Joule, volume 3, issue 1, pages 279-289

Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions

Publication typeJournal Article
Publication date2019-01-01
Journal: Joule
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor39.8
ISSN25424351
General Energy
Abstract
Summary The current efficiency of NH3 electrosynthesis from N2 and H2O is ultralow as a result of poor selectivity in most catalysts. Here, we demonstrate that under ambient conditions, MXene (Ti3C2Tx) nanosheets attached to a vertically aligned metal host can achieve a high faradic efficiency (5.78%) at an ultralow potential for NH3 electrosynthesis. On the basis of experimental and theoretical evidence, the basal plane of MXene is relatively inert, and its higher activity is related to a greater number of exposed edge sites. This work elucidates that significantly improved selectivity of NH3 electrosynthesis can be achieved by tuning active sites and retarding hydrogen evolution activity. The proposed strategy provides a new opportunity to optimize the surface properties of 2D catalysts for efficient N2 fixation under ambient conditions.

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GOST Copy
Luo Y. et al. Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions // Joule. 2019. Vol. 3. No. 1. pp. 279-289.
GOST all authors (up to 50) Copy
Luo Y., Chen G., Ding L., Chen X., Ding L. X., Wang H. Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions // Joule. 2019. Vol. 3. No. 1. pp. 279-289.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1016/j.joule.2018.09.011
UR - https://doi.org/10.1016%2Fj.joule.2018.09.011
TI - Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions
T2 - Joule
AU - Luo, Yaru
AU - Chen, Gaofeng
AU - Ding, Li
AU - Chen, Xinzhi
AU - Ding, Liang Xin
AU - Wang, Haihui
PY - 2019
DA - 2019/01/01 00:00:00
PB - Elsevier
SP - 279-289
IS - 1
VL - 3
SN - 2542-4351
ER -
BibTex |
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BibTex Copy
@article{2019_Luo
author = {Yaru Luo and Gaofeng Chen and Li Ding and Xinzhi Chen and Liang Xin Ding and Haihui Wang},
title = {Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions},
journal = {Joule},
year = {2019},
volume = {3},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016%2Fj.joule.2018.09.011},
number = {1},
pages = {279--289},
doi = {10.1016/j.joule.2018.09.011}
}
MLA
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MLA Copy
Luo, Yaru, et al. “Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions.” Joule, vol. 3, no. 1, Jan. 2019, pp. 279-289. https://doi.org/10.1016%2Fj.joule.2018.09.011.
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