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Journal of Molecular Liquids, volume 242, pages 160-167

Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K

Lebedeva Elena Yu 1
Petrovskaya Svetlana G 1
Ivanova Nadezhda G 3
Publication typeJournal Article
Publication date2017-09-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor6
ISSN01677322, 18733166
Materials Chemistry
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
Spectroscopy
Atomic and Molecular Physics, and Optics
Condensed Matter Physics
Abstract
Abstract Density measurements on solutions of 2,4-dimethyl-6,8-diethyl-2,4,6,8-tatraazabicyclo[3.3.0]octane-3,7-dione or Mebicaret in normal (H2O) and heavy (D2O) water were carried out with a precision of 0.012 kg·m− 3 using the Anton Paar DMA 5000 M vibrating tube densimeter. All experiments were performed within the temperature range between 278.15 K and 318.15 K (with a step of 10 K) at the pressure to be ca. 99.6 kPa. The solution aquamolality was ranged from 0.02 to 0.2 mol ∙(55.51 mol of solvent)− 1 for each of H/D isotopically distinguishable systems compared. The standard (partial at infinite dilution) molar volumes (V2o) and expansibilities (Ep , 2o) of the solute as well as volume-related second virial coefficients (v22) were derived from the data on a solution density. The behavior of solvent isotope effects (IEs) on the considered quantities was described given the structure- and interaction-related peculiarities of the Mebicaret molecule as well as H2O and D2O media. The volume-related interaction characteristics for the solute of interest were discussed using the results of our previous densimetric and calorimetric studies with the participation of similar N-tetraalkylated glycoluril-derivatives.

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Ivanov E. et al. Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K // Journal of Molecular Liquids. 2017. Vol. 242. pp. 160-167.
GOST all authors (up to 50) Copy
Ivanov E., Lebedeva E. Yu., Petrovskaya S. G., Baranov V. V., Kravchenko A. N., Ivanova N. G. Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K // Journal of Molecular Liquids. 2017. Vol. 242. pp. 160-167.
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RIS Copy
TY - JOUR
DO - 10.1016/j.molliq.2017.07.003
UR - https://doi.org/10.1016%2Fj.molliq.2017.07.003
TI - Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K
T2 - Journal of Molecular Liquids
AU - Ivanov, Evgeniy
AU - Lebedeva, Elena Yu
AU - Petrovskaya, Svetlana G
AU - Kravchenko, Angelina N.
AU - Ivanova, Nadezhda G
AU - Baranov, Vladimir V
PY - 2017
DA - 2017/09/01 00:00:00
PB - Elsevier
SP - 160-167
VL - 242
SN - 0167-7322
SN - 1873-3166
ER -
BibTex
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BibTex Copy
@article{2017_Ivanov
author = {Evgeniy Ivanov and Elena Yu Lebedeva and Svetlana G Petrovskaya and Angelina N. Kravchenko and Nadezhda G Ivanova and Vladimir V Baranov},
title = {Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K},
journal = {Journal of Molecular Liquids},
year = {2017},
volume = {242},
publisher = {Elsevier},
month = {sep},
url = {https://doi.org/10.1016%2Fj.molliq.2017.07.003},
pages = {160--167},
doi = {10.1016/j.molliq.2017.07.003}
}
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