Luminescent properties of binary MO-2SiO2 (M = Ca2+, Sr2+, Ba2+) glasses doped with Ce3+, Tb3+ and Dy3+
M Korjik
2
,
A. Fedorov
2
,
G Dosovitsky
3
,
O Akimova
3
,
E Gordienko
3
,
Mauro Fasoli
4
,
V Mechinsky
2
,
A. Vedda
4
,
Federico Moretti
4
Publication type: Journal Article
Publication date: 2018-10-01
scimago Q1
wos Q1
SJR: 1.192
CiteScore: 11.8
Impact factor: 6.3
ISSN: 09258388, 18734669
Materials Chemistry
Metals and Alloys
Mechanical Engineering
Mechanics of Materials
Abstract
Binary alkali-earth silicate glasses doped with Ce3+, Tb3+, and Dy3+ were obtained by melt-quenching technique and their photo- and radio-luminescence properties were investigated. The disordered structure of the glass is responsible for an inhomogeneous broadening of the electronic radiative 5d1 energy level of Ce3+ due to their localization in several positions with different surroundings, possessing a slightly different local ligand field. The influence of glass matrix composition on the Stokes shift as a function of ionic radius of the cation was shown. The radio-luminescence spectral shapes were related to the simultaneous occurrence of emissions from all Ce3+ configurations with relative weights proportional to their abundance in the glasses. The possibility of excitation of Ce3+ in different localizations was demonstrated and confirmed by the systematic shift of emission from excitation. On the contrary, no shift was observed in the Tb3+ and Dy3+ doped glasses, thanks to the lower effect of ligand field on their radiative electronic levels.
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Tratsiak Y. V. et al. Luminescent properties of binary MO-2SiO2 (M = Ca2+, Sr2+, Ba2+) glasses doped with Ce3+, Tb3+ and Dy3+ // Journal of Alloys and Compounds. 2018. Vol. 765. pp. 207-212.
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Tratsiak Y. V., Korjik M., Fedorov A., Dosovitsky G., Akimova O., Gordienko E., Fasoli M., Mechinsky V., Trusova E. E., Vedda A., Moretti F. Luminescent properties of binary MO-2SiO2 (M = Ca2+, Sr2+, Ba2+) glasses doped with Ce3+, Tb3+ and Dy3+ // Journal of Alloys and Compounds. 2018. Vol. 765. pp. 207-212.
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TY - JOUR
DO - 10.1016/j.jallcom.2018.06.210
UR - https://doi.org/10.1016/j.jallcom.2018.06.210
TI - Luminescent properties of binary MO-2SiO2 (M = Ca2+, Sr2+, Ba2+) glasses doped with Ce3+, Tb3+ and Dy3+
T2 - Journal of Alloys and Compounds
AU - Tratsiak, Yauhen V
AU - Korjik, M
AU - Fedorov, A.
AU - Dosovitsky, G
AU - Akimova, O
AU - Gordienko, E
AU - Fasoli, Mauro
AU - Mechinsky, V
AU - Trusova, Ekaterina E
AU - Vedda, A.
AU - Moretti, Federico
PY - 2018
DA - 2018/10/01
PB - Elsevier
SP - 207-212
VL - 765
SN - 0925-8388
SN - 1873-4669
ER -
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BibTex (up to 50 authors)
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@article{2018_Tratsiak,
author = {Yauhen V Tratsiak and M Korjik and A. Fedorov and G Dosovitsky and O Akimova and E Gordienko and Mauro Fasoli and V Mechinsky and Ekaterina E Trusova and A. Vedda and Federico Moretti},
title = {Luminescent properties of binary MO-2SiO2 (M = Ca2+, Sr2+, Ba2+) glasses doped with Ce3+, Tb3+ and Dy3+},
journal = {Journal of Alloys and Compounds},
year = {2018},
volume = {765},
publisher = {Elsevier},
month = {oct},
url = {https://doi.org/10.1016/j.jallcom.2018.06.210},
pages = {207--212},
doi = {10.1016/j.jallcom.2018.06.210}
}