Physical Review B, volume 104, issue 6, publication number 064510

Absence of conventional room-temperature superconductivity at high pressure in carbon-doped H3S

Wang Tianchun ¹

Hirayama Motoaki ^{1, 2}

Nomoto Takuya ¹

Koretsune Takashi ³

Arita Ryotaro ^{1, 2}

Flores-Livas José A. ^{2, 4}

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan |

RIKEN Center for Emergent Matter Science, 2-1 Hirosawa, Wako 351-0198, Japan |

Department of Physics, Tohoku University, 6-3 Aza-Aoba, Sendai 980-8578 Japan |

⁴

Dipartimento di Fisica, Università di Roma La Sapienza, Piazzale Aldo Moro 5, I-00185 Roma, Italy

Sapienza University of Rome

University of Bari Aldo Moro

Publication type: Journal Article

Publication date: 2021-08-25

American Physical Society (APS)

Journal: Physical Review B

Quartile SCImago

Quartile WOS

Impact factor: 3.7

ISSN: 24699950, 24699969, 10980121, 1550235X

DOI: 10.1103/PhysRevB.104.064510

Copy DOI

Abstract

In this work, we show that the same theoretical tools that successfully explain other hydrides systems under pressure seem to be at odds with the recently claimed conventional room temperature superconductivity of the carbonaceous sulfur hydride. We support our conclusions with I) the absence of a dominant low-enthalpy stoichiometry and crystal structure in the ternary phase diagram. II) Only the thermodynamics of C-doping phases appears to be marginally competing in enthalpy against H$_3$S. III) Accurate results of the transition temperature given by ab initio Migdal-Eliashberg calculations differ by more than 110 K to recently theoretical claims explaining the high-temperature superconductivity in carbonaceous-hydrogen sulfide. A novel mechanism of superconductivity or a breakdown of current theories in this system is possibly behind the disagreement.

By date By citations

Citations by journals

	1 2 3 4 5 6
Journal of Applied Physics	Journal of Applied Physics, 6, 15.38% Journal of Applied Physics 6 publications, 15.38%
Physical Review B	Physical Review B, 6, 15.38% Physical Review B 6 publications, 15.38%
Journal of Physics Condensed Matter	Journal of Physics Condensed Matter, 3, 7.69% Journal of Physics Condensed Matter 3 publications, 7.69%
Matter and Radiation at Extremes	Matter and Radiation at Extremes, 3, 7.69% Matter and Radiation at Extremes 3 publications, 7.69%
Physical Review Materials	Physical Review Materials, 3, 7.69% Physical Review Materials 3 publications, 7.69%
Journal of Superconductivity and Novel Magnetism	Journal of Superconductivity and Novel Magnetism, 2, 5.13% Journal of Superconductivity and Novel Magnetism 2 publications, 5.13%
ACS Omega	ACS Omega, 2, 5.13% ACS Omega 2 publications, 5.13%
Journal of Chemical Physics	Journal of Chemical Physics, 2, 5.13% Journal of Chemical Physics 2 publications, 5.13%
Advanced Materials	Advanced Materials, 1, 2.56% Advanced Materials 1 publication, 2.56%
Physical Review Research	Physical Review Research, 1, 2.56% Physical Review Research 1 publication, 2.56%
Uspekhi Fizicheskih Nauk	Uspekhi Fizicheskih Nauk, 1, 2.56% Uspekhi Fizicheskih Nauk 1 publication, 2.56%
npj Computational Materials	npj Computational Materials, 1, 2.56% npj Computational Materials 1 publication, 2.56%
Physica C: Superconductivity and its Applications	Physica C: Superconductivity and its Applications, 1, 2.56% Physica C: Superconductivity and its Applications 1 publication, 2.56%
Wiley Interdisciplinary Reviews: Computational Molecular Science	Wiley Interdisciplinary Reviews: Computational Molecular Science, 1, 2.56% Wiley Interdisciplinary Reviews: Computational Molecular Science 1 publication, 2.56%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 1, 2.56% Journal of Physical Chemistry C 1 publication, 2.56%
Chemical Communications	Chemical Communications, 1, 2.56% Chemical Communications 1 publication, 2.56%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 1, 2.56% Journal of Materials Chemistry C 1 publication, 2.56%
Research	Research, 1, 2.56% Research 1 publication, 2.56%
Physics-Uspekhi	Physics-Uspekhi, 1, 2.56% Physics-Uspekhi 1 publication, 2.56%
	1 2 3 4 5 6

Citations by publishers

	2 4 6 8 10 12
American Institute of Physics (AIP)	American Institute of Physics (AIP), 11, 28.21% American Institute of Physics (AIP) 11 publications, 28.21%
American Physical Society (APS)	American Physical Society (APS), 10, 25.64% American Physical Society (APS) 10 publications, 25.64%
IOP Publishing	IOP Publishing, 3, 7.69% IOP Publishing 3 publications, 7.69%
Springer Nature	Springer Nature, 3, 7.69% Springer Nature 3 publications, 7.69%
American Chemical Society (ACS)	American Chemical Society (ACS), 3, 7.69% American Chemical Society (ACS) 3 publications, 7.69%
Wiley	Wiley, 2, 5.13% Wiley 2 publications, 5.13%
Uspekhi Fizicheskikh Nauk Journal	Uspekhi Fizicheskikh Nauk Journal, 2, 5.13% Uspekhi Fizicheskikh Nauk Journal 2 publications, 5.13%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 2, 5.13% Royal Society of Chemistry (RSC) 2 publications, 5.13%
Elsevier	Elsevier, 1, 2.56% Elsevier 1 publication, 2.56%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 2.56% American Association for the Advancement of Science (AAAS) 1 publication, 2.56%
	2 4 6 8 10 12

We do not take into account publications that without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

{"yearsCitations":{"type":"bar","data":{"show":true,"labels":[2021,2022,2023,2024],"ids":[0,0,0,0],"codes":[0,0,0,0],"imageUrls":["","","",""],"datasets":[{"label":"Citations number","data":[6,24,6,3],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":["15.38","61.54","15.38","7.69"],"barThickness":null}]},"options":{"indexAxis":"x","maintainAspectRatio":true,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"}},"x":{"ticks":{"stepSize":1,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"}}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Citations per year","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"journals":{"type":"bar","data":{"show":true,"labels":["Journal of Applied Physics","Physical Review B","Journal of Physics Condensed Matter","Matter and Radiation at Extremes","Physical Review Materials","Journal of Superconductivity and Novel Magnetism","ACS Omega","Journal of Chemical Physics","Advanced Materials","Physical Review Research","Uspekhi Fizicheskih Nauk","npj Computational Materials","Physica C: Superconductivity and its Applications","Wiley Interdisciplinary Reviews: Computational Molecular Science","Journal of Physical Chemistry C","Chemical Communications","Journal of Materials Chemistry C","Research","Physics-Uspekhi"],"ids":[11951,25280,4579,23140,7673,23841,18901,544,25159,26813,25355,19672,9363,22866,8859,9073,3848,5257,10345],"codes":[0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0],"imageUrls":["\/storage\/images\/resized\/ARM4e6URKRsbRZvIF0vFis9DjxGloBjnBYJXbHmZ_medium.webp","\/storage\/images\/resized\/nrK64iXHTzj43wMrfN1ZoUQ0vanswGzWPN45K3jA_medium.webp","\/storage\/images\/resized\/LsKy6OnmmmRGcAU6CZgWQvNiP1polbaSLNrN7zqj_medium.webp","\/storage\/images\/resized\/ARM4e6URKRsbRZvIF0vFis9DjxGloBjnBYJXbHmZ_medium.webp","\/storage\/images\/resized\/nrK64iXHTzj43wMrfN1ZoUQ0vanswGzWPN45K3jA_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/ARM4e6URKRsbRZvIF0vFis9DjxGloBjnBYJXbHmZ_medium.webp","\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","\/storage\/images\/resized\/nrK64iXHTzj43wMrfN1ZoUQ0vanswGzWPN45K3jA_medium.webp","\/storage\/images\/resized\/FwiqB0ziXtO1uDSVpBYJ2sLrjRF4fgUy0rywXJa7_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/leiAYcRDGTSl5B1eCnwpSGqmDEUEfDPPoYisFGhT_medium.webp","\/storage\/images\/resized\/leiAYcRDGTSl5B1eCnwpSGqmDEUEfDPPoYisFGhT_medium.webp","\/storage\/images\/resized\/s10mcsCV4OAUg9O2KrqOquQC0PhyLMI8hUUkuflM_medium.webp","\/storage\/images\/resized\/FwiqB0ziXtO1uDSVpBYJ2sLrjRF4fgUy0rywXJa7_medium.webp"],"datasets":[{"label":"","data":[6,6,3,3,3,2,2,2,1,1,1,1,1,1,1,1,1,1,1],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":[15.38,15.38,7.69,7.69,7.69,5.13,5.13,5.13,2.56,2.56,2.56,2.56,2.56,2.56,2.56,2.56,2.56,2.56,2.56],"barThickness":13}]},"options":{"indexAxis":"y","maintainAspectRatio":false,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"}},"x":{"ticks":{"stepSize":null,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"}}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Journals","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"publishers":{"type":"bar","data":{"show":true,"labels":["American Institute of Physics (AIP)","American Physical Society (APS)","IOP Publishing","Springer Nature","American Chemical Society (ACS)","Wiley","Uspekhi Fizicheskikh Nauk Journal","Royal Society of Chemistry (RSC)","Elsevier","American Association for the Advancement of Science (AAAS)"],"ids":[250,1539,2075,8,40,11,6903,123,17,189],"codes":[0,0,0,0,0,0,0,0,0,0],"imageUrls":["\/storage\/images\/resized\/ARM4e6URKRsbRZvIF0vFis9DjxGloBjnBYJXbHmZ_medium.webp","\/storage\/images\/resized\/nrK64iXHTzj43wMrfN1ZoUQ0vanswGzWPN45K3jA_medium.webp","\/storage\/images\/resized\/LsKy6OnmmmRGcAU6CZgWQvNiP1polbaSLNrN7zqj_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","\/storage\/images\/resized\/FwiqB0ziXtO1uDSVpBYJ2sLrjRF4fgUy0rywXJa7_medium.webp","\/storage\/images\/resized\/leiAYcRDGTSl5B1eCnwpSGqmDEUEfDPPoYisFGhT_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/s10mcsCV4OAUg9O2KrqOquQC0PhyLMI8hUUkuflM_medium.webp"],"datasets":[{"label":"","data":[11,10,3,3,3,2,2,2,1,1],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":[28.21,25.64,7.69,7.69,7.69,5.13,5.13,5.13,2.56,2.56],"barThickness":13}]},"options":{"indexAxis":"y","maintainAspectRatio":false,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"}},"x":{"ticks":{"stepSize":null,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"}}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Publishers","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}}}

Metrics

Cite this

GOST |

Cite this

GOST Copy

Wang T. et al. Absence of conventional room-temperature superconductivity at high pressure in carbon-doped H3S // Physical Review B. 2021. Vol. 104. No. 6. 064510

GOST all authors (up to 50) Copy

Wang T., Hirayama M., Nomoto T., Koretsune T., Arita R., Flores-Livas J. A. Absence of conventional room-temperature superconductivity at high pressure in carbon-doped H3S // Physical Review B. 2021. Vol. 104. No. 6. 064510

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1103/PhysRevB.104.064510

UR - https://doi.org/10.1103%2FPhysRevB.104.064510

TI - Absence of conventional room-temperature superconductivity at high pressure in carbon-doped H3S

T2 - Physical Review B

AU - Wang, Tianchun

AU - Hirayama, Motoaki

AU - Nomoto, Takuya

AU - Koretsune, Takashi

AU - Arita, Ryotaro

AU - Flores-Livas, José A.

PY - 2021

DA - 2021/08/25 00:00:00

PB - American Physical Society (APS)

IS - 6

VL - 104

SN - 2469-9950

SN - 2469-9969

SN - 1098-0121

SN - 1550-235X

ER -

BibTex

Cite this

BibTex Copy

@article{2021_Wang,

author = {Tianchun Wang and Motoaki Hirayama and Takuya Nomoto and Takashi Koretsune and Ryotaro Arita and José A. Flores-Livas},

title = {Absence of conventional room-temperature superconductivity at high pressure in carbon-doped H3S},

journal = {Physical Review B},

year = {2021},

volume = {104},

publisher = {American Physical Society (APS)},

month = {aug},

url = {https://doi.org/10.1103%2FPhysRevB.104.064510},

number = {6},

doi = {10.1103/PhysRevB.104.064510}

}

Found error?

Publisher

American Physical Society (APS)

Journal

Physical Review B

Quartile SCImago

Quartile WOS

Impact factor

3.7

ISSN

24699950 (Print)
24699969 (Electronic)
10980121 (Print)
1550235X (Electronic)

Profiles

Arita, Ryotaro