volume 482 pages 8-15

Control of the composition and crystal structure of exchange reaction products of rare-earth acetates with pivalic acid

Publication typeJournal Article
Publication date2018-10-01
scimago Q3
wos Q2
SJR0.393
CiteScore5.5
Impact factor3.2
ISSN00201693, 18733255
Materials Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Abstract The rare-earth metal(III) complexes [M2(piv)6(Hpiv)6] (monoclinic, P21/c, 1), [M2(piv)6(Hpiv)6]·Hpiv (monoclinic, C2/c, 2), [M(piv)3]n (trigonal, P63/m, 3), and [(Hpiv)2(iPrOH)2Sm2(piv)6]·2Hpiv (triclinic, P-1, 4), where piv is (CH3)3CCO2−, were synthesized, and their structures were determined by single-crystal X-ray diffraction (SC-XRD). The crystallization was shown to be controllable by varying the nature of the salting-out agent – the non-coordinating organic solvent in the M(OAc)3·4H2O–Hpiv system. The following bulky single-phase samples were obtained: dimers 1 or 2 with M = Pr, Nd, Sm, Eu, and Gd using hexane C6H14; dimer 1 or 1D polymer 3 with M = Y, Er, and Yb using EtOH; dimers 2 or 4 with M = Sm using iPrOH. A reversible phase transition to a commensurate modulated modification (P21/c) was observed for crystals of 1 (Pn). The magnetic properties of complexes 1a (Pr), 1b (Nd), 4 (Sm), 1d (Eu), 1f (Dy), 1 g (Ho), and 1 h (Er) were investigated.
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Fomina I. et al. Control of the composition and crystal structure of exchange reaction products of rare-earth acetates with pivalic acid // Inorganica Chimica Acta. 2018. Vol. 482. pp. 8-15.
GOST all authors (up to 50) Copy
Fomina I., Ilyukhin A. B., Gavrikov A., Aleksandrov G. G., Fatyushina E. V., Gavrilkin S. Yu., Bogomyakov A. S., Eremenko I. L. Control of the composition and crystal structure of exchange reaction products of rare-earth acetates with pivalic acid // Inorganica Chimica Acta. 2018. Vol. 482. pp. 8-15.
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RIS Copy
TY - JOUR
DO - 10.1016/j.ica.2018.05.033
UR - https://linkinghub.elsevier.com/retrieve/pii/S0020169318305036
TI - Control of the composition and crystal structure of exchange reaction products of rare-earth acetates with pivalic acid
T2 - Inorganica Chimica Acta
AU - Fomina, I.G.
AU - Ilyukhin, Andrey B.
AU - Gavrikov, A
AU - Aleksandrov, Grygory G.
AU - Fatyushina, Elena V
AU - Gavrilkin, Sergey Yu
AU - Bogomyakov, Artem S
AU - Eremenko, Igor L.
PY - 2018
DA - 2018/10/01
PB - Elsevier
SP - 8-15
VL - 482
SN - 0020-1693
SN - 1873-3255
ER -
BibTex
Cite this
BibTex (up to 50 authors) Copy
@article{2018_Fomina,
author = {I.G. Fomina and Andrey B. Ilyukhin and A Gavrikov and Grygory G. Aleksandrov and Elena V Fatyushina and Sergey Yu Gavrilkin and Artem S Bogomyakov and Igor L. Eremenko},
title = {Control of the composition and crystal structure of exchange reaction products of rare-earth acetates with pivalic acid},
journal = {Inorganica Chimica Acta},
year = {2018},
volume = {482},
publisher = {Elsevier},
month = {oct},
url = {https://linkinghub.elsevier.com/retrieve/pii/S0020169318305036},
pages = {8--15},
doi = {10.1016/j.ica.2018.05.033}
}