Advanced Functional Materials, volume 31, issue 18, pages 2100686

Ultra‐Compliant and Tough Thermochromic Polymer for Self‐Regulated Smart Windows

Publication typeJournal Article
Publication date2021-02-26
scimago Q1
SJR5.496
CiteScore29.5
Impact factor18.5
ISSN1616301X, 16163028
Electronic, Optical and Magnetic Materials
Electrochemistry
Condensed Matter Physics
Biomaterials
Abstract
Smart windows have shown powerful potential in modulating sunlight and energy management. However, there has not been a single system that can simultaneously possess all desired properties, that is, high compliance, wide tunability, and autonomous regulation. Here, a novel system based on polyhedral oligomeric silsesquioxane crosslinked poloxamer is demonstrated. The as-synthesized material simultaneously possesses a number of the desired properties for smart windows. In addition, with the incorporation of gold nanorods, the as-fabricated smart window can be operated in an autonomous fashion with its transmission being modulated automatically upon environmental temperature shifts. Finally, the high toughness and high stretchability (10 000% strain) of the material also pave a way for future applications in wearable displays or flexible window screens.
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