molecular Physics, and Optics
Condensed Matter Physics
Radiation
Abstract
Electron structure of pivalate heterometallic trinuclear complexes with a triangular structure and varying ligands environment is studied by the XPS method. An effect of substitution of one of the Fe atoms by M Mn, Co, Ni on Fe2p and M2p spectra is studied. Redistribution of electron density in an OCO group upon formation of complexes and introduction of donor ligands is discovered. Correlation of the characteristics of photoelectron spectra with the variation of ligands environment is studied. The complexes are assigned to high-spin ones with Fe in oxidation state III, and M, II. A relation is established between Fe2p-spectra characteristics and electron affinity of M ions.
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Ivanova T. et al. XPS study of the electron structure of heterometallic trinuclear complexes Fe2M(μ3-O)(μ-Piv)6(HPiv)3 (MMn, Co, Ni) // Journal of Electron Spectroscopy and Related Phenomena. 2015. Vol. 205. pp. 1-5.
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Ivanova T., Kochur A., Maslakov K., Kiskin M. A., Savilov S. V., Lunin V. V., Novotortsev V. M., Eremenko I. L. XPS study of the electron structure of heterometallic trinuclear complexes Fe2M(μ3-O)(μ-Piv)6(HPiv)3 (MMn, Co, Ni) // Journal of Electron Spectroscopy and Related Phenomena. 2015. Vol. 205. pp. 1-5.
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TY - JOUR
DO - 10.1016/j.elspec.2015.07.002
UR - https://doi.org/10.1016/j.elspec.2015.07.002
TI - XPS study of the electron structure of heterometallic trinuclear complexes Fe2M(μ3-O)(μ-Piv)6(HPiv)3 (MMn, Co, Ni)
T2 - Journal of Electron Spectroscopy and Related Phenomena
AU - Ivanova, T.M.
AU - Kochur, Andrei
AU - Maslakov, Konstantin
AU - Kiskin, Mikhail A.
AU - Savilov, Serguei V.
AU - Lunin, V. V.
AU - Novotortsev, V. M.
AU - Eremenko, Igor L.
PY - 2015
DA - 2015/11/01
PB - Elsevier
SP - 1-5
VL - 205
SN - 0368-2048
SN - 1873-2526
ER -
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BibTex (up to 50 authors)
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@article{2015_Ivanova,
author = {T.M. Ivanova and Andrei Kochur and Konstantin Maslakov and Mikhail A. Kiskin and Serguei V. Savilov and V. V. Lunin and V. M. Novotortsev and Igor L. Eremenko},
title = {XPS study of the electron structure of heterometallic trinuclear complexes Fe2M(μ3-O)(μ-Piv)6(HPiv)3 (MMn, Co, Ni)},
journal = {Journal of Electron Spectroscopy and Related Phenomena},
year = {2015},
volume = {205},
publisher = {Elsevier},
month = {nov},
url = {https://doi.org/10.1016/j.elspec.2015.07.002},
pages = {1--5},
doi = {10.1016/j.elspec.2015.07.002}
}