Advanced Functional Materials, volume 27, issue 6, pages 1604629

Ag/Ag₂S Nanocrystals for High Sensitivity Near-Infrared Luminescence Nanothermometry

Diego Ruiz ¹

Saimon M. Silva ²

María Acebrón ^{1, 3}

Cristina Palencia ⁴

André Silva ¹

J. Cabanillas-Gonzalez ¹

Miguel Lopez-Haro ⁵

Ana Belén Hungrı́a ⁵

D. Jaque ^{2, 6}

B.H. Juárez ^{1, 3}

Hide authors affiliations Show authors affiliations: 6 affiliations

IMDEA Nanoscience; Faraday 9, Campus Cantoblanco 28049 Madrid Spain |

Fluorescence Imaging Group; Materials Physics Department; Faculty of Science; Universidad Autónoma de Madrid; 28049 Madrid Spain |

Applied Physical-Chemistry Department; Faculty of Science; Universidad Autónoma de Madrid; 28049 Madrid Spain |

⁴

Institute of Physical Chemistry; University of Hamburg; Grindelallee, 117 20146 Hamburg Germany |

⁵

Nanomaterials and Catalysis Lab; Cádiz University; Campus Universitario Rio San Pedro s/n 11150 Puerto Real Cádiz Spain |

⁶

Instituto Ramón y Cajal de Investigación Sanitaria; IRYCIS; Hospital Ramón y Cajal; 28034 Madrid Spain |

Publication type: Journal Article

Publication date: 2016-12-28

Wiley

Journal: Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor: 19

ISSN: 1616301X, 16163028

DOI: 10.1002/adfm.201604629

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Electronic, Optical and Magnetic Materials

Electrochemistry

Condensed Matter Physics

Biomaterials

Abstract

Temperature sensing in biological media (cells, tissues, and living organisms) has become essential in the development of the last generation of diagnostics and therapeutic strategies. Thermometry can be used for early detection of different diseases, such as cancer, stroke, or inflammation processes, one of whose incipient symptoms is the appearance of localized temperature singularities. Luminescence nanothermometry, as a tool to accurately provide temperature sensing in biological media, requires the rational design and development of nanothermometers operating in the second biological window. In this work, this is achieved using Ag/Ag2S nanocrystals as multiparametric thermal sensing probes. Temperature sensing with remarkably high sensitivity (4% °C−1) is possible through intensity‐based measurements, as their infrared emission is strongly quenched by small temperature variations within the biological range (15–50 °C). Heating also results in a remarkable redshift of the emission band, which allows for concentration‐independent temperature sensing based on infrared ratiometric measurements, with thermal sensitivity close to 2% °C−1. These results make Ag/Ag2S nanocrystals the most sensitive among all noncomposite nanothermometers operating in the second biological window reported so far, allowing for deep‐tissue temperature measurements with low uncertainty (0.2 °C).

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Citations by journals

	1 2 3 4 5 6 7
Advanced Functional Materials	Advanced Functional Materials, 7, 5.98% Advanced Functional Materials 7 publications, 5.98%
Journal of Luminescence	Journal of Luminescence, 5, 4.27% Journal of Luminescence 5 publications, 4.27%
Advanced Materials	Advanced Materials, 5, 4.27% Advanced Materials 5 publications, 4.27%
Ceramics International	Ceramics International, 4, 3.42% Ceramics International 4 publications, 3.42%
Nano Letters	Nano Letters, 4, 3.42% Nano Letters 4 publications, 3.42%
ACS applied materials & interfaces	ACS applied materials & interfaces, 4, 3.42% ACS applied materials & interfaces 4 publications, 3.42%
RSC Advances	RSC Advances, 3, 2.56% RSC Advances 3 publications, 2.56%
Advanced Science	Advanced Science, 3, 2.56% Advanced Science 3 publications, 2.56%
Small	Small, 3, 2.56% Small 3 publications, 2.56%
Laser and Photonics Reviews	Laser and Photonics Reviews, 3, 2.56% Laser and Photonics Reviews 3 publications, 2.56%
Chemistry of Materials	Chemistry of Materials, 3, 2.56% Chemistry of Materials 3 publications, 2.56%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 2.56% Journal of Materials Chemistry C 3 publications, 2.56%
Journal of Materials Chemistry B	Journal of Materials Chemistry B, 3, 2.56% Journal of Materials Chemistry B 3 publications, 2.56%
Optics and Spectroscopy (English translation of Optika i Spektroskopiya)	Optics and Spectroscopy (English translation of Optika i Spektroskopiya), 2, 1.71% Optics and Spectroscopy (English translation of Optika i Spektroskopiya) 2 publications, 1.71%
Scientific Reports	Scientific Reports, 2, 1.71% Scientific Reports 2 publications, 1.71%
Materials Research Bulletin	Materials Research Bulletin, 2, 1.71% Materials Research Bulletin 2 publications, 1.71%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 2, 1.71% Journal of Alloys and Compounds 2 publications, 1.71%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.71% Chemical Engineering Journal 2 publications, 1.71%
Advanced Engineering Materials	Advanced Engineering Materials, 2, 1.71% Advanced Engineering Materials 2 publications, 1.71%
Advanced Optical Materials	Advanced Optical Materials, 2, 1.71% Advanced Optical Materials 2 publications, 1.71%
Nanoscale	Nanoscale, 2, 1.71% Nanoscale 2 publications, 1.71%
Chemical Society Reviews	Chemical Society Reviews, 2, 1.71% Chemical Society Reviews 2 publications, 1.71%
Materials Horizons	Materials Horizons, 2, 1.71% Materials Horizons 2 publications, 1.71%
Dalton Transactions	Dalton Transactions, 2, 1.71% Dalton Transactions 2 publications, 1.71%
TrAC - Trends in Analytical Chemistry	TrAC - Trends in Analytical Chemistry, 2, 1.71% TrAC - Trends in Analytical Chemistry 2 publications, 1.71%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 1, 0.85% Journal of Physical Chemistry C 1 publication, 0.85%
ACS Photonics	ACS Photonics, 1, 0.85% ACS Photonics 1 publication, 0.85%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 1, 0.85% Journal of Materials Science: Materials in Electronics 1 publication, 0.85%
ECS Journal of Solid State Science and Technology	ECS Journal of Solid State Science and Technology, 1, 0.85% ECS Journal of Solid State Science and Technology 1 publication, 0.85%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25 30
Wiley	Wiley, 30, 25.64% Wiley 30 publications, 25.64%
Elsevier	Elsevier, 27, 23.08% Elsevier 27 publications, 23.08%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 21, 17.95% Royal Society of Chemistry (RSC) 21 publications, 17.95%
American Chemical Society (ACS)	American Chemical Society (ACS), 17, 14.53% American Chemical Society (ACS) 17 publications, 14.53%
Springer Nature	Springer Nature, 7, 5.98% Springer Nature 7 publications, 5.98%
Pleiades Publishing	Pleiades Publishing, 3, 2.56% Pleiades Publishing 3 publications, 2.56%
The Electrochemical Society	The Electrochemical Society, 1, 0.85% The Electrochemical Society 1 publication, 0.85%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 0.85% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 0.85%
Japan Society for Analytical Chemistry	Japan Society for Analytical Chemistry, 1, 0.85% Japan Society for Analytical Chemistry 1 publication, 0.85%
IOP Publishing	IOP Publishing, 1, 0.85% IOP Publishing 1 publication, 0.85%
Taylor & Francis	Taylor & Francis, 1, 0.85% Taylor & Francis 1 publication, 0.85%
Optical Society of America	Optical Society of America, 1, 0.85% Optical Society of America 1 publication, 0.85%
Cold Spring Harbor Laboratory	Cold Spring Harbor Laboratory, 1, 0.85% Cold Spring Harbor Laboratory 1 publication, 0.85%
Chinese Physical Society	Chinese Physical Society, 1, 0.85% Chinese Physical Society 1 publication, 0.85%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.85% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.85%
	5 10 15 20 25 30

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Ruiz D. et al. Ag/Ag2S Nanocrystals for High Sensitivity Near-Infrared Luminescence Nanothermometry // Advanced Functional Materials. 2016. Vol. 27. No. 6. p. 1604629.

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Ruiz D., Silva S. M., Acebrón M., Palencia C., Silva A., Cabanillas-Gonzalez J., Lopez-Haro M., Hungrı́a A. B., Jaque D., Juárez B. Ag/Ag2S Nanocrystals for High Sensitivity Near-Infrared Luminescence Nanothermometry // Advanced Functional Materials. 2016. Vol. 27. No. 6. p. 1604629.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1002/adfm.201604629

UR - https://doi.org/10.1002/adfm.201604629

TI - Ag/Ag2S Nanocrystals for High Sensitivity Near-Infrared Luminescence Nanothermometry

T2 - Advanced Functional Materials

AU - Acebrón, María

AU - Ruiz, Diego

AU - Silva, Saimon M.

AU - Palencia, Cristina

AU - Silva, André

AU - Cabanillas-Gonzalez, J.

AU - Lopez-Haro, Miguel

AU - Hungrı́a, Ana Belén

AU - Jaque, D.

AU - Juárez, B.H.

PY - 2016

DA - 2016/12/28 00:00:00

PB - Wiley

SP - 1604629

IS - 6

VL - 27

SN - 1616-301X

SN - 1616-3028

ER -

BibTex |

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BibTex Copy

@article{2016_Ruiz,

author = {María Acebrón and Diego Ruiz and Saimon M. Silva and Cristina Palencia and André Silva and J. Cabanillas-Gonzalez and Miguel Lopez-Haro and Ana Belén Hungrı́a and D. Jaque and B.H. Juárez},

title = {Ag/Ag2S Nanocrystals for High Sensitivity Near-Infrared Luminescence Nanothermometry},

journal = {Advanced Functional Materials},

year = {2016},

volume = {27},

publisher = {Wiley},

month = {dec},

url = {https://doi.org/10.1002/adfm.201604629},

number = {6},

pages = {1604629},

doi = {10.1002/adfm.201604629}

}

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Ruiz, Diego, et al. “Ag/Ag2S Nanocrystals for High Sensitivity Near-Infrared Luminescence Nanothermometry.” Advanced Functional Materials, vol. 27, no. 6, Dec. 2016, p. 1604629. https://doi.org/10.1002/adfm.201604629.

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Wiley

Journal

Advanced Functional Materials

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Quartile WOS

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1616301X (Print)
16163028 (Electronic)