Efficient Conversion of Methane to Aromatics by Coupling Methylation Reaction
Тип публикации: Journal Article
Дата публикации: 2016-07-20
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 3.541
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Краткое описание
We report that the coupling of methane dehydroaromatization (MDA) and methanol methylation over a Mo/HZSM-5 catalyst can realize the direct conversion of methane to benzene, toluene, and xylene (BTX) with long-time steady state (60 h), higher activity (26.4%), and selectivity of BTX (>90%) at atmospheric pressure and 973 K. Based on characterization, it was confirmed that the formed benzene can be effectively methylated by methanol, leading to high activity and stability, which proves that the coke from polycondensation of the formed benzene results in rapid deactivation of MDA.
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MLA
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ГОСТ
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Liu Y. et al. Efficient Conversion of Methane to Aromatics by Coupling Methylation Reaction // ACS Catalysis. 2016. Vol. 6. No. 8. pp. 5366-5370.
ГОСТ со всеми авторами (до 50)
Скопировать
Liu Y., Li D., Wang T., Liu Y., Teng X., Zhang Y. Efficient Conversion of Methane to Aromatics by Coupling Methylation Reaction // ACS Catalysis. 2016. Vol. 6. No. 8. pp. 5366-5370.
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RIS
Скопировать
TY - JOUR
DO - 10.1021/acscatal.6b01362
UR - https://doi.org/10.1021/acscatal.6b01362
TI - Efficient Conversion of Methane to Aromatics by Coupling Methylation Reaction
T2 - ACS Catalysis
AU - Liu, Yi
AU - Li, Defu
AU - Wang, Tianyun
AU - Liu, Yang
AU - Teng, Xu
AU - Zhang, Yi
PY - 2016
DA - 2016/07/20
PB - American Chemical Society (ACS)
SP - 5366-5370
IS - 8
VL - 6
SN - 2155-5435
ER -
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BibTex (до 50 авторов)
Скопировать
@article{2016_Liu,
author = {Yi Liu and Defu Li and Tianyun Wang and Yang Liu and Xu Teng and Yi Zhang},
title = {Efficient Conversion of Methane to Aromatics by Coupling Methylation Reaction},
journal = {ACS Catalysis},
year = {2016},
volume = {6},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/acscatal.6b01362},
number = {8},
pages = {5366--5370},
doi = {10.1021/acscatal.6b01362}
}
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MLA
Скопировать
Liu, Yi, et al. “Efficient Conversion of Methane to Aromatics by Coupling Methylation Reaction.” ACS Catalysis, vol. 6, no. 8, Jul. 2016, pp. 5366-5370. https://doi.org/10.1021/acscatal.6b01362.
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