Angewandte Chemie - International Edition, volume 57, issue 31, pages 9749-9753
Coating Polymeric Carbon Nitride Photoanodes on Conductive Y:ZnO Nanorod Arrays for Overall Water Splitting
Publication type: Journal Article
Publication date: 2018-07-04
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
Polymeric carbon nitride (PCN) photosensitizers are proposed replacements for their inorganic counterparts in solar-to-fuel conversion via photoelectrochemical water splitting. However, intense charge recombination, primarily because of surface defects, limits the use of PCN in PEC systems. Now, photoanodes are designed by coating PCN films onto highly conductive yttrium-doped zinc oxide (Y:ZnO) nanorods (NRs) serving as charge collectors. The generation of charge carriers can therefore be promoted by this type II alignment. The charge collectors would be kept nearby for charge separation and transport to be used in the interfacial redox reactions. The photocurrent density of the polymer electrode is improved to 0.4 mA cm-2 at 1.23 V vs. the reversible hydrogen electrode in a Na2 SO4 electrolyte solution under AM 1.5 illumination. The result reveals a more than 50-fold enhancement over the PCN films achieved by powder; the efficiency can be preserved at 95 % for 160 minutes.
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Citations by publishers
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Fang Y. et al. Coating Polymeric Carbon Nitride Photoanodes on Conductive Y:ZnO Nanorod Arrays for Overall Water Splitting // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 31. pp. 9749-9753.
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Fang Y., Xu Y., Li X., Ma Y., Wang X. Coating Polymeric Carbon Nitride Photoanodes on Conductive Y:ZnO Nanorod Arrays for Overall Water Splitting // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 31. pp. 9749-9753.
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TY - JOUR
DO - 10.1002/anie.201804530
UR - https://doi.org/10.1002/anie.201804530
TI - Coating Polymeric Carbon Nitride Photoanodes on Conductive Y:ZnO Nanorod Arrays for Overall Water Splitting
T2 - Angewandte Chemie - International Edition
AU - Xu, Yuntao
AU - Li, Xiaochun
AU - Ma, Yiwen
AU - Wang, Xinchen
AU - Fang, Yuanxing
PY - 2018
DA - 2018/07/04 00:00:00
PB - Wiley
SP - 9749-9753
IS - 31
VL - 57
SN - 1433-7851
SN - 1521-3773
ER -
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@article{2018_Fang,
author = {Yuntao Xu and Xiaochun Li and Yiwen Ma and Xinchen Wang and Yuanxing Fang},
title = {Coating Polymeric Carbon Nitride Photoanodes on Conductive Y:ZnO Nanorod Arrays for Overall Water Splitting},
journal = {Angewandte Chemie - International Edition},
year = {2018},
volume = {57},
publisher = {Wiley},
month = {jul},
url = {https://doi.org/10.1002/anie.201804530},
number = {31},
pages = {9749--9753},
doi = {10.1002/anie.201804530}
}
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MLA
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Fang, Yuanxing, et al. “Coating Polymeric Carbon Nitride Photoanodes on Conductive Y:ZnO Nanorod Arrays for Overall Water Splitting.” Angewandte Chemie - International Edition, vol. 57, no. 31, Jul. 2018, pp. 9749-9753. https://doi.org/10.1002/anie.201804530.