Journal of Photochemistry and Photobiology A: Chemistry, volume 163, issue 3, pages 347-358
Comparative study of photoorientation phenomena in photosensitive azobenzene-containing homopolymers and copolymers
Publication type: Journal Article
Publication date: 2004-05-01
Quartile SCImago
Q2
Quartile WOS
Q2
Impact factor: 4.3
ISSN: 10106030, 18732666
General Chemistry
General Chemical Engineering
General Physics and Astronomy
Abstract
Peculiarities of photoorientational behavior under the action of polarized and nonpolarized light of different wavelengths on films of a homopolymer and a related copolymer were studied. The homopolymer consists of polyacrylate main chain and photosensitive azobenzene side groups, whereas the copolymer also contains nonphotosensitive bulky cholesterol-containing side groups. It was shown that the irradiation of thin spin-coated films of the polymers by polarized UV light leads to the appearance of small dichroism which is not stable under prolonged irradiation. This phenomenon associated with the photoselection and photoorientation processes takes place because only the azobenzenes with the molecular long axis perpendicular to the direction of the electric field vector of the incident light are inactive, but the others are activated for isomerization cycles accompanied by a motion of their molecular long axis until they are perpendicular to the direction of the electric field vector. The irradiation with linearly polarized visible light (436 nm) results in a strong increase of the in-plane orientation of the azobenzene groups. The maximal value of the photoinduced anisotropy is larger in the case of the copolymer. It was also found that the irradiation with nonpolarized visible light leads to an out-of-plane order in polymers films, i.e. in this case of the azobenzene moieties simultaneously adopt orientation along film normal. The comparative study of above-mentioned phenomenon allowed to find the influence of different factors, such as irradiation wavelength, polymer structure and film thickness on the kinetics, the photoinduced dichroism and the order parameter values.
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Stumpe J. et al. Comparative study of photoorientation phenomena in photosensitive azobenzene-containing homopolymers and copolymers // Journal of Photochemistry and Photobiology A: Chemistry. 2004. Vol. 163. No. 3. pp. 347-358.
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Stumpe J., Bobrovsky A., Boiko N. I., Shibaev V. Comparative study of photoorientation phenomena in photosensitive azobenzene-containing homopolymers and copolymers // Journal of Photochemistry and Photobiology A: Chemistry. 2004. Vol. 163. No. 3. pp. 347-358.
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TY - JOUR
DO - 10.1016/j.jphotochem.2004.01.021
UR - https://doi.org/10.1016%2Fj.jphotochem.2004.01.021
TI - Comparative study of photoorientation phenomena in photosensitive azobenzene-containing homopolymers and copolymers
T2 - Journal of Photochemistry and Photobiology A: Chemistry
AU - Stumpe, Joachim
AU - Bobrovsky, Alexey
AU - Boiko, N. I.
AU - Shibaev, Valery
PY - 2004
DA - 2004/05/01 00:00:00
PB - Elsevier
SP - 347-358
IS - 3
VL - 163
SN - 1010-6030
SN - 1873-2666
ER -
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@article{2004_Stumpe,
author = {Joachim Stumpe and Alexey Bobrovsky and N. I. Boiko and Valery Shibaev},
title = {Comparative study of photoorientation phenomena in photosensitive azobenzene-containing homopolymers and copolymers},
journal = {Journal of Photochemistry and Photobiology A: Chemistry},
year = {2004},
volume = {163},
publisher = {Elsevier},
month = {may},
url = {https://doi.org/10.1016%2Fj.jphotochem.2004.01.021},
number = {3},
pages = {347--358},
doi = {10.1016/j.jphotochem.2004.01.021}
}
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Stumpe, Joachim, et al. “Comparative study of photoorientation phenomena in photosensitive azobenzene-containing homopolymers and copolymers.” Journal of Photochemistry and Photobiology A: Chemistry, vol. 163, no. 3, May. 2004, pp. 347-358. https://doi.org/10.1016%2Fj.jphotochem.2004.01.021.
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