Journal of Physical Chemistry A, volume 122, issue 1, pages 159-166

Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix

Publication typeJournal Article
Publication date2017-12-21
Quartile SCImago
Q2
Quartile WOS
Q2
Impact factor2.9
ISSN10895639, 15205215
Physical and Theoretical Chemistry
Abstract
We report on the complex of a noble-gas hydride HXeOH with carbon monoxide. This species is prepared via the annealing-induced H + Xe + OH···CO reaction in a xenon matrix, the OH···CO complexes being produced by VUV photolysis of the H2O···CO complexes. The H-Xe stretching mode of the HXeOH···CO complex absorbs at 1590.3 cm-1 and it is blue-shifted by 12.7 cm-1 from the H-Xe stretching band of HXeOH monomer. The observed blue shift indicates the stabilization of the H-Xe bond upon complexation, which is characteristic of complexes of noble-gas hydrides. The HXeOH···CO species is the first complex of a noble-gas hydride with carbon monoxide and the second observed complex of HXeOH. On the basis of the MP2/aug-cc-pVTZ-PP calculations, the experimental complex is assigned to the structure, where the carbon atom of CO interacts with the oxygen atom of HXeOH.

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Ryazantsev S. V. et al. Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix // Journal of Physical Chemistry A. 2017. Vol. 122. No. 1. pp. 159-166.
GOST all authors (up to 50) Copy
Ryazantsev S. V., Lundell J., Feldman V. I., Khriachtchev L. Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix // Journal of Physical Chemistry A. 2017. Vol. 122. No. 1. pp. 159-166.
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TY - JOUR
DO - 10.1021/acs.jpca.7b10293
UR - https://doi.org/10.1021%2Facs.jpca.7b10293
TI - Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix
T2 - Journal of Physical Chemistry A
AU - Ryazantsev, Sergey V
AU - Khriachtchev, Leonid
AU - Lundell, Jan
AU - Feldman, Vladimir I.
PY - 2017
DA - 2017/12/21 00:00:00
PB - American Chemical Society (ACS)
SP - 159-166
IS - 1
VL - 122
SN - 1089-5639
SN - 1520-5215
ER -
BibTex |
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BibTex Copy
@article{2017_Ryazantsev
author = {Sergey V Ryazantsev and Leonid Khriachtchev and Jan Lundell and Vladimir I. Feldman},
title = {Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix},
journal = {Journal of Physical Chemistry A},
year = {2017},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021%2Facs.jpca.7b10293},
number = {1},
pages = {159--166},
doi = {10.1021/acs.jpca.7b10293}
}
MLA
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Ryazantsev, Sergey V., et al. “Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix.” Journal of Physical Chemistry A, vol. 122, no. 1, Dec. 2017, pp. 159-166. https://doi.org/10.1021%2Facs.jpca.7b10293.
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