Open Access
Journal of Molecular Liquids, volume 242, pages 160-167
Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K
Publication type: Journal Article
Publication date: 2017-09-01
Journal:
Journal of Molecular Liquids
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 6
ISSN: 01677322, 18733166
Materials Chemistry
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
Spectroscopy
Atomic and Molecular Physics, and Optics
Condensed Matter Physics
Abstract
Abstract Density measurements on solutions of 2,4-dimethyl-6,8-diethyl-2,4,6,8-tatraazabicyclo[3.3.0]octane-3,7-dione or Mebicaret in normal (H2O) and heavy (D2O) water were carried out with a precision of 0.012 kg·m− 3 using the Anton Paar DMA 5000 M vibrating tube densimeter. All experiments were performed within the temperature range between 278.15 K and 318.15 K (with a step of 10 K) at the pressure to be ca. 99.6 kPa. The solution aquamolality was ranged from 0.02 to 0.2 mol ∙(55.51 mol of solvent)− 1 for each of H/D isotopically distinguishable systems compared. The standard (partial at infinite dilution) molar volumes (V2o) and expansibilities (Ep , 2o) of the solute as well as volume-related second virial coefficients (v22) were derived from the data on a solution density. The behavior of solvent isotope effects (IEs) on the considered quantities was described given the structure- and interaction-related peculiarities of the Mebicaret molecule as well as H2O and D2O media. The volume-related interaction characteristics for the solute of interest were discussed using the results of our previous densimetric and calorimetric studies with the participation of similar N-tetraalkylated glycoluril-derivatives.
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Ivanov E. et al. Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K // Journal of Molecular Liquids. 2017. Vol. 242. pp. 160-167.
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Ivanov E., Lebedeva E. Yu., Petrovskaya S. G., Baranov V. V., Kravchenko A. N., Ivanova N. G. Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K // Journal of Molecular Liquids. 2017. Vol. 242. pp. 160-167.
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TY - JOUR
DO - 10.1016/j.molliq.2017.07.003
UR - https://doi.org/10.1016%2Fj.molliq.2017.07.003
TI - Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K
T2 - Journal of Molecular Liquids
AU - Ivanov, Evgeniy
AU - Lebedeva, Elena Yu
AU - Petrovskaya, Svetlana G
AU - Kravchenko, Angelina N.
AU - Ivanova, Nadezhda G
AU - Baranov, Vladimir V
PY - 2017
DA - 2017/09/01 00:00:00
PB - Elsevier
SP - 160-167
VL - 242
SN - 0167-7322
SN - 1873-3166
ER -
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@article{2017_Ivanov
author = {Evgeniy Ivanov and Elena Yu Lebedeva and Svetlana G Petrovskaya and Angelina N. Kravchenko and Nadezhda G Ivanova and Vladimir V Baranov},
title = {Volume-related interaction parameters for dilute solutions of Mebicaret (2,4-dimethyl-6,8-diethylglycoluril) in normal and heavy water between 278.15 K and 318.15 K},
journal = {Journal of Molecular Liquids},
year = {2017},
volume = {242},
publisher = {Elsevier},
month = {sep},
url = {https://doi.org/10.1016%2Fj.molliq.2017.07.003},
pages = {160--167},
doi = {10.1016/j.molliq.2017.07.003}
}