Advanced Materials, volume 31, issue 50, pages 1902029
Intermolecular Chemistry in Solid Polymer Electrolytes for High‐Energy‐Density Lithium Batteries
1
Dalian National Laboratory for Clean Energy Dalian 116023 China
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2
Qingdao Industrial Energy Storage Research InstituteQingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences No. 189 Songling Road Qingdao 266101 China
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Publication type: Journal Article
Publication date: 2019-08-22
Journal:
Advanced Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 29.4
ISSN: 09359648, 15214095
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Solid polymer electrolytes (SPEs) have aroused wide interest in lithium batteries because of their sufficient mechanical properties, superior safety performances, and excellent processability. However, ionic conductivity and high‐voltage compatibility of SPEs are still yet to meet the requirement of future energy‐storage systems, representing significant barriers to progress. In this regard, intermolecular interactions in SPEs have attracted attention, and they can significantly impact on the Li+ motion and frontier orbital energy level of SPEs. Recent advances in improving electrochemcial performance of SPEs are reviewed, and the underlying mechanism of these proposed strategies related to intermolecular interaction is discussed, including ion–dipole, hydrogen bonds, π–π stacking, and Lewis acid–base interactions. It is hoped that this review can inspire a deeper consideration on this critical issue, which can pave new pathway to improve ionic conductivity and high‐voltage performance of SPEs.
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Zhou Q. et al. Intermolecular Chemistry in Solid Polymer Electrolytes for High‐Energy‐Density Lithium Batteries // Advanced Materials. 2019. Vol. 31. No. 50. p. 1902029.
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Zhou Q., Sun Y., Dong S., Li X., Cui G. Intermolecular Chemistry in Solid Polymer Electrolytes for High‐Energy‐Density Lithium Batteries // Advanced Materials. 2019. Vol. 31. No. 50. p. 1902029.
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TY - JOUR
DO - 10.1002/adma.201902029
UR - https://onlinelibrary.wiley.com/doi/10.1002/adma.201902029
TI - Intermolecular Chemistry in Solid Polymer Electrolytes for High‐Energy‐Density Lithium Batteries
T2 - Advanced Materials
AU - Zhou, Qian
AU - Dong, Shanmu
AU - Cui, Guanglei
AU - Sun, Ying
AU - Li, Xianfeng
PY - 2019
DA - 2019/08/22 00:00:00
PB - Wiley
SP - 1902029
IS - 50
VL - 31
SN - 0935-9648
SN - 1521-4095
ER -
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@article{2019_Zhou,
author = {Qian Zhou and Shanmu Dong and Guanglei Cui and Ying Sun and Xianfeng Li},
title = {Intermolecular Chemistry in Solid Polymer Electrolytes for High‐Energy‐Density Lithium Batteries},
journal = {Advanced Materials},
year = {2019},
volume = {31},
publisher = {Wiley},
month = {aug},
url = {https://onlinelibrary.wiley.com/doi/10.1002/adma.201902029},
number = {50},
pages = {1902029},
doi = {10.1002/adma.201902029}
}
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MLA
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Zhou, Qian, et al. “Intermolecular Chemistry in Solid Polymer Electrolytes for High‐Energy‐Density Lithium Batteries.” Advanced Materials, vol. 31, no. 50, Aug. 2019, p. 1902029. https://onlinelibrary.wiley.com/doi/10.1002/adma.201902029.
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