Advanced Functional Materials, volume 22, issue 8, pages 1741-1748

High-Sensitivity p-n Junction Photodiodes Based on PbS Nanocrystal Quantum Dots

Bhola N Pal ¹

Istvan Robel ¹

Aditya D. Mohite ²

Rawiwan Laocharoensuk ²

Donald J Werder ¹

Victor I. Klimov ¹

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Center for Advanced Solar Photophysics, Chemistry Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USA. |

Center for Integrated Nanotechnologies, Los Alamos National Laboratory, Los Alamos, NM, 87545, USA. |

Publication type: Journal Article

Publication date: 2012-02-13

Wiley

Journal: Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor: 19

ISSN: 1616301X, 16163028

DOI: 10.1002/adfm.201102532

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Electronic, Optical and Magnetic Materials

Electrochemistry

Condensed Matter Physics

Biomaterials

Abstract

Chemically synthesized nanocrystal quantum dots (NQDs) are promising materials for applications in solution-processable optoelectronic devices such as light emitting diodes, photodetectors, and solar cells. Here, we fabricate and study two types of p-n junction photodiodes in which the photoactive p-layer is made from PbS NQDs while the transparent n-layer is fabricated from wide bandgap oxides (ZnO or TiO 2). By using a p-n junction architecture we are able to significantly reduce the dark current compared to earlier Schottky junction devices without reducing external quantum efficiency (EQE), which reaches values of up to ∼80%. The use of this device architecture also allows us to significantly reduce noise and obtain high detectivity (>10 12 cm Hz 1/2 W -1) extending to the near infrared past 1 μm. We observe that the spectral shape of the photoresponse exhibits a significant dependence on applied bias, and specifically, the EQE sharply increases around 500-600 nm at reverse biases greater than 1 V. We attribute this behavior to a turn-on of an additional contribution to the photocurrent due to electrons excited to the conduction band from the occupied mid-gap states.

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Citations by journals

	1 2 3 4 5 6 7
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 7, 4.83% Journal of Physical Chemistry C 7 publications, 4.83%
Advanced Functional Materials	Advanced Functional Materials, 6, 4.14% Advanced Functional Materials 6 publications, 4.14%
RSC Advances	RSC Advances, 6, 4.14% RSC Advances 6 publications, 4.14%
Advanced Materials	Advanced Materials, 5, 3.45% Advanced Materials 5 publications, 3.45%
Nanoscale	Nanoscale, 5, 3.45% Nanoscale 5 publications, 3.45%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 5, 3.45% Journal of Materials Chemistry C 5 publications, 3.45%
IEEE Transactions on Electron Devices	IEEE Transactions on Electron Devices, 5, 3.45% IEEE Transactions on Electron Devices 5 publications, 3.45%
Applied Physics Letters	Applied Physics Letters, 3, 2.07% Applied Physics Letters 3 publications, 2.07%
Nanomaterials	Nanomaterials, 3, 2.07% Nanomaterials 3 publications, 2.07%
Applied Surface Science	Applied Surface Science, 3, 2.07% Applied Surface Science 3 publications, 2.07%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 3, 2.07% Journal of Alloys and Compounds 3 publications, 2.07%
Advanced Optical Materials	Advanced Optical Materials, 3, 2.07% Advanced Optical Materials 3 publications, 2.07%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 2.07% ACS applied materials & interfaces 3 publications, 2.07%
ACS Photonics	ACS Photonics, 3, 2.07% ACS Photonics 3 publications, 2.07%
CrystEngComm	CrystEngComm, 3, 2.07% CrystEngComm 3 publications, 2.07%
Chemical Communications	Chemical Communications, 3, 2.07% Chemical Communications 3 publications, 2.07%
Sensors	Sensors, 2, 1.38% Sensors 2 publications, 1.38%
Nature Photonics	Nature Photonics, 2, 1.38% Nature Photonics 2 publications, 1.38%
Journal of Electronic Materials	Journal of Electronic Materials, 2, 1.38% Journal of Electronic Materials 2 publications, 1.38%
Scientific Reports	Scientific Reports, 2, 1.38% Scientific Reports 2 publications, 1.38%
Nanotechnology	Nanotechnology, 2, 1.38% Nanotechnology 2 publications, 1.38%
Optical Materials	Optical Materials, 2, 1.38% Optical Materials 2 publications, 1.38%
Sensors and Actuators, B: Chemical	Sensors and Actuators, B: Chemical, 2, 1.38% Sensors and Actuators, B: Chemical 2 publications, 1.38%
Small	Small, 2, 1.38% Small 2 publications, 1.38%
Advanced Science	Advanced Science, 2, 1.38% Advanced Science 2 publications, 1.38%
Nano Letters	Nano Letters, 2, 1.38% Nano Letters 2 publications, 1.38%
ACS Nano	ACS Nano, 2, 1.38% ACS Nano 2 publications, 1.38%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 2, 1.38% Journal of Physical Chemistry Letters 2 publications, 1.38%
IEEE Transactions on Nanotechnology	IEEE Transactions on Nanotechnology, 2, 1.38% IEEE Transactions on Nanotechnology 2 publications, 1.38%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 25, 17.24% Royal Society of Chemistry (RSC) 25 publications, 17.24%
American Chemical Society (ACS)	American Chemical Society (ACS), 24, 16.55% American Chemical Society (ACS) 24 publications, 16.55%
Wiley	Wiley, 23, 15.86% Wiley 23 publications, 15.86%
Elsevier	Elsevier, 18, 12.41% Elsevier 18 publications, 12.41%
Springer Nature	Springer Nature, 15, 10.34% Springer Nature 15 publications, 10.34%
IEEE	IEEE, 10, 6.9% IEEE 10 publications, 6.9%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 8, 5.52% Multidisciplinary Digital Publishing Institute (MDPI) 8 publications, 5.52%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 2.07% American Institute of Physics (AIP) 3 publications, 2.07%
IOP Publishing	IOP Publishing, 3, 2.07% IOP Publishing 3 publications, 2.07%
Taylor & Francis	Taylor & Francis, 2, 1.38% Taylor & Francis 2 publications, 1.38%
American Physical Society (APS)	American Physical Society (APS), 1, 0.69% American Physical Society (APS) 1 publication, 0.69%
Uspekhi Fizicheskikh Nauk Journal	Uspekhi Fizicheskikh Nauk Journal, 1, 0.69% Uspekhi Fizicheskikh Nauk Journal 1 publication, 0.69%
Cambridge University Press	Cambridge University Press, 1, 0.69% Cambridge University Press 1 publication, 0.69%
Pleiades Publishing	Pleiades Publishing, 1, 0.69% Pleiades Publishing 1 publication, 0.69%
Optical Society of America	Optical Society of America, 1, 0.69% Optical Society of America 1 publication, 0.69%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.69% American Association for the Advancement of Science (AAAS) 1 publication, 0.69%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.69% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.69%
	5 10 15 20 25

We do not take into account publications without a DOI.
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Pal B. N. et al. High-Sensitivity p-n Junction Photodiodes Based on PbS Nanocrystal Quantum Dots // Advanced Functional Materials. 2012. Vol. 22. No. 8. pp. 1741-1748.

GOST all authors (up to 50) Copy

Pal B. N., Robel I., Mohite A. D., Laocharoensuk R., Werder D. J., Klimov V. I. High-Sensitivity p-n Junction Photodiodes Based on PbS Nanocrystal Quantum Dots // Advanced Functional Materials. 2012. Vol. 22. No. 8. pp. 1741-1748.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1002/adfm.201102532

UR - https://doi.org/10.1002/adfm.201102532

TI - High-Sensitivity p-n Junction Photodiodes Based on PbS Nanocrystal Quantum Dots

T2 - Advanced Functional Materials

AU - Pal, Bhola N

AU - Robel, Istvan

AU - Mohite, Aditya D.

AU - Laocharoensuk, Rawiwan

AU - Werder, Donald J

AU - Klimov, Victor I.

PY - 2012

DA - 2012/02/13 00:00:00

PB - Wiley

SP - 1741-1748

IS - 8

VL - 22

SN - 1616-301X

SN - 1616-3028

ER -

BibTex |

Cite this

BibTex Copy

@article{2012_Pal,

author = {Bhola N Pal and Istvan Robel and Aditya D. Mohite and Rawiwan Laocharoensuk and Donald J Werder and Victor I. Klimov},

title = {High-Sensitivity p-n Junction Photodiodes Based on PbS Nanocrystal Quantum Dots},

journal = {Advanced Functional Materials},

year = {2012},

volume = {22},

publisher = {Wiley},

month = {feb},

url = {https://doi.org/10.1002/adfm.201102532},

number = {8},

pages = {1741--1748},

doi = {10.1002/adfm.201102532}

}

MLA

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MLA Copy

Pal, Bhola N., et al. “High-Sensitivity p-n Junction Photodiodes Based on PbS Nanocrystal Quantum Dots.” Advanced Functional Materials, vol. 22, no. 8, Feb. 2012, pp. 1741-1748. https://doi.org/10.1002/adfm.201102532.

Found error?

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Wiley

Journal

Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor

ISSN

1616301X (Print)
16163028 (Electronic)