ACS Applied Nano Materials, volume 4, issue 4, pages 4208-4215
Mapping Elevated Temperatures with a Micrometer Resolution Using the Luminescence of Chemically Stable Upconversion Nanoparticles
Van Omme J Tijn
2
,
Van Den Heuvel Dave J
1
,
Vonk Sander J W
1
,
Spruit Ronald G
2
,
Meirer Florian
3
,
Pérez Garza H Hugo
2
,
Meijerink A.
1
,
Rabouw Freddy T.
3
,
Geitenbeek Robin G.
3
1
Condensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht University, Princetonplein 1, Utrecht 3584 CC, The Netherlands
|
2
DENSsolutions B.V., Informaticalaan 12, Delft 2628 ZD, The Netherlands
|
3
Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterials Science, Utrecht University, Universiteitsweg 99, Utrecht 3584 CG, The Netherlands
|
Publication type: Journal Article
Publication date: 2021-03-30
Journal:
ACS Applied Nano Materials
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 5.9
ISSN: 25740970
PubMed ID:
34085030
General Materials Science
Abstract
The temperature-sensitive luminescence of nanoparticles enables their application as remote thermometers. The size of these nanothermometers makes them ideal to map temperatures with a high spatial resolution. However, high spatial resolution mapping of temperatures >373 K has remained challenging. Here, we realize nanothermometry with high spatial resolutions at elevated temperatures using chemically stable upconversion nanoparticles and confocal microscopy. We test this method on a microelectromechanical heater and study the temperature homogeneity. Our experiments reveal distortions in the luminescence spectra that are intrinsic to high-resolution measurements of samples with nanoscale photonic inhomogeneities. In particular, the spectra are affected by the high-power excitation as well as by scattering and reflection of the emitted light. The latter effect has an increasing impact at elevated temperatures. We present a procedure to correct these distortions. As a result, we extend the range of high-resolution nanothermometry beyond 500 K with a precision of 1–4 K. This work will improve the accuracy of nanothermometry not only in micro- and nanoelectronics but also in other fields with photonically inhomogeneous substrates.
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1
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Citations by publishers
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1 publication, 1.82%
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2
4
6
8
10
12
14
16
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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van Swieten T. P. et al. Mapping Elevated Temperatures with a Micrometer Resolution Using the Luminescence of Chemically Stable Upconversion Nanoparticles // ACS Applied Nano Materials. 2021. Vol. 4. No. 4. pp. 4208-4215.
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van Swieten T. P., Van Omme J. T., Van Den Heuvel D. J., Vonk S. J. W., Spruit R. G., Meirer F., Pérez Garza H. H., Weckhuysen B. M., Meijerink A., Rabouw F. T., Geitenbeek R. G. Mapping Elevated Temperatures with a Micrometer Resolution Using the Luminescence of Chemically Stable Upconversion Nanoparticles // ACS Applied Nano Materials. 2021. Vol. 4. No. 4. pp. 4208-4215.
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TY - JOUR
DO - 10.1021/acsanm.1c00657
UR - https://doi.org/10.1021%2Facsanm.1c00657
TI - Mapping Elevated Temperatures with a Micrometer Resolution Using the Luminescence of Chemically Stable Upconversion Nanoparticles
T2 - ACS Applied Nano Materials
AU - Van Den Heuvel, Dave J
AU - van Swieten, Thomas P.
AU - Van Omme, J Tijn
AU - Vonk, Sander J W
AU - Meirer, Florian
AU - Meijerink, A.
AU - Rabouw, Freddy T.
AU - Spruit, Ronald G
AU - Pérez Garza, H Hugo
AU - Weckhuysen, Bert Marc
AU - Geitenbeek, Robin G.
PY - 2021
DA - 2021/03/30 00:00:00
PB - American Chemical Society (ACS)
SP - 4208-4215
IS - 4
VL - 4
PMID - 34085030
SN - 2574-0970
ER -
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@article{2021_van Swieten,
author = {Dave J Van Den Heuvel and Thomas P. van Swieten and J Tijn Van Omme and Sander J W Vonk and Florian Meirer and A. Meijerink and Freddy T. Rabouw and Ronald G Spruit and H Hugo Pérez Garza and Bert Marc Weckhuysen and Robin G. Geitenbeek},
title = {Mapping Elevated Temperatures with a Micrometer Resolution Using the Luminescence of Chemically Stable Upconversion Nanoparticles},
journal = {ACS Applied Nano Materials},
year = {2021},
volume = {4},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021%2Facsanm.1c00657},
number = {4},
pages = {4208--4215},
doi = {10.1021/acsanm.1c00657}
}
Cite this
MLA
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van Swieten, Thomas P., et al. “Mapping Elevated Temperatures with a Micrometer Resolution Using the Luminescence of Chemically Stable Upconversion Nanoparticles.” ACS Applied Nano Materials, vol. 4, no. 4, Mar. 2021, pp. 4208-4215. https://doi.org/10.1021%2Facsanm.1c00657.