Advanced Materials, volume 31, issue 17, pages 1805580

A Facet‐Specific Quantum Dot Passivation Strategy for Colloid Management and Efficient Infrared Photovoltaics

Younghoon Kim ¹

Fanglin Che ¹

Jea Woong Jo ¹

Taiho Park ¹

F. Pelayo García de Arquer ¹

Oleksandr Voznyy ¹

Bin Sun ¹

Jung Hwan Kim ¹

Min-Jae Choi ¹

Rafael Quintero-Torres ¹

Fengjia Fan ¹

Chih Shan Tan ¹

Eva Bladt ²

Grant C. Walters ¹

Andrew H. Proppe ¹

Chengqin Zou ¹

Haifeng Yuan ^{1, 3}

Sara Bals ²

J. Hofkens ³

Maarten Roeffaers ⁴

Sjoerd Hoogland ¹

Edward H. Sargent ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of Electrical and Computer EngineeringUniversity of Toronto 10 King's College Road Toronto Ontario M5S 3G4 Canada |

Electron Microscopy for Materials Science (EMAT)University of Antwerp Groenenborgerlaan 171 B‐2020 Antwerp Belgium |

Departement of ChemistryKU Leuven Celestijnenlaan 200F 3001 Heverlee Belgium |

⁴

Center for Surface Chemistry and CatalysisFaculty of Bioscience EngineeringKU Leuven 3001 Heverlee Belgium |

Publication type: Journal Article

Publication date: 2019-03-12

Wiley

Journal: Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor: 29.4

ISSN: 09359648, 15214095

DOI: 10.1002/adma.201805580

Copy DOI

General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

Colloidal nanocrystals combine size- and facet-dependent properties with solution processing. They offer thus a compelling suite of materials for technological applications. Their size- and facet-tunable features are studied in synthesis; however, to exploit their features in optoelectronic devices, it will be essential to translate control over size and facets from the colloid all the way to the film. Larger-diameter colloidal quantum dots (CQDs) offer the attractive possibility of harvesting infrared (IR) solar energy beyond absorption of silicon photovoltaics. These CQDs exhibit facets (nonpolar (100)) undisplayed in small-diameter CQDs; and the materials chemistry of smaller nanocrystals fails consequently to translate to materials for the short-wavelength IR regime. A new colloidal management strategy targeting the passivation of both (100) and (111) facets is demonstrated using distinct choices of cations and anions. The approach leads to narrow-bandgap CQDs with impressive colloidal stability and photoluminescence quantum yield. Photophysical studies confirm a reduction both in Stokes shift (≈47 meV) and Urbach tail (≈29 meV). This approach provides a ≈50% increase in the power conversion efficiency of IR photovoltaics compared to controls, and a ≈70% external quantum efficiency at their excitonic peak.

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	1 2 3 4 5 6 7 8
ACS applied materials & interfaces	ACS applied materials & interfaces, 8, 8.7% ACS applied materials & interfaces 8 publications, 8.7%
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Advanced Functional Materials	Advanced Functional Materials, 4, 4.35% Advanced Functional Materials 4 publications, 4.35%
Advanced Energy Materials	Advanced Energy Materials, 4, 4.35% Advanced Energy Materials 4 publications, 4.35%
Small	Small, 4, 4.35% Small 4 publications, 4.35%
ACS Energy Letters	ACS Energy Letters, 4, 4.35% ACS Energy Letters 4 publications, 4.35%
Advanced Optical Materials	Advanced Optical Materials, 3, 3.26% Advanced Optical Materials 3 publications, 3.26%
ACS Applied Nano Materials	ACS Applied Nano Materials, 3, 3.26% ACS Applied Nano Materials 3 publications, 3.26%
Applied Sciences (Switzerland)	Applied Sciences (Switzerland), 2, 2.17% Applied Sciences (Switzerland) 2 publications, 2.17%
Nature Communications	Nature Communications, 2, 2.17% Nature Communications 2 publications, 2.17%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 2, 2.17% Solar Energy Materials and Solar Cells 2 publications, 2.17%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 2.17% Chemical Engineering Journal 2 publications, 2.17%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 2, 2.17% Coordination Chemistry Reviews 2 publications, 2.17%
Advanced Science	Advanced Science, 2, 2.17% Advanced Science 2 publications, 2.17%
Chemistry of Materials	Chemistry of Materials, 2, 2.17% Chemistry of Materials 2 publications, 2.17%
ACS Nano	ACS Nano, 2, 2.17% ACS Nano 2 publications, 2.17%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 2.17% Journal of Materials Chemistry A 2 publications, 2.17%
Energy and Environmental Science	Energy and Environmental Science, 2, 2.17% Energy and Environmental Science 2 publications, 2.17%
Journal of Applied Physics	Journal of Applied Physics, 1, 1.09% Journal of Applied Physics 1 publication, 1.09%
Applied Physics Letters	Applied Physics Letters, 1, 1.09% Applied Physics Letters 1 publication, 1.09%
Energies	Energies, 1, 1.09% Energies 1 publication, 1.09%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 1, 1.09% Journal of Solid State Electrochemistry 1 publication, 1.09%
Nano Research	Nano Research, 1, 1.09% Nano Research 1 publication, 1.09%
Sensors and Actuators, B: Chemical	Sensors and Actuators, B: Chemical, 1, 1.09% Sensors and Actuators, B: Chemical 1 publication, 1.09%
Journal of Materials Science and Technology	Journal of Materials Science and Technology, 1, 1.09% Journal of Materials Science and Technology 1 publication, 1.09%
Joule	Joule, 1, 1.09% Joule 1 publication, 1.09%
iScience	iScience, 1, 1.09% iScience 1 publication, 1.09%
Nano Energy	Nano Energy, 1, 1.09% Nano Energy 1 publication, 1.09%
Matter	Matter, 1, 1.09% Matter 1 publication, 1.09%
Small Structures	Small Structures, 1, 1.09% Small Structures 1 publication, 1.09%
	1 2 3 4 5 6 7 8

Citations by publishers

	5 10 15 20 25 30 35
Wiley	Wiley, 34, 36.96% Wiley 34 publications, 36.96%
American Chemical Society (ACS)	American Chemical Society (ACS), 23, 25% American Chemical Society (ACS) 23 publications, 25%
Elsevier	Elsevier, 11, 11.96% Elsevier 11 publications, 11.96%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 9, 9.78% Royal Society of Chemistry (RSC) 9 publications, 9.78%
Springer Nature	Springer Nature, 5, 5.43% Springer Nature 5 publications, 5.43%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 4, 4.35% Multidisciplinary Digital Publishing Institute (MDPI) 4 publications, 4.35%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 2.17% American Institute of Physics (AIP) 2 publications, 2.17%
American Physical Society (APS)	American Physical Society (APS), 1, 1.09% American Physical Society (APS) 1 publication, 1.09%
IEEE	IEEE, 1, 1.09% IEEE 1 publication, 1.09%
IOP Publishing	IOP Publishing, 1, 1.09% IOP Publishing 1 publication, 1.09%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.09% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.09%
	5 10 15 20 25 30 35

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Kim Y. et al. A Facet‐Specific Quantum Dot Passivation Strategy for Colloid Management and Efficient Infrared Photovoltaics // Advanced Materials. 2019. Vol. 31. No. 17. p. 1805580.

GOST all authors (up to 50) Copy

Kim Y., Che F., Jo J. W., Park T., Pelayo García de Arquer F., Voznyy O., Sun B., Kim J. H., Choi M., Quintero-Torres R., Fan F., Tan C. S., Bladt E., Walters G. C., Proppe A. H., Zou C., Yuan H., Bals S., Hofkens J., Roeffaers M., Hoogland S., Sargent E. H. A Facet‐Specific Quantum Dot Passivation Strategy for Colloid Management and Efficient Infrared Photovoltaics // Advanced Materials. 2019. Vol. 31. No. 17. p. 1805580.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adma.201805580

UR - https://doi.org/10.1002/adma.201805580

TI - A Facet‐Specific Quantum Dot Passivation Strategy for Colloid Management and Efficient Infrared Photovoltaics

T2 - Advanced Materials

AU - Che, Fanglin

AU - Bladt, Eva

AU - Sargent, Edward H.

AU - Kim, Younghoon

AU - Jo, Jea Woong

AU - Park, Taiho

AU - Pelayo García de Arquer, F.

AU - Voznyy, Oleksandr

AU - Sun, Bin

AU - Kim, Jung Hwan

AU - Choi, Min-Jae

AU - Quintero-Torres, Rafael

AU - Fan, Fengjia

AU - Tan, Chih Shan

AU - Walters, Grant C.

AU - Proppe, Andrew H.

AU - Zou, Chengqin

AU - Yuan, Haifeng

AU - Bals, Sara

AU - Hofkens, J.

AU - Roeffaers, Maarten

AU - Hoogland, Sjoerd

PY - 2019

DA - 2019/03/12 00:00:00

PB - Wiley

SP - 1805580

IS - 17

VL - 31

SN - 0935-9648

SN - 1521-4095

ER -

BibTex |

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BibTex Copy

@article{2019_Kim,

author = {Fanglin Che and Eva Bladt and Edward H. Sargent and Younghoon Kim and Jea Woong Jo and Taiho Park and F. Pelayo García de Arquer and Oleksandr Voznyy and Bin Sun and Jung Hwan Kim and Min-Jae Choi and Rafael Quintero-Torres and Fengjia Fan and Chih Shan Tan and Grant C. Walters and Andrew H. Proppe and Chengqin Zou and Haifeng Yuan and Sara Bals and J. Hofkens and Maarten Roeffaers and Sjoerd Hoogland},

title = {A Facet‐Specific Quantum Dot Passivation Strategy for Colloid Management and Efficient Infrared Photovoltaics},

journal = {Advanced Materials},

year = {2019},

volume = {31},

publisher = {Wiley},

month = {mar},

url = {https://doi.org/10.1002/adma.201805580},

number = {17},

pages = {1805580},

doi = {10.1002/adma.201805580}

}

MLA

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MLA Copy

Kim, Younghoon, et al. “A Facet‐Specific Quantum Dot Passivation Strategy for Colloid Management and Efficient Infrared Photovoltaics.” Advanced Materials, vol. 31, no. 17, Mar. 2019, p. 1805580. https://doi.org/10.1002/adma.201805580.

Found error?

Publisher

Wiley

Journal

Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor

29.4

ISSN

09359648 (Print)
15214095 (Electronic)