Advanced Materials, volume 31, issue 10, pages 1807243

Lithium-Graphite Paste: An Interface Compatible Anode for Solid-State Batteries

Ji’an Duan ¹

Wangyan Wu ¹

Adelaide M Nolan ²

Tengrui Wang ¹

Jiayun Wen ¹

Chenchen Hu ¹

Yifei Mo ²

Wei Luo ¹

Yun-Hui Huang ¹

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Institute of New Energy for Vehicles; School of Materials Science and Engineering; Tongji University; Shanghai 201804 China |

Department of Materials Science and Engineering; University of Maryland; College Park MD 20742 USA |

Publication type: Journal Article

Publication date: 2019-01-21

Wiley

Journal: Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor: 29.4

ISSN: 09359648, 15214095

DOI: 10.1002/adma.201807243

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General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

All-solid-state batteries (ASSBs) with ceramic-based solid-state electrolytes (SSEs) enable high safety that is inaccessible with conventional lithium-ion batteries. Lithium metal, the ultimate anode with the highest specific capacity, also becomes available with nonflammable SSEs in ASSBs, which offers promising energy density. The rapid development of ASSBs, however, is significantly hampered by the large interfacial resistance as a matched lithium/ceramic interface that is not easy to pursue. Here, a lithium-graphite (Li-C) composite anode is fabricated, which shows a dramatic modification in wettability with garnet SSE. An intimate Li-C/garnet interface is obtained by casting Li-C composite onto garnet-type SSE, delivering an interfacial resistance as low as 11 Ω cm2 . As a comparison, pure Li/garnet interface gives a large resistance of 381 Ω cm2 . Such improvement can be ascribed to the experiment-measured increased viscosity of Li-C composite and simulation-verified limited interfacial reaction. The Li-C/garnet/Li-C symmetric cell exhibits stable plating/striping performance with small voltage hysteresis and endures a critical current density up to 1.0 mA cm-2 . The full cell paired with LiFePO4 shows stable cycle performance, comparable to the cell with liquid electrolyte. The present work demonstrates a promising strategy to develop ceramic-compatible lithium metal-based anodes and hence low-impedance ASSBs.

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Citations by journals

	2 4 6 8 10 12 14 16 18
Advanced Functional Materials	Advanced Functional Materials, 17, 7.83% Advanced Functional Materials 17 publications, 7.83%
ACS applied materials & interfaces	ACS applied materials & interfaces, 16, 7.37% ACS applied materials & interfaces 16 publications, 7.37%
Advanced Energy Materials	Advanced Energy Materials, 12, 5.53% Advanced Energy Materials 12 publications, 5.53%
ACS Applied Energy Materials	ACS Applied Energy Materials, 9, 4.15% ACS Applied Energy Materials 9 publications, 4.15%
Advanced Materials	Advanced Materials, 8, 3.69% Advanced Materials 8 publications, 3.69%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 7, 3.23% Journal of Materials Chemistry A 7 publications, 3.23%
Chemical Engineering Journal	Chemical Engineering Journal, 6, 2.76% Chemical Engineering Journal 6 publications, 2.76%
Nano Energy	Nano Energy, 6, 2.76% Nano Energy 6 publications, 2.76%
Small	Small, 6, 2.76% Small 6 publications, 2.76%
Rare Metals	Rare Metals, 5, 2.3% Rare Metals 5 publications, 2.3%
Angewandte Chemie	Angewandte Chemie, 5, 2.3% Angewandte Chemie 5 publications, 2.3%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 5, 2.3% Angewandte Chemie - International Edition 5 publications, 2.3%
Energy and Environmental Science	Energy and Environmental Science, 5, 2.3% Energy and Environmental Science 5 publications, 2.3%
Nature Communications	Nature Communications, 4, 1.84% Nature Communications 4 publications, 1.84%
Energy Storage Materials	Energy Storage Materials, 4, 1.84% Energy Storage Materials 4 publications, 1.84%
Nano Letters	Nano Letters, 4, 1.84% Nano Letters 4 publications, 1.84%
Matter	Matter, 3, 1.38% Matter 3 publications, 1.38%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 3, 1.38% Electrochemical Energy Reviews 3 publications, 1.38%
ACS Nano	ACS Nano, 3, 1.38% ACS Nano 3 publications, 1.38%
ACS Energy Letters	ACS Energy Letters, 3, 1.38% ACS Energy Letters 3 publications, 1.38%
Energy Technology	Energy Technology, 3, 1.38% Energy Technology 3 publications, 1.38%
Advanced Science	Advanced Science, 2, 0.92% Advanced Science 2 publications, 0.92%
Frontiers in Chemistry	Frontiers in Chemistry, 2, 0.92% Frontiers in Chemistry 2 publications, 0.92%
Batteries	Batteries, 2, 0.92% Batteries 2 publications, 0.92%
Materials Today	Materials Today, 2, 0.92% Materials Today 2 publications, 0.92%
Ceramics International	Ceramics International, 2, 0.92% Ceramics International 2 publications, 0.92%
Small Methods	Small Methods, 2, 0.92% Small Methods 2 publications, 0.92%
Batteries & Supercaps	Batteries & Supercaps, 2, 0.92% Batteries & Supercaps 2 publications, 0.92%
Energy & Environmental Materials	Energy & Environmental Materials, 2, 0.92% Energy & Environmental Materials 2 publications, 0.92%
	2 4 6 8 10 12 14 16 18

Citations by publishers

	10 20 30 40 50 60 70 80
Wiley	Wiley, 77, 35.48% Wiley 77 publications, 35.48%
American Chemical Society (ACS)	American Chemical Society (ACS), 45, 20.74% American Chemical Society (ACS) 45 publications, 20.74%
Elsevier	Elsevier, 37, 17.05% Elsevier 37 publications, 17.05%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 19, 8.76% Royal Society of Chemistry (RSC) 19 publications, 8.76%
Springer Nature	Springer Nature, 15, 6.91% Springer Nature 15 publications, 6.91%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 5, 2.3% Nonferrous Metals Society of China 5 publications, 2.3%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 1.38% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 1.38%
Frontiers Media S.A.	Frontiers Media S.A., 2, 0.92% Frontiers Media S.A. 2 publications, 0.92%
Chinese Physical Society	Chinese Physical Society, 2, 0.92% Chinese Physical Society 2 publications, 0.92%
OAE Publishing Inc.	OAE Publishing Inc., 2, 0.92% OAE Publishing Inc. 2 publications, 0.92%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 0.46% American Institute of Physics (AIP) 1 publication, 0.46%
Bentham Science	Bentham Science, 1, 0.46% Bentham Science 1 publication, 0.46%
The Electrochemical Society	The Electrochemical Society, 1, 0.46% The Electrochemical Society 1 publication, 0.46%
Tsinghua University Press	Tsinghua University Press, 1, 0.46% Tsinghua University Press 1 publication, 0.46%
University of Science and Technology Beijing	University of Science and Technology Beijing, 1, 0.46% University of Science and Technology Beijing 1 publication, 0.46%
Electrochemical Science Group, University of Belgrade	Electrochemical Science Group, University of Belgrade, 1, 0.46% Electrochemical Science Group, University of Belgrade 1 publication, 0.46%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.46% American Association for the Advancement of Science (AAAS) 1 publication, 0.46%
Hans Publishers	Hans Publishers, 1, 0.46% Hans Publishers 1 publication, 0.46%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.46% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.46%
	10 20 30 40 50 60 70 80

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GOST Copy

Duan J. et al. Lithium-Graphite Paste: An Interface Compatible Anode for Solid-State Batteries // Advanced Materials. 2019. Vol. 31. No. 10. p. 1807243.

GOST all authors (up to 50) Copy

Duan J., Wu W., Nolan A. M., Wang T., Wen J., Hu C., Mo Y., Luo W., Huang Y. Lithium-Graphite Paste: An Interface Compatible Anode for Solid-State Batteries // Advanced Materials. 2019. Vol. 31. No. 10. p. 1807243.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1002/adma.201807243

UR - https://doi.org/10.1002/adma.201807243

TI - Lithium-Graphite Paste: An Interface Compatible Anode for Solid-State Batteries

T2 - Advanced Materials

AU - Duan, Ji’an

AU - Wu, Wangyan

AU - Wang, Tengrui

AU - Wen, Jiayun

AU - Hu, Chenchen

AU - Luo, Wei

AU - Nolan, Adelaide M

AU - Mo, Yifei

AU - Huang, Yun-Hui

PY - 2019

DA - 2019/01/21 00:00:00

PB - Wiley

SP - 1807243

IS - 10

VL - 31

SN - 0935-9648

SN - 1521-4095

ER -

BibTex |

Cite this

BibTex Copy

@article{2019_Duan,

author = {Ji’an Duan and Wangyan Wu and Tengrui Wang and Jiayun Wen and Chenchen Hu and Wei Luo and Adelaide M Nolan and Yifei Mo and Yun-Hui Huang},

title = {Lithium-Graphite Paste: An Interface Compatible Anode for Solid-State Batteries},

journal = {Advanced Materials},

year = {2019},

volume = {31},

publisher = {Wiley},

month = {jan},

url = {https://doi.org/10.1002/adma.201807243},

number = {10},

pages = {1807243},

doi = {10.1002/adma.201807243}

}

MLA

Cite this

MLA Copy

Duan, Ji’an, et al. “Lithium-Graphite Paste: An Interface Compatible Anode for Solid-State Batteries.” Advanced Materials, vol. 31, no. 10, Jan. 2019, p. 1807243. https://doi.org/10.1002/adma.201807243.

Found error?

Publisher

Wiley

Journal

Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor

29.4

ISSN

09359648 (Print)
15214095 (Electronic)