Advanced Functional Materials, volume 31, issue 28, pages 2101523

Facile Design of Sulfide‐Based all Solid‐State Lithium Metal Battery: In Situ Polymerization within Self‐Supported Porous Argyrodite Skeleton

YANTAO WANG ^{1, 2}

Jiangwei Ju ¹

Shanmu Dong ¹

Yiyuan Yan ¹

Feng Jiang ¹

Longfei Cui ¹

Qinglei Wang ¹

Xiaoqi Han ¹

Guanglei Cui ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

Qingdao Industrial Energy Storage Research Institute Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao 266101 P. R. China |

School of Future Technology University of Chinese Academy of Sciences Beijing 100049 P. R. China |

Publication type: Journal Article

Publication date: 2021-04-29

Wiley

Journal: Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor: 19

ISSN: 1616301X, 16163028

DOI: 10.1002/adfm.202101523

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Electronic, Optical and Magnetic Materials

Electrochemistry

Condensed Matter Physics

Biomaterials

Abstract

All solid-state batteries holds great promise for superiorly safe and high energy electrochemical energy storage. The ionic conductivity of electrolytes and its interfacial compatibility with the electrode are two critical factors in determining the electrochemical performance of all solid-state batteries. It is a great challenge to simultaneously demonstrate fantastic ionic conductivity and compatible electrolyte/electrode interface to acquire a well-performed all solid-state battery. By in situ polymerizing poly(ethylene glycol) methyl ether acrylate within a self-supported 3D porous Li-argyrodite (Li6PS5Cl) skeleton, the two bottlenecks are tackled successfully at once. As a result, all solid-state lithium metal batteries with a 4.5 V LiNi0.8Mn0.1Co0.1O2 cathode designed by this integrated strategy demonstrates a high Coulombic efficiency exceeding 99% at room temperature. Solid-state nuclear magnetic resonance data suggest that Li+ mainly migrates along the continuous Li6PS5Cl phase to result in a room temperature conductivity of 4.6 × 10−4 S cm−1, which is 128 times higher than that of the corresponding polymer. Meanwhile, the inferior solid–solid electrolyte/electrode interface is integrated via in situ polymerization to lessen the interfacial resistance significantly. This study thereby provides a very promising strategy of solid electrolyte design to simultaneously meet both high ionic conductivity and good interfacial compatibility towards practical high-energy-density all solid-state lithium batteries.

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ACS applied materials & interfaces	ACS applied materials & interfaces, 10, 11.36% ACS applied materials & interfaces 10 publications, 11.36%
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Chemical Engineering Journal	Chemical Engineering Journal, 5, 5.68% Chemical Engineering Journal 5 publications, 5.68%
Nano-Micro Letters	Nano-Micro Letters, 4, 4.55% Nano-Micro Letters 4 publications, 4.55%
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Journal of Energy Chemistry	Journal of Energy Chemistry, 3, 3.41% Journal of Energy Chemistry 3 publications, 3.41%
Advanced Functional Materials	Advanced Functional Materials, 3, 3.41% Advanced Functional Materials 3 publications, 3.41%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 3, 3.41% Journal of Materials Chemistry A 3 publications, 3.41%
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Electrochemical Energy Reviews	Electrochemical Energy Reviews, 2, 2.27% Electrochemical Energy Reviews 2 publications, 2.27%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 2, 2.27% Journal of Colloid and Interface Science 2 publications, 2.27%
Energy & Environmental Materials	Energy & Environmental Materials, 2, 2.27% Energy & Environmental Materials 2 publications, 2.27%
Angewandte Chemie	Angewandte Chemie, 2, 2.27% Angewandte Chemie 2 publications, 2.27%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 2, 2.27% Angewandte Chemie - International Edition 2 publications, 2.27%
Advanced Materials	Advanced Materials, 2, 2.27% Advanced Materials 2 publications, 2.27%
Applied Physics Letters	Applied Physics Letters, 1, 1.14% Applied Physics Letters 1 publication, 1.14%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 1, 1.14% Journal of the Electrochemical Society 1 publication, 1.14%
RSC Advances	RSC Advances, 1, 1.14% RSC Advances 1 publication, 1.14%
Frontiers in Chemistry	Frontiers in Chemistry, 1, 1.14% Frontiers in Chemistry 1 publication, 1.14%
Nano Research	Nano Research, 1, 1.14% Nano Research 1 publication, 1.14%
Journal of Membrane Science	Journal of Membrane Science, 1, 1.14% Journal of Membrane Science 1 publication, 1.14%
Chemical Engineering Science	Chemical Engineering Science, 1, 1.14% Chemical Engineering Science 1 publication, 1.14%
eTransportation	eTransportation, 1, 1.14% eTransportation 1 publication, 1.14%
Journal of Power Sources	Journal of Power Sources, 1, 1.14% Journal of Power Sources 1 publication, 1.14%
Batteries & Supercaps	Batteries & Supercaps, 1, 1.14% Batteries & Supercaps 1 publication, 1.14%
Carbon Energy	Carbon Energy, 1, 1.14% Carbon Energy 1 publication, 1.14%
InfoMat	InfoMat, 1, 1.14% InfoMat 1 publication, 1.14%
Small Structures	Small Structures, 1, 1.14% Small Structures 1 publication, 1.14%
Macromolecular Chemistry and Physics	Macromolecular Chemistry and Physics, 1, 1.14% Macromolecular Chemistry and Physics 1 publication, 1.14%
	2 4 6 8 10

Citations by publishers

	5 10 15 20 25 30 35
Wiley	Wiley, 32, 36.36% Wiley 32 publications, 36.36%
Elsevier	Elsevier, 16, 18.18% Elsevier 16 publications, 18.18%
American Chemical Society (ACS)	American Chemical Society (ACS), 14, 15.91% American Chemical Society (ACS) 14 publications, 15.91%
Springer Nature	Springer Nature, 11, 12.5% Springer Nature 11 publications, 12.5%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 8, 9.09% Royal Society of Chemistry (RSC) 8 publications, 9.09%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 1.14% American Institute of Physics (AIP) 1 publication, 1.14%
The Electrochemical Society	The Electrochemical Society, 1, 1.14% The Electrochemical Society 1 publication, 1.14%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.14% Frontiers Media S.A. 1 publication, 1.14%
Tsinghua University Press	Tsinghua University Press, 1, 1.14% Tsinghua University Press 1 publication, 1.14%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.14% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.14%
	5 10 15 20 25 30 35

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WANG Y. et al. Facile Design of Sulfide‐Based all Solid‐State Lithium Metal Battery: In Situ Polymerization within Self‐Supported Porous Argyrodite Skeleton // Advanced Functional Materials. 2021. Vol. 31. No. 28. p. 2101523.

GOST all authors (up to 50) Copy

WANG Y., Ju J., Dong S., Yan Y., Jiang F., Cui L., Wang Q., Han X., Cui G. Facile Design of Sulfide‐Based all Solid‐State Lithium Metal Battery: In Situ Polymerization within Self‐Supported Porous Argyrodite Skeleton // Advanced Functional Materials. 2021. Vol. 31. No. 28. p. 2101523.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adfm.202101523

UR - https://doi.org/10.1002/adfm.202101523

TI - Facile Design of Sulfide‐Based all Solid‐State Lithium Metal Battery: In Situ Polymerization within Self‐Supported Porous Argyrodite Skeleton

T2 - Advanced Functional Materials

AU - WANG, YANTAO

AU - Dong, Shanmu

AU - Yan, Yiyuan

AU - Cui, Longfei

AU - Wang, Qinglei

AU - Han, Xiaoqi

AU - Cui, Guanglei

AU - Ju, Jiangwei

AU - Jiang, Feng

PY - 2021

DA - 2021/04/29 00:00:00

PB - Wiley

SP - 2101523

IS - 28

VL - 31

SN - 1616-301X

SN - 1616-3028

ER -

BibTex |

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BibTex Copy

@article{2021_WANG,

author = {YANTAO WANG and Shanmu Dong and Yiyuan Yan and Longfei Cui and Qinglei Wang and Xiaoqi Han and Guanglei Cui and Jiangwei Ju and Feng Jiang},

title = {Facile Design of Sulfide‐Based all Solid‐State Lithium Metal Battery: In Situ Polymerization within Self‐Supported Porous Argyrodite Skeleton},

journal = {Advanced Functional Materials},

year = {2021},

volume = {31},

publisher = {Wiley},

month = {apr},

url = {https://doi.org/10.1002/adfm.202101523},

number = {28},

pages = {2101523},

doi = {10.1002/adfm.202101523}

}

MLA

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MLA Copy

WANG, YANTAO, et al. “Facile Design of Sulfide‐Based all Solid‐State Lithium Metal Battery: In Situ Polymerization within Self‐Supported Porous Argyrodite Skeleton.” Advanced Functional Materials, vol. 31, no. 28, Apr. 2021, p. 2101523. https://doi.org/10.1002/adfm.202101523.

Found error?

Publisher

Wiley

Journal

Advanced Functional Materials

Quartile SCImago

Quartile WOS

Impact factor

ISSN

1616301X (Print)
16163028 (Electronic)