Advanced Functional Materials, volume 32, issue 34, pages 2203551
Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries
Boran Tao
1, 2, 3
,
Chaojun Ren
4
,
Hongda Li
1, 2
,
Baosheng Liu
1
,
Xiaobo Jia
1
,
Xinwei Dong
1
,
SHAOHUI ZHANG
1
,
Haixin Chang
2, 3
4
Beijing Aerospace Propulsion Institute No.1 South Dahongmen Road Beijing 100076 China
|
Publication type: Journal Article
Publication date: 2022-06-29
Journal:
Advanced Functional Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 19
ISSN: 1616301X, 16163028
Electronic, Optical and Magnetic Materials
Electrochemistry
Condensed Matter Physics
Biomaterials
Abstract
As an integral part of all-solid-state lithium (Li) batteries (ASSLBs), solid-state electrolytes (SSEs) must meet requirements in high ionic conductivity, electrochemical/chemical stability toward the electrode. The ionic conductivity of the Li super ionic conductor (LISICON) is limited, and the thio-LISICON is improved by replacing O2− in the LISICON with S2−. Currently, the ionic conductivity of Li10GeP2S12 (LGPS) has exceeded 10 mS cm−1, which meets the demands of commercial ASSLBs. However, poor stability of SSEs, baneful interfacial reactions, Li dendrite growth, and other factors have impeded the development of ASSLBs. Hence, this review first traces the development progress of thio-/LISICON and LGPS-type SSEs, analyzes the complicated ion transport mechanism, and summarizes the effective strategies for improving ionic conductivity. Moreover, exciting methods focusing on electrode interface engineering are outlined separately. As to SSE/anode interface, poor chemical or electrochemical compatibility, poor interfacial contact, and the mechanisms of dendrite formation are discussed. For the SSE/cathode interface, poor interfacial stability and non-intimate solid–solid contact are daunting challenges. Then, effective methods to improve interface stability and electrochemical performance of ASSLBs with LGPS-type SSEs are introduced. Finally, combined with the present chances and challenges, the possible future developing directions of LGPS-based ASSLBs and the perspectives are proposed.
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Citations by publishers
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6
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10
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18
20
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Elsevier
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2 publications, 4.08%
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2 publications, 4.08%
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1 publication, 2.04%
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Hindawi Limited
1 publication, 2.04%
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OAE Publishing Inc.
1 publication, 2.04%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 2.04%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Tao B. et al. Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries // Advanced Functional Materials. 2022. Vol. 32. No. 34. p. 2203551.
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Tao B., Ren C., Li H., Liu B., Jia X., Dong X., ZHANG S., Chang H. Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries // Advanced Functional Materials. 2022. Vol. 32. No. 34. p. 2203551.
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TY - JOUR
DO - 10.1002/adfm.202203551
UR - https://doi.org/10.1002/adfm.202203551
TI - Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries
T2 - Advanced Functional Materials
AU - Tao, Boran
AU - Ren, Chaojun
AU - Li, Hongda
AU - Liu, Baosheng
AU - Jia, Xiaobo
AU - Dong, Xinwei
AU - ZHANG, SHAOHUI
AU - Chang, Haixin
PY - 2022
DA - 2022/06/29 00:00:00
PB - Wiley
SP - 2203551
IS - 34
VL - 32
SN - 1616-301X
SN - 1616-3028
ER -
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@article{2022_Tao,
author = {Boran Tao and Chaojun Ren and Hongda Li and Baosheng Liu and Xiaobo Jia and Xinwei Dong and SHAOHUI ZHANG and Haixin Chang},
title = {Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries},
journal = {Advanced Functional Materials},
year = {2022},
volume = {32},
publisher = {Wiley},
month = {jun},
url = {https://doi.org/10.1002/adfm.202203551},
number = {34},
pages = {2203551},
doi = {10.1002/adfm.202203551}
}
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MLA
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Tao, Boran, et al. “Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries.” Advanced Functional Materials, vol. 32, no. 34, Jun. 2022, p. 2203551. https://doi.org/10.1002/adfm.202203551.