Unusual selective allylation of norbornadiene in the presence of palladium nanoclusters
E. M. Evstigneeva
1
,
O S Manulik
1
,
V. R. Flid
1
,
I P Stolyarov
2
,
N.Yu. Kozitsyna
2
,
M.N. Vargaftik
2
,
I. I. Moiseev
2
Publication type: Journal Article
Publication date: 2004-06-01
scimago Q3
SJR: 0.305
CiteScore: 2.8
Impact factor: —
ISSN: 10665285, 15739171
General Chemistry
Abstract
The reaction of norbornadiene (NBD) with allyl acetate in the presence of the nanocluster Pd147phen32O60(OCOBut)30 (Pd-147; phen is 1,10-phenanthroline) and PPh3 in acetonitrile is nonselective and is accompanied by the decomposition of the cluster, affording the same allylation products of NBD as the reaction with Pd3(OAc)6 or Pd(dba)2 (dba is dibenzylideneacetone) combined with PPh3. In contrast, in the ionic liquid [bmim][BF4] (bmim is 1-butyl-3-methylimidazolinium), the Pd-147 is not decomposed and the reaction occurs selectively to give methylidene(vinyl)norbornene as the sole product. The data obtained suggest that in an ionic liquid, the reaction under study is catalyzed by the nanocluster Pd-147 rather than by the products of its decomposition.
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Total citations:
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Citations from 2024:
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Evstigneeva E. M. et al. Unusual selective allylation of norbornadiene in the presence of palladium nanoclusters // Russian Chemical Bulletin. 2004. Vol. 53. No. 6. pp. 1345-1348.
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Evstigneeva E. M., Manulik O. S., Flid V. R., Stolyarov I. P., Kozitsyna N., Vargaftik M., Moiseev I. I. Unusual selective allylation of norbornadiene in the presence of palladium nanoclusters // Russian Chemical Bulletin. 2004. Vol. 53. No. 6. pp. 1345-1348.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1023/B:RUCB.0000042298.81687.dd
UR - http://link.springer.com/10.1023/B:RUCB.0000042298.81687.dd
TI - Unusual selective allylation of norbornadiene in the presence of palladium nanoclusters
T2 - Russian Chemical Bulletin
AU - Evstigneeva, E. M.
AU - Manulik, O S
AU - Flid, V. R.
AU - Stolyarov, I P
AU - Kozitsyna, N.Yu.
AU - Vargaftik, M.N.
AU - Moiseev, I. I.
PY - 2004
DA - 2004/06/01
PB - Springer Nature
SP - 1345-1348
IS - 6
VL - 53
SN - 1066-5285
SN - 1573-9171
ER -
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BibTex (up to 50 authors)
Copy
@article{2004_Evstigneeva,
author = {E. M. Evstigneeva and O S Manulik and V. R. Flid and I P Stolyarov and N.Yu. Kozitsyna and M.N. Vargaftik and I. I. Moiseev},
title = {Unusual selective allylation of norbornadiene in the presence of palladium nanoclusters},
journal = {Russian Chemical Bulletin},
year = {2004},
volume = {53},
publisher = {Springer Nature},
month = {jun},
url = {http://link.springer.com/10.1023/B:RUCB.0000042298.81687.dd},
number = {6},
pages = {1345--1348},
doi = {10.1023/B:RUCB.0000042298.81687.dd}
}
Cite this
MLA
Copy
Evstigneeva, E. M., et al. “Unusual selective allylation of norbornadiene in the presence of palladium nanoclusters.” Russian Chemical Bulletin, vol. 53, no. 6, Jun. 2004, pp. 1345-1348. http://link.springer.com/10.1023/B:RUCB.0000042298.81687.dd.
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