Advanced Functional Materials, volume 30, issue 4, pages 1907379

Cation‐Exchange Synthesis of Highly Monodisperse PbS Quantum Dots from ZnS Nanorods for Efficient Infrared Solar Cells

Yong Xia ¹

Sisi Liu ¹

Kai Wang ¹

Xiaokun Yang ²

Linyuan Lian ¹

Zhiming Zhang ¹

Jungang He ³

Guijie Liang ⁴

Song Wang ⁴

Manlin Tan ⁵

Haisheng Song ²

Daoli Zhang ¹

Yamei Liu ⁶

Jiang Hong Tang ²

Matthew C Beard ⁷

Jianbing Zhang ¹

Hide authors affiliations Show authors affiliations: 7 affiliations

School of Optical and Electronic Information Huazhong University of Science and Technology 1037 Luoyu Road Wuhan Hubei 430074 China |

Wuhan National Laboratory for Optoelectronics (WNLO) and School of Engineering Sciences Huazhong University of Science and Technology Wuhan Hubei 430074 China |

School of Materials Science and Engineering Wuhan Institute of Technology Wuhan Hubei 430205 China |

⁴

Hubei Key Laboratory of Low Dimensional Optoelectronic Materials and Devices Hubei University of Arts and Science Xiangyang Hubei 441053 China |

⁵

Research Institute of Tsinghua University in Shenzhen Shenzhen Guangdong 518057 China |

⁶

Ultrafast Photophysics of Quantum Devices Department of Physics and Astronomy Clemson University Clemson SC 29634 USA |

⁷

Chemistry and Nanoscience Center National Renewable Energy Laboratory Golden CO 80401 USA |

Publication type: Journal Article

Publication date: 2019-11-04

Wiley

Journal: Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor: 19

ISSN: 1616301X, 16163028

DOI: 10.1002/adfm.201907379

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Electronic, Optical and Magnetic Materials

Electrochemistry

Condensed Matter Physics

Biomaterials

Abstract

Infrared solar cells that utilize low-bandgap colloidal quantum dots (QDs) are promising devices to enhance the utilization of solar energy by expanding the harvested photons of common photovoltaics into the infrared region. However, the present synthesis of PbS QDs cannot produce highly efficient infrared solar cells. Here, a general synthesis is developed for low-bandgap PbS QDs (0.65–1 eV) via cation exchange from ZnS nanorods (NRs). First, ZnS NRs are converted to superlattices with segregated PbS domains within each rod. Then, sulfur precursors are released via the dissolution of the ZnS NRs during the cation exchange, which promotes size focusing of PbS QDs. PbS QDs synthesized through this new method have the advantages of high monodispersity, ease-of-size control, in situ passivation of chloride, high stability, and a “clean” surface. Infrared solar cells based on these PbS QDs with different bandgaps are fabricated, using conventional ligand exchange and device structure. All of the devices produced in this manner show excellent performance, showcasing the high quality of the PbS QDs. The highest performance of infrared solar cells is achieved using ≈0.95 eV PbS QDs, exhibiting an efficiency of 10.0% under AM 1.5 solar illumination, a perovskite-filtered efficiency of 4.2%, and a silicon-filtered efficiency of 1.1%.

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ACS applied materials & interfaces	ACS applied materials & interfaces, 5, 5.95% ACS applied materials & interfaces 5 publications, 5.95%
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Advanced Science	Advanced Science, 2, 2.38% Advanced Science 2 publications, 2.38%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 2, 2.38% Journal of Physical Chemistry C 2 publications, 2.38%
Nanoscale Horizons	Nanoscale Horizons, 2, 2.38% Nanoscale Horizons 2 publications, 2.38%
Frontiers of Optoelectronics	Frontiers of Optoelectronics, 2, 2.38% Frontiers of Optoelectronics 2 publications, 2.38%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 2, 2.38% Journal of Materials Chemistry C 2 publications, 2.38%
ACS Applied Nano Materials	ACS Applied Nano Materials, 2, 2.38% ACS Applied Nano Materials 2 publications, 2.38%
SmartMat	SmartMat, 1, 1.19% SmartMat 1 publication, 1.19%
Applied Physics Letters	Applied Physics Letters, 1, 1.19% Applied Physics Letters 1 publication, 1.19%
Journal of Applied Physics	Journal of Applied Physics, 1, 1.19% Journal of Applied Physics 1 publication, 1.19%
Nature Electronics	Nature Electronics, 1, 1.19% Nature Electronics 1 publication, 1.19%
Journal of Materials Science	Journal of Materials Science, 1, 1.19% Journal of Materials Science 1 publication, 1.19%
Aerosol Science and Engineering	Aerosol Science and Engineering, 1, 1.19% Aerosol Science and Engineering 1 publication, 1.19%
Science China: Physics, Mechanics and Astronomy	Science China: Physics, Mechanics and Astronomy, 1, 1.19% Science China: Physics, Mechanics and Astronomy 1 publication, 1.19%
Science Bulletin	Science Bulletin, 1, 1.19% Science Bulletin 1 publication, 1.19%
Nano-Micro Letters	Nano-Micro Letters, 1, 1.19% Nano-Micro Letters 1 publication, 1.19%
Journal of Solid State Chemistry	Journal of Solid State Chemistry, 1, 1.19% Journal of Solid State Chemistry 1 publication, 1.19%
Journal of Materials Science and Technology	Journal of Materials Science and Technology, 1, 1.19% Journal of Materials Science and Technology 1 publication, 1.19%
Advances in Natural Sciences: Nanoscience and Nanotechnology	Advances in Natural Sciences: Nanoscience and Nanotechnology, 1, 1.19% Advances in Natural Sciences: Nanoscience and Nanotechnology 1 publication, 1.19%
iScience	iScience, 1, 1.19% iScience 1 publication, 1.19%
Nano Energy	Nano Energy, 1, 1.19% Nano Energy 1 publication, 1.19%
	1 2 3 4 5

Citations by publishers

	5 10 15 20 25 30
Wiley	Wiley, 29, 34.52% Wiley 29 publications, 34.52%
American Chemical Society (ACS)	American Chemical Society (ACS), 17, 20.24% American Chemical Society (ACS) 17 publications, 20.24%
Springer Nature	Springer Nature, 11, 13.1% Springer Nature 11 publications, 13.1%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 11, 13.1% Royal Society of Chemistry (RSC) 11 publications, 13.1%
Elsevier	Elsevier, 7, 8.33% Elsevier 7 publications, 8.33%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 2.38% American Institute of Physics (AIP) 2 publications, 2.38%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 2.38% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 2.38%
IOP Publishing	IOP Publishing, 2, 2.38% IOP Publishing 2 publications, 2.38%
Science in China Press	Science in China Press, 1, 1.19% Science in China Press 1 publication, 1.19%
American Physical Society (APS)	American Physical Society (APS), 1, 1.19% American Physical Society (APS) 1 publication, 1.19%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.19% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.19%
	5 10 15 20 25 30

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Xia Y. et al. Cation‐Exchange Synthesis of Highly Monodisperse PbS Quantum Dots from ZnS Nanorods for Efficient Infrared Solar Cells // Advanced Functional Materials. 2019. Vol. 30. No. 4. p. 1907379.

GOST all authors (up to 50) Copy

Xia Y., Liu S., Wang K., Yang X., Lian L., Zhang Z., He J., Liang G., Wang S., Tan M., Song H., Zhang D., Liu Y., Tang J. H., Beard M. C., Zhang J. Cation‐Exchange Synthesis of Highly Monodisperse PbS Quantum Dots from ZnS Nanorods for Efficient Infrared Solar Cells // Advanced Functional Materials. 2019. Vol. 30. No. 4. p. 1907379.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adfm.201907379

UR - https://doi.org/10.1002/adfm.201907379

TI - Cation‐Exchange Synthesis of Highly Monodisperse PbS Quantum Dots from ZnS Nanorods for Efficient Infrared Solar Cells

T2 - Advanced Functional Materials

AU - Yang, Xiaokun

AU - Lian, Linyuan

AU - He, Jungang

AU - Liang, Guijie

AU - Wang, Song

AU - Tan, Manlin

AU - Zhang, Jianbing

AU - Xia, Yong

AU - Liu, Sisi

AU - Wang, Kai

AU - Zhang, Zhiming

AU - Song, Haisheng

AU - Zhang, Daoli

AU - Liu, Yamei

AU - Tang, Jiang Hong

AU - Beard, Matthew C

PY - 2019

DA - 2019/11/04 00:00:00

PB - Wiley

SP - 1907379

IS - 4

VL - 30

SN - 1616-301X

SN - 1616-3028

ER -

BibTex |

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BibTex Copy

@article{2019_Xia,

author = {Xiaokun Yang and Linyuan Lian and Jungang He and Guijie Liang and Song Wang and Manlin Tan and Jianbing Zhang and Yong Xia and Sisi Liu and Kai Wang and Zhiming Zhang and Haisheng Song and Daoli Zhang and Yamei Liu and Jiang Hong Tang and Matthew C Beard},

title = {Cation‐Exchange Synthesis of Highly Monodisperse PbS Quantum Dots from ZnS Nanorods for Efficient Infrared Solar Cells},

journal = {Advanced Functional Materials},

year = {2019},

volume = {30},

publisher = {Wiley},

month = {nov},

url = {https://doi.org/10.1002/adfm.201907379},

number = {4},

pages = {1907379},

doi = {10.1002/adfm.201907379}

}

MLA

Cite this

MLA Copy

Xia, Yong, et al. “Cation‐Exchange Synthesis of Highly Monodisperse PbS Quantum Dots from ZnS Nanorods for Efficient Infrared Solar Cells.” Advanced Functional Materials, vol. 30, no. 4, Nov. 2019, p. 1907379. https://doi.org/10.1002/adfm.201907379.

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Publisher

Wiley

Journal

Advanced Functional Materials

Quartile SCImago

Quartile WOS

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1616301X (Print)
16163028 (Electronic)