Advanced Materials, volume 34, issue 20, pages 2200856

Highly Stable Halide‐Electrolyte‐Based All‐Solid‐State Li–Se Batteries

Xiaona Li ¹

Jianwen Liang ^{1, 2}

Jung-Tae Kim ¹

Jiamin Fu ¹

Hui Duan ¹

Ning Chen ³

Ruying Li ¹

Shangqian Zhao ²

Jiantao Wang ²

Huan Huang ⁴

Xueliang Andy Sun ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of Mechanical and Materials Engineering University of Western Ontario 1151 Richmond St London Ontario N6A 3K7 Canada |

China Automotive Battery Research Institute Co. Ltd 5th Floor, No. 43, Mining Building, North Sanhuan Middle Road Beijing 100088 China |

Canadian Light Source 44 Innovation Boulevard Saskatoon SK S7N 2V3 Canada |

⁴

Glabat Solid‐State Battery Inc. 700 Collip Circle London ON N6G 4X8 Canada |

Publication type: Journal Article

Publication date: 2022-04-17

Wiley

Journal: Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor: 29.4

ISSN: 09359648, 15214095

DOI: 10.1002/adma.202200856

Copy DOI

General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

Solid-state Li-S and Li-Se batteries are promising devices that can address the safety and electrochemical stability issues that arise from liquid-based systems. However, solid-state Li-Se/S batteries usually present poor cycling stability due to the high resistance interfaces and decomposition of solid electrolytes caused by their narrow electrochemical stability windows. Here, an integrated solid-state Li-Se battery based on a halide Li3 HoCl6 solid electrolyte with high ionic conductivity is presented. The intrinsic wide electrochemical stability window of the Li3 HoCl6 and its stability toward Se and the lithiated species effectively inhibit degeneration of the electrolyte and the Se cathode by suppressing side reactions. The inherent thermodynamic mechanism of the lithiation/delithiation process of the Se cathode in solid is also revealed and confirmed by theoretical calculations. The battery achieves a reversible capacity of 402 mAh g-1 after 750 cycles. The electrochemical performance, thermodynamic lithiation/delithiation mechanism, and stability of metal-halide-based Li-Se batteries confer theoretical study and practical applicability that extends to other energy-storage systems.

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Angewandte Chemie	Angewandte Chemie, 3, 4.62% Angewandte Chemie 3 publications, 4.62%
Nature	Nature, 2, 3.08% Nature 2 publications, 3.08%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 2, 3.08% Electrochemical Energy Reviews 2 publications, 3.08%
ACS Nano	ACS Nano, 2, 3.08% ACS Nano 2 publications, 3.08%
Advanced Functional Materials	Advanced Functional Materials, 2, 3.08% Advanced Functional Materials 2 publications, 3.08%
Science China Chemistry	Science China Chemistry, 1, 1.54% Science China Chemistry 1 publication, 1.54%
ACS applied materials & interfaces	ACS applied materials & interfaces, 1, 1.54% ACS applied materials & interfaces 1 publication, 1.54%
EcoMat	EcoMat, 1, 1.54% EcoMat 1 publication, 1.54%
Batteries	Batteries, 1, 1.54% Batteries 1 publication, 1.54%
Frontiers in Energy Research	Frontiers in Energy Research, 1, 1.54% Frontiers in Energy Research 1 publication, 1.54%
ACS Applied Nano Materials	ACS Applied Nano Materials, 1, 1.54% ACS Applied Nano Materials 1 publication, 1.54%
Materials Today	Materials Today, 1, 1.54% Materials Today 1 publication, 1.54%
Scripta Materialia	Scripta Materialia, 1, 1.54% Scripta Materialia 1 publication, 1.54%
Journal of Physics: Conference Series	Journal of Physics: Conference Series, 1, 1.54% Journal of Physics: Conference Series 1 publication, 1.54%
Advanced Science	Advanced Science, 1, 1.54% Advanced Science 1 publication, 1.54%
Ionics	Ionics, 1, 1.54% Ionics 1 publication, 1.54%
Chemical Reviews	Chemical Reviews, 1, 1.54% Chemical Reviews 1 publication, 1.54%
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Chemical Science	Chemical Science, 1, 1.54% Chemical Science 1 publication, 1.54%
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Advanced Composites and Hybrid Materials	Advanced Composites and Hybrid Materials, 1, 1.54% Advanced Composites and Hybrid Materials 1 publication, 1.54%
Progress in Materials Science	Progress in Materials Science, 1, 1.54% Progress in Materials Science 1 publication, 1.54%
MRS Bulletin	MRS Bulletin, 1, 1.54% MRS Bulletin 1 publication, 1.54%
Nano Letters	Nano Letters, 1, 1.54% Nano Letters 1 publication, 1.54%
Nature Communications	Nature Communications, 1, 1.54% Nature Communications 1 publication, 1.54%
	1 2 3 4 5 6

Citations by publishers

	5 10 15 20 25 30
Wiley	Wiley, 27, 41.54% Wiley 27 publications, 41.54%
Springer Nature	Springer Nature, 11, 16.92% Springer Nature 11 publications, 16.92%
American Chemical Society (ACS)	American Chemical Society (ACS), 9, 13.85% American Chemical Society (ACS) 9 publications, 13.85%
Elsevier	Elsevier, 6, 9.23% Elsevier 6 publications, 9.23%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 3, 4.62% Royal Society of Chemistry (RSC) 3 publications, 4.62%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 3.08% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 3.08%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.54% Frontiers Media S.A. 1 publication, 1.54%
IOP Publishing	IOP Publishing, 1, 1.54% IOP Publishing 1 publication, 1.54%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 1.54% American Association for the Advancement of Science (AAAS) 1 publication, 1.54%
Cambridge University Press	Cambridge University Press, 1, 1.54% Cambridge University Press 1 publication, 1.54%
American Vacuum Society	American Vacuum Society, 1, 1.54% American Vacuum Society 1 publication, 1.54%
OAE Publishing Inc.	OAE Publishing Inc., 1, 1.54% OAE Publishing Inc. 1 publication, 1.54%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.54% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.54%
	5 10 15 20 25 30

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Li X. et al. Highly Stable Halide‐Electrolyte‐Based All‐Solid‐State Li–Se Batteries // Advanced Materials. 2022. Vol. 34. No. 20. p. 2200856.

GOST all authors (up to 50) Copy

Li X., Liang J., Kim J., Fu J., Duan H., Chen N., Li R., Zhao S., Wang J., Huang H., Sun X. A. Highly Stable Halide‐Electrolyte‐Based All‐Solid‐State Li–Se Batteries // Advanced Materials. 2022. Vol. 34. No. 20. p. 2200856.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/adma.202200856

UR - https://doi.org/10.1002/adma.202200856

TI - Highly Stable Halide‐Electrolyte‐Based All‐Solid‐State Li–Se Batteries

T2 - Advanced Materials

AU - Liang, Jianwen

AU - Kim, Jung-Tae

AU - Fu, Jiamin

AU - Duan, Hui

AU - Li, Ruying

AU - Zhao, Shangqian

AU - Li, Xiaona

AU - Sun, Xueliang Andy

AU - Chen, Ning

AU - Wang, Jiantao

AU - Huang, Huan

PY - 2022

DA - 2022/04/17 00:00:00

PB - Wiley

SP - 2200856

IS - 20

VL - 34

SN - 0935-9648

SN - 1521-4095

ER -

BibTex |

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BibTex Copy

@article{2022_Li,

author = {Jianwen Liang and Jung-Tae Kim and Jiamin Fu and Hui Duan and Ruying Li and Shangqian Zhao and Xiaona Li and Xueliang Andy Sun and Ning Chen and Jiantao Wang and Huan Huang},

title = {Highly Stable Halide‐Electrolyte‐Based All‐Solid‐State Li–Se Batteries},

journal = {Advanced Materials},

year = {2022},

volume = {34},

publisher = {Wiley},

month = {apr},

url = {https://doi.org/10.1002/adma.202200856},

number = {20},

pages = {2200856},

doi = {10.1002/adma.202200856}

}

MLA

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MLA Copy

Li, Xiaona, et al. “Highly Stable Halide‐Electrolyte‐Based All‐Solid‐State Li–Se Batteries.” Advanced Materials, vol. 34, no. 20, Apr. 2022, p. 2200856. https://doi.org/10.1002/adma.202200856.

Found error?

Publisher

Wiley

Journal

Advanced Materials

Quartile SCImago

Quartile WOS

Impact factor

29.4

ISSN

09359648 (Print)
15214095 (Electronic)