Advanced Materials, volume 32, issue 2, pages 1905517

Nacre‐Inspired Composite Electrolytes for Load‐Bearing Solid‐State Lithium‐Metal Batteries

Aijun Li ^{1, 2}

Xiangbiao Liao ³

Hanrui Zhang ²

Lei Shi ⁴

Peiyu Wang ²

Qian Cheng ²

James Borovilas ²

Zeyuan Li ²

Wenlong Huang ²

Zhenxuan Fu ²

Martin Dontigny ⁵

Karim Zaghib ⁵

Kristin Myers ⁴

Xiuyun Chuan ¹

Xi Chen ³

Yuan Yang ²

Hide authors affiliations Show authors affiliations: 5 affiliations

Key Laboratory of Orogenic Belts and Crustal Evolution School of Earth and Space Sciences Peking University Beijing 100871 China |

Program of Materials Science and Engineering Department of Applied Physics and Applied Mathematics Columbia University New York NY 10027 USA |

Earth Engineering Center Center for Advanced Materials for Energy and Environment Department of Earth and Environmental Engineering Columbia University New York NY 10027 USA |

⁴

Department of Mechanical Engineering Columbia University New York NY 10027 USA |

⁵

IREQ‐Institute Recherche d'Hydro‐Québec Varennes Québec J3X 1S1 Canada |

Publication type: Journal Article

Publication date: 2019-11-29

Wiley

Journal: Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor: 29.4

ISSN: 09359648, 15214095

DOI: 10.1002/adma.201905517

Copy DOI

General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

Solid-state lithium-metal batteries with solid electrolytes are promising for next-generation energy-storage devices. However, it remains challenging to develop solid electrolytes that are both mechanically robust and strong against external mechanical load, due to the brittleness of ceramic electrolytes and the softness of polymer electrolytes. Herein, a nacre-inspired design of ceramic/polymer solid composite electrolytes with a “brick-and-mortar” microstructure is proposed. The nacre-like ceramic/polymer electrolyte (NCPE) simultaneously possesses a much higher fracture strain (1.1%) than pure ceramic electrolytes (0.13%) and a much larger ultimate flexural modulus (7.8 GPa) than pure polymer electrolytes (20 MPa). The electrochemical performance of NCPE is also much better than pure ceramic or polymer electrolytes, especially under mechanical load. A 5 × 5 cm2 pouch cell with LAGP/poly(ether-acrylate) NCPE exhibits stable cycling with a capacity retention of 95.6% over 100 cycles at room temperature, even undergoes a large point load of 10 N. In contrast, cells based on pure ceramic and pure polymer electrolyte show poor cycle life. The NCPE provides a new design for solid composite electrolyte and opens up new possibilities for future solid-state lithium-metal batteries and structural energy storage.

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Citations by journals

	1 2 3 4 5
Advanced Functional Materials	Advanced Functional Materials, 5, 4.55% Advanced Functional Materials 5 publications, 4.55%
ACS applied materials & interfaces	ACS applied materials & interfaces, 5, 4.55% ACS applied materials & interfaces 5 publications, 4.55%
Small	Small, 4, 3.64% Small 4 publications, 3.64%
ACS Applied Energy Materials	ACS Applied Energy Materials, 4, 3.64% ACS Applied Energy Materials 4 publications, 3.64%
Advanced Energy Materials	Advanced Energy Materials, 4, 3.64% Advanced Energy Materials 4 publications, 3.64%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 3.64% Journal of Materials Chemistry A 4 publications, 3.64%
Angewandte Chemie	Angewandte Chemie, 3, 2.73% Angewandte Chemie 3 publications, 2.73%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 3, 2.73% Angewandte Chemie - International Edition 3 publications, 2.73%
Advanced Materials	Advanced Materials, 3, 2.73% Advanced Materials 3 publications, 2.73%
Advanced Science	Advanced Science, 3, 2.73% Advanced Science 3 publications, 2.73%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 2, 1.82% Materials Chemistry Frontiers 2 publications, 1.82%
Small Methods	Small Methods, 2, 1.82% Small Methods 2 publications, 1.82%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 2, 1.82% Journal of the Electrochemical Society 2 publications, 1.82%
Nanomaterials	Nanomaterials, 2, 1.82% Nanomaterials 2 publications, 1.82%
Materials	Materials, 2, 1.82% Materials 2 publications, 1.82%
Nature Communications	Nature Communications, 2, 1.82% Nature Communications 2 publications, 1.82%
Nano Research	Nano Research, 2, 1.82% Nano Research 2 publications, 1.82%
Materials Today	Materials Today, 2, 1.82% Materials Today 2 publications, 1.82%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.82% Chemical Engineering Journal 2 publications, 1.82%
Composites Science and Technology	Composites Science and Technology, 2, 1.82% Composites Science and Technology 2 publications, 1.82%
ACS Energy Letters	ACS Energy Letters, 2, 1.82% ACS Energy Letters 2 publications, 1.82%
Battery Energy	Battery Energy, 2, 1.82% Battery Energy 2 publications, 1.82%
Nano-Micro Letters	Nano-Micro Letters, 1, 0.91% Nano-Micro Letters 1 publication, 0.91%
Composites Part B: Engineering	Composites Part B: Engineering, 1, 0.91% Composites Part B: Engineering 1 publication, 0.91%
Journal of Advanced Ceramics	Journal of Advanced Ceramics, 1, 0.91% Journal of Advanced Ceramics 1 publication, 0.91%
Ionics	Ionics, 1, 0.91% Ionics 1 publication, 0.91%
Journal of Electroanalytical Chemistry	Journal of Electroanalytical Chemistry, 1, 0.91% Journal of Electroanalytical Chemistry 1 publication, 0.91%
Nano Energy	Nano Energy, 1, 0.91% Nano Energy 1 publication, 0.91%
Electrochimica Acta	Electrochimica Acta, 1, 0.91% Electrochimica Acta 1 publication, 0.91%
	1 2 3 4 5

Citations by publishers

	5 10 15 20 25 30 35 40 45 50
Wiley	Wiley, 46, 41.82% Wiley 46 publications, 41.82%
Elsevier	Elsevier, 20, 18.18% Elsevier 20 publications, 18.18%
American Chemical Society (ACS)	American Chemical Society (ACS), 14, 12.73% American Chemical Society (ACS) 14 publications, 12.73%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 9, 8.18% Royal Society of Chemistry (RSC) 9 publications, 8.18%
Springer Nature	Springer Nature, 7, 6.36% Springer Nature 7 publications, 6.36%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 4, 3.64% Multidisciplinary Digital Publishing Institute (MDPI) 4 publications, 3.64%
The Electrochemical Society	The Electrochemical Society, 2, 1.82% The Electrochemical Society 2 publications, 1.82%
Tsinghua University Press	Tsinghua University Press, 1, 0.91% Tsinghua University Press 1 publication, 0.91%
IOP Publishing	IOP Publishing, 1, 0.91% IOP Publishing 1 publication, 0.91%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.91% Nonferrous Metals Society of China 1 publication, 0.91%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.91% Frontiers Media S.A. 1 publication, 0.91%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.91% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.91%
	5 10 15 20 25 30 35 40 45 50

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Li A. et al. Nacre‐Inspired Composite Electrolytes for Load‐Bearing Solid‐State Lithium‐Metal Batteries // Advanced Materials. 2019. Vol. 32. No. 2. p. 1905517.

GOST all authors (up to 50) Copy

Li A., Liao X., Zhang H., Shi L., Wang P., Cheng Q., Borovilas J., Li Z., Huang W., Fu Z., Dontigny M., Zaghib K., Myers K., Chuan X., Chen X., Yang Y. Nacre‐Inspired Composite Electrolytes for Load‐Bearing Solid‐State Lithium‐Metal Batteries // Advanced Materials. 2019. Vol. 32. No. 2. p. 1905517.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adma.201905517

UR - https://doi.org/10.1002/adma.201905517

TI - Nacre‐Inspired Composite Electrolytes for Load‐Bearing Solid‐State Lithium‐Metal Batteries

T2 - Advanced Materials

AU - Li, Aijun

AU - Wang, Peiyu

AU - Borovilas, James

AU - Huang, Wenlong

AU - Fu, Zhenxuan

AU - Chuan, Xiuyun

AU - Yang, Yuan

AU - Liao, Xiangbiao

AU - Zhang, Hanrui

AU - Shi, Lei

AU - Cheng, Qian

AU - Li, Zeyuan

AU - Dontigny, Martin

AU - Zaghib, Karim

AU - Myers, Kristin

AU - Chen, Xi

PY - 2019

DA - 2019/11/29 00:00:00

PB - Wiley

SP - 1905517

IS - 2

VL - 32

SN - 0935-9648

SN - 1521-4095

ER -

BibTex |

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BibTex Copy

@article{2019_Li,

author = {Aijun Li and Peiyu Wang and James Borovilas and Wenlong Huang and Zhenxuan Fu and Xiuyun Chuan and Yuan Yang and Xiangbiao Liao and Hanrui Zhang and Lei Shi and Qian Cheng and Zeyuan Li and Martin Dontigny and Karim Zaghib and Kristin Myers and Xi Chen},

title = {Nacre‐Inspired Composite Electrolytes for Load‐Bearing Solid‐State Lithium‐Metal Batteries},

journal = {Advanced Materials},

year = {2019},

volume = {32},

publisher = {Wiley},

month = {nov},

url = {https://doi.org/10.1002/adma.201905517},

number = {2},

pages = {1905517},

doi = {10.1002/adma.201905517}

}

MLA

Cite this

MLA Copy

Li, Aijun, et al. “Nacre‐Inspired Composite Electrolytes for Load‐Bearing Solid‐State Lithium‐Metal Batteries.” Advanced Materials, vol. 32, no. 2, Nov. 2019, p. 1905517. https://doi.org/10.1002/adma.201905517.

Found error?

Publisher

Wiley

Journal

Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor

29.4

ISSN

09359648 (Print)
15214095 (Electronic)