Advanced Functional Materials, volume 32, issue 24, pages 2201498
Interface Engineering of a Ceramic Electrolyte by Ta 2 O 5 Nanofilms for Ultrastable Lithium Metal Batteries
Publication type: Journal Article
Publication date: 2022-03-08
Journal:
Advanced Functional Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 19
ISSN: 1616301X, 16163028
Electronic, Optical and Magnetic Materials
Electrochemistry
Condensed Matter Physics
Biomaterials
Abstract
Solid-state batteries (SSBs) are promising for next-generation energy storage with advantages in both energy density and safety, but are challenged by the poor solid-to-solid contact between solid-state electrolytes (SSEs) and electrodes, particularly the lithium anode. Herein, a facile coordination-assisted deposition process is employed to build artificial Ta2O5 nanofilms on SSEs, which is lithiophilic and has high stability against metallic lithium, thereby ensuring an intimate and stable interface between SSEs and lithium anode to sustain extended cycles. The feasibility is verified by using Li6.5La3Zr1.5Ta0.5O12 (LLZT), a garnet-typed SSEs, as a model system. It is shown that a 12 nm Ta2O5 nanofilm is able to significantly decrease the interfacial resistance from 1258 to 9 Ω cm2 with a high critical current density reaching 2.0 mA cm−2 for the assembled symmetric cell, which shows an unprecedented capability to survive long-term cycling over 5200 h. This control strategy is also able to enable the use of the commercialized cathode materials of LiFePO4 and LiNi0.83Co0.07Mn0.1O2 in SSBs with both high reversible capacity and cycling capability. The study opens up a research avenue for the delicately carved interlayers through a scalable and reliable manufacturing process which can accelerate the commercialization of SSEs.
Top-30
Citations by journals
|
1
2
3
4
|
|
|
Advanced Functional Materials
4 publications, 16.67%
|
|
|
Journal of Alloys and Compounds
2 publications, 8.33%
|
|
|
Interdisciplinary Materials
2 publications, 8.33%
|
|
|
Rare Metals
2 publications, 8.33%
|
|
|
Applied Physics Letters
1 publication, 4.17%
|
|
|
Batteries
1 publication, 4.17%
|
|
|
Ionics
1 publication, 4.17%
|
|
|
Cell Reports Physical Science
1 publication, 4.17%
|
|
|
Advanced Energy Materials
1 publication, 4.17%
|
|
|
Chemical Engineering Journal
1 publication, 4.17%
|
|
|
Nano Research
1 publication, 4.17%
|
|
|
Energy & Fuels
1 publication, 4.17%
|
|
|
ACS applied materials & interfaces
1 publication, 4.17%
|
|
|
Journal of Power Sources
1 publication, 4.17%
|
|
|
Progress in Materials Science
1 publication, 4.17%
|
|
|
Materials Chemistry Frontiers
1 publication, 4.17%
|
|
|
Electrochemical Energy Reviews
1 publication, 4.17%
|
|
|
Russian Chemical Reviews
1 publication, 4.17%
|
|
|
1
2
3
4
|
Citations by publishers
|
1
2
3
4
5
6
7
|
|
|
Wiley
7 publications, 29.17%
|
|
|
Elsevier
6 publications, 25%
|
|
|
Springer Nature
3 publications, 12.5%
|
|
|
American Chemical Society (ACS)
2 publications, 8.33%
|
|
|
Nonferrous Metals Society of China
2 publications, 8.33%
|
|
|
American Institute of Physics (AIP)
1 publication, 4.17%
|
|
|
Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 4.17%
|
|
|
Royal Society of Chemistry (RSC)
1 publication, 4.17%
|
|
|
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 4.17%
|
|
|
1
2
3
4
5
6
7
|
- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
{"yearsCitations":{"type":"bar","data":{"show":true,"labels":[2022,2023,2024],"ids":[0,0,0],"codes":[0,0,0],"imageUrls":["","",""],"datasets":[{"label":"Citations number","data":[8,10,6],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6"],"percentage":["33.33","41.67","25"],"barThickness":null}]},"options":{"indexAxis":"x","maintainAspectRatio":true,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":false},"x":{"ticks":{"stepSize":1,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":false}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Citations per year","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"journals":{"type":"bar","data":{"show":true,"labels":["Advanced Functional Materials","Journal of Alloys and Compounds","Interdisciplinary Materials","Rare Metals","Applied Physics Letters","Batteries","Ionics","Cell Reports Physical Science","Advanced Energy Materials","Chemical Engineering Journal","Nano Research","Energy & Fuels","ACS applied materials & interfaces","Journal of Power Sources","Progress in Materials Science","Materials Chemistry Frontiers","Electrochemical Energy Reviews","Russian Chemical Reviews"],"ids":[7715,4015,30049,18829,4202,19798,12191,26452,22475,16275,12211,10347,1458,14844,21250,7063,25884,23802],"codes":[0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0,0],"imageUrls":["\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","","\/storage\/images\/resized\/ARM4e6URKRsbRZvIF0vFis9DjxGloBjnBYJXbHmZ_medium.webp","\/storage\/images\/resized\/MjH1ITP7lMYGxeqUZfkt2BnVLgjkk413jwBV97XX_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/leiAYcRDGTSl5B1eCnwpSGqmDEUEfDPPoYisFGhT_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/9Mus3KG1Tkd7Bwaurt8H3RwWh0CxRlGoO6ng9UK1_medium.webp"],"datasets":[{"label":"","data":[4,2,2,2,1,1,1,1,1,1,1,1,1,1,1,1,1,1],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":[16.67,8.33,8.33,8.33,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17,4.17],"barThickness":13}]},"options":{"indexAxis":"y","maintainAspectRatio":false,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":false},"x":{"ticks":{"stepSize":null,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":false}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Journals","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"publishers":{"type":"bar","data":{"show":true,"labels":["Wiley","Elsevier","Springer Nature","American Chemical Society (ACS)","Nonferrous Metals Society of China","American Institute of Physics (AIP)","Multidisciplinary Digital Publishing Institute (MDPI)","Royal Society of Chemistry (RSC)","Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii"],"ids":[11,17,8,40,1585,250,202,123,9422],"codes":[0,0,0,0,0,0,0,0,0],"imageUrls":["\/storage\/images\/resized\/bRyGpdm98BkAUYiK1YFNpl5Z7hPu6Gd87gbIeuG3_medium.webp","\/storage\/images\/resized\/GDnYOu1UpMMfMMRV6Aqle4H0YLLsraeD9IP9qScG_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","","\/storage\/images\/resized\/ARM4e6URKRsbRZvIF0vFis9DjxGloBjnBYJXbHmZ_medium.webp","\/storage\/images\/resized\/MjH1ITP7lMYGxeqUZfkt2BnVLgjkk413jwBV97XX_medium.webp","\/storage\/images\/resized\/leiAYcRDGTSl5B1eCnwpSGqmDEUEfDPPoYisFGhT_medium.webp","\/storage\/images\/resized\/9Mus3KG1Tkd7Bwaurt8H3RwWh0CxRlGoO6ng9UK1_medium.webp"],"datasets":[{"label":"","data":[7,6,3,2,2,1,1,1,1],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":[29.17,25,12.5,8.33,8.33,4.17,4.17,4.17,4.17],"barThickness":13}]},"options":{"indexAxis":"y","maintainAspectRatio":false,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":false},"x":{"ticks":{"stepSize":null,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":false}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Publishers","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"yearsCitationsQuartiles":{"type":"bar","data":{"show":true,"labels":[2022,2023,2024],"ids":[],"codes":[],"imageUrls":[],"datasets":[{"label":"Q4","backgroundColor":"rgb(221,90,78)","data":[0,0,0],"percentage":["0","0","0"]},{"label":"Q3","backgroundColor":"rgb(251, 163,83)","data":[0,0,0],"percentage":["0","0","0"]},{"label":"Q2","backgroundColor":"rgb(232, 213, 89)","data":[2,0,0],"percentage":["8.33","0","0"]},{"label":"Q1","backgroundColor":"rgb(164, 207, 99)","data":[6,9,5],"percentage":["25","37.5","20.83"]},{"label":"Quartile not defined","backgroundColor":"#E5E7EB","data":[0,1,1],"percentage":["0","4.17","4.17"]}]},"options":{"indexAxis":"x","maintainAspectRatio":true,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":true},"x":{"ticks":{"stepSize":1,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":true}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Citations quartiles by SCImago per year","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"yearsCitationsQuartilesWs":{"type":"bar","data":{"show":true,"labels":[2022,2023,2024],"ids":[],"codes":[],"imageUrls":[],"datasets":[{"label":"Q4","backgroundColor":"rgb(221,90,78)","data":[0,0,0],"percentage":["0","0","0"]},{"label":"Q3","backgroundColor":"rgb(251, 163,83)","data":[0,0,0],"percentage":["0","0","0"]},{"label":"Q2","backgroundColor":"rgb(232, 213, 89)","data":[3,0,0],"percentage":["12.5","0","0"]},{"label":"Q1","backgroundColor":"rgb(164, 207, 99)","data":[5,9,5],"percentage":["20.83","37.5","20.83"]},{"label":"Quartile not defined","backgroundColor":"#E5E7EB","data":[0,1,1],"percentage":["0","4.17","4.17"]}]},"options":{"indexAxis":"x","maintainAspectRatio":true,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":true},"x":{"ticks":{"stepSize":1,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"},"stacked":true}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Citations quartiles by WoS per year","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}}}
Are you a researcher?
Create a profile to get free access to personal recommendations for colleagues and new articles.
Metrics
Cite this
GOST |
RIS |
BibTex |
MLA
Cite this
GOST
Copy
Guo S. et al. Interface Engineering of a Ceramic Electrolyte by Ta 2 O 5 Nanofilms for Ultrastable Lithium Metal Batteries // Advanced Functional Materials. 2022. Vol. 32. No. 24. p. 2201498.
GOST all authors (up to 50)
Copy
Guo S., Wu T., Sun Y., Zhang S. D., Li B., Zhang H. S., Qi M. Y., Liu X. H., Cao A., Wan L. Interface Engineering of a Ceramic Electrolyte by Ta 2 O 5 Nanofilms for Ultrastable Lithium Metal Batteries // Advanced Functional Materials. 2022. Vol. 32. No. 24. p. 2201498.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/adfm.202201498
UR - https://doi.org/10.1002/adfm.202201498
TI - Interface Engineering of a Ceramic Electrolyte by Ta 2 O 5 Nanofilms for Ultrastable Lithium Metal Batteries
T2 - Advanced Functional Materials
AU - Guo, Sijie
AU - Wu, Ting-Ting
AU - Sun, Yong-Gang
AU - Zhang, Si Dong
AU - Zhang, Hong Shen
AU - Qi, Mu Yao
AU - Liu, Xian Hu
AU - Cao, Anmin
AU - Wan, Lijun
AU - Li, Bing
PY - 2022
DA - 2022/03/08 00:00:00
PB - Wiley
SP - 2201498
IS - 24
VL - 32
SN - 1616-301X
SN - 1616-3028
ER -
Cite this
BibTex
Copy
@article{2022_Guo,
author = {Sijie Guo and Ting-Ting Wu and Yong-Gang Sun and Si Dong Zhang and Hong Shen Zhang and Mu Yao Qi and Xian Hu Liu and Anmin Cao and Lijun Wan and Bing Li},
title = {Interface Engineering of a Ceramic Electrolyte by Ta 2 O 5 Nanofilms for Ultrastable Lithium Metal Batteries},
journal = {Advanced Functional Materials},
year = {2022},
volume = {32},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/adfm.202201498},
number = {24},
pages = {2201498},
doi = {10.1002/adfm.202201498}
}
Cite this
MLA
Copy
Guo, Sijie, et al. “Interface Engineering of a Ceramic Electrolyte by Ta 2 O 5 Nanofilms for Ultrastable Lithium Metal Batteries.” Advanced Functional Materials, vol. 32, no. 24, Mar. 2022, p. 2201498. https://doi.org/10.1002/adfm.202201498.