Advanced Functional Materials, volume 28, issue 42, pages 1804502
Optimization of Charge Carrier Extraction in Colloidal Quantum Dots Short-Wave Infrared Photodiodes through Optical Engineering
Epimitheas Georgitzikis
1, 2
,
Pawel E Malinowski
1
,
Jorick Maes
3, 4
,
Afshin Hadipour
1
,
Zeger Hens
3, 4
,
Paul Heremans
1, 2
,
David Cheyns
1
Publication type: Journal Article
Publication date: 2018-09-06
Journal:
Advanced Functional Materials
Q1
Q1
SJR: 5.496
CiteScore: 29.5
Impact factor: 18.5
ISSN: 1616301X, 16163028
Electronic, Optical and Magnetic Materials
Electrochemistry
Condensed Matter Physics
Biomaterials
Abstract
Colloidal quantum dots (QDs) have attracted scientific interest for infrared (IR) optoelectronic devices due to their bandgap tunability and the ease of fabrication on arbitrary substrates. In this work, short-wave IR photodetectors based on lead sulfide (PbS) QDs with high detectivity and low dark current is demonstrated. Using a combination of time-resolved photoluminescence, carrier transport, and capacitance-voltage measurements, it is proved that the charge carrier diffusion length in the QD layer is negligible such that only photogenerated charges in the space charge region can be collected. To maximize the carrier extraction, an optical model for PbS QD-based photodiodes is developed, and through optical engineering, the cavity at the wavelength of choice is optimized. This universal optimization recipe is applied to detectors sensitive to wavelengths above 1.4 mu m, leading to external quantum efficiency of 30% and specific detectivity (D*) in the range of 10(12) Jones.
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Georgitzikis E. et al. Optimization of Charge Carrier Extraction in Colloidal Quantum Dots Short-Wave Infrared Photodiodes through Optical Engineering // Advanced Functional Materials. 2018. Vol. 28. No. 42. p. 1804502.
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Georgitzikis E., Malinowski P. E., Maes J., Hadipour A., Hens Z., Heremans P., Cheyns D. Optimization of Charge Carrier Extraction in Colloidal Quantum Dots Short-Wave Infrared Photodiodes through Optical Engineering // Advanced Functional Materials. 2018. Vol. 28. No. 42. p. 1804502.
Cite this
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TY - JOUR
DO - 10.1002/adfm.201804502
UR - https://doi.org/10.1002/adfm.201804502
TI - Optimization of Charge Carrier Extraction in Colloidal Quantum Dots Short-Wave Infrared Photodiodes through Optical Engineering
T2 - Advanced Functional Materials
AU - Georgitzikis, Epimitheas
AU - Malinowski, Pawel E
AU - Maes, Jorick
AU - Hadipour, Afshin
AU - Hens, Zeger
AU - Heremans, Paul
AU - Cheyns, David
PY - 2018
DA - 2018/09/06
PB - Wiley
SP - 1804502
IS - 42
VL - 28
SN - 1616-301X
SN - 1616-3028
ER -
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@article{2018_Georgitzikis,
author = {Epimitheas Georgitzikis and Pawel E Malinowski and Jorick Maes and Afshin Hadipour and Zeger Hens and Paul Heremans and David Cheyns},
title = {Optimization of Charge Carrier Extraction in Colloidal Quantum Dots Short-Wave Infrared Photodiodes through Optical Engineering},
journal = {Advanced Functional Materials},
year = {2018},
volume = {28},
publisher = {Wiley},
month = {sep},
url = {https://doi.org/10.1002/adfm.201804502},
number = {42},
pages = {1804502},
doi = {10.1002/adfm.201804502}
}
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Georgitzikis, Epimitheas, et al. “Optimization of Charge Carrier Extraction in Colloidal Quantum Dots Short-Wave Infrared Photodiodes through Optical Engineering.” Advanced Functional Materials, vol. 28, no. 42, Sep. 2018, p. 1804502. https://doi.org/10.1002/adfm.201804502.