Open Access
Optics Express, volume 28, issue 15, pages 22462
All-optical reversible control of integrated resonant cavity by a self-assembled azobenzene monolayer.
He Jinghan
1
,
Kovach Andre
2
,
Chen Dongyu
3
,
Saris Patrick J G
2
,
Yu Raymond
4
,
Armani Andrea
1
2
These Authors contributed equally to this work
Publication type: Journal Article
Publication date: 2020-07-14
Atomic and Molecular Physics, and Optics
Abstract
The next frontier in photonics will rely on the synergistic combination of disparate material systems. One unique organic molecule is azobenzene. This molecule can reversibly change conformations when optically excited in the blue (trans-to-cis) or mid-IR (cis-to-trans). Here, we form an oriented monolayer of azobenzene-containing 4-(4-diethylaminophenylazo)pyridine (Aazo) on SiO2 optical resonators. Due to the uniformity of the Aazo layers, quality factors over 106 are achieved. To control the photo-response, the density of Aazo groups is tuned by integrating methyl spacer molecules. Using a pair of lasers, the molecule is reversibly flipped between molecular conformations, inducing a refractive index change which results in a resonant wavelength shift. The magnitude of the shift scales with the relative surface density of Aazo. To investigate reproducibility and stability of the organic monolayer, three switching cycles are demonstrated, and the performance is consistent even after a device is stored in air for 6 months.
Citations by journals
1
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Macromolecules
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Macromolecules
1 publication, 14.29%
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Nanophotonics
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Nanophotonics
1 publication, 14.29%
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Nature Reviews Chemistry
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1 publication, 14.29%
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1 publication, 14.29%
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npj 2D Materials and Applications
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1 publication, 14.29%
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1
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Citations by publishers
1
2
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Springer Nature
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Springer Nature
2 publications, 28.57%
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American Chemical Society (ACS)
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American Chemical Society (ACS)
1 publication, 14.29%
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Walter de Gruyter
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Walter de Gruyter
1 publication, 14.29%
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Elsevier
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Elsevier
1 publication, 14.29%
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1
2
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He J. et al. All-optical reversible control of integrated resonant cavity by a self-assembled azobenzene monolayer. // Optics Express. 2020. Vol. 28. No. 15. p. 22462.
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He J., Kovach A., Chen D., Saris P. J. G., Yu R., Armani A. All-optical reversible control of integrated resonant cavity by a self-assembled azobenzene monolayer. // Optics Express. 2020. Vol. 28. No. 15. p. 22462.
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TY - JOUR
DO - 10.1364/OE.397776
UR - https://doi.org/10.1364%2FOE.397776
TI - All-optical reversible control of integrated resonant cavity by a self-assembled azobenzene monolayer.
T2 - Optics Express
AU - He, Jinghan
AU - Kovach, Andre
AU - Chen, Dongyu
AU - Saris, Patrick J G
AU - Yu, Raymond
AU - Armani, Andrea
PY - 2020
DA - 2020/07/14 00:00:00
PB - Optical Society of America
SP - 22462
IS - 15
VL - 28
SN - 1094-4087
ER -
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@article{2020_He
author = {Jinghan He and Andre Kovach and Dongyu Chen and Patrick J G Saris and Raymond Yu and Andrea Armani},
title = {All-optical reversible control of integrated resonant cavity by a self-assembled azobenzene monolayer.},
journal = {Optics Express},
year = {2020},
volume = {28},
publisher = {Optical Society of America},
month = {jul},
url = {https://doi.org/10.1364%2FOE.397776},
number = {15},
pages = {22462},
doi = {10.1364/OE.397776}
}
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MLA
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He, Jinghan, et al. “All-optical reversible control of integrated resonant cavity by a self-assembled azobenzene monolayer..” Optics Express, vol. 28, no. 15, Jul. 2020, p. 22462. https://doi.org/10.1364%2FOE.397776.