Asymmetric Intermolecular Rauhut−Currier Reaction for the Construction of 3,3-Disubstituted Oxindoles with Quaternary Stereogenic Centers
Тип публикации: Journal Article
Дата публикации: 2017-09-27
SCImago Q1
WOS Q1
БС1
SJR: 0.704
CiteScore: 6.9
Impact factor: 3.7
ISSN: 16154150, 16154169
General Chemistry
Краткое описание
A remote cross Rauhut−Currier reaction utilizing vinyl ketones and para-quinone methides derived from isatins was realized, which was successfully catalyzed using bifunctional phosphines, furnishing chiral 3,3-disubstituted oxindoles in excellent enantioselectivities and high yields. The mechanistic studies demonstrated the key role of the alkyl hydrogen of the vinyl ketones, which conceivably interacted with the para-quinone methide carbonyl group via the hydrogen bond, offering a new insight for the design of novel asymmetric reactions.
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Wang H. et al. Asymmetric Intermolecular Rauhut−Currier Reaction for the Construction of 3,3-Disubstituted Oxindoles with Quaternary Stereogenic Centers // Advanced Synthesis and Catalysis. 2017. Vol. 359. No. 22. pp. 3934-3939.
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Wang H., Wang K., Man Y., Gao X., Yang L., Ren Y., Li N., Tang B., ZHAO G. Asymmetric Intermolecular Rauhut−Currier Reaction for the Construction of 3,3-Disubstituted Oxindoles with Quaternary Stereogenic Centers // Advanced Synthesis and Catalysis. 2017. Vol. 359. No. 22. pp. 3934-3939.
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TY - JOUR
DO - 10.1002/adsc.201700649
UR - https://doi.org/10.1002/adsc.201700649
TI - Asymmetric Intermolecular Rauhut−Currier Reaction for the Construction of 3,3-Disubstituted Oxindoles with Quaternary Stereogenic Centers
T2 - Advanced Synthesis and Catalysis
AU - Wang, Hongyu
AU - Wang, Kaiye
AU - Man, Yunquan
AU - Gao, Xiaonan
AU - Yang, Limin
AU - Ren, Yanfei
AU - Li, Na
AU - Tang, Bo
AU - ZHAO, Gang
PY - 2017
DA - 2017/09/27
PB - Wiley
SP - 3934-3939
IS - 22
VL - 359
SN - 1615-4150
SN - 1615-4169
ER -
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@article{2017_Wang,
author = {Hongyu Wang and Kaiye Wang and Yunquan Man and Xiaonan Gao and Limin Yang and Yanfei Ren and Na Li and Bo Tang and Gang ZHAO},
title = {Asymmetric Intermolecular Rauhut−Currier Reaction for the Construction of 3,3-Disubstituted Oxindoles with Quaternary Stereogenic Centers},
journal = {Advanced Synthesis and Catalysis},
year = {2017},
volume = {359},
publisher = {Wiley},
month = {sep},
url = {https://doi.org/10.1002/adsc.201700649},
number = {22},
pages = {3934--3939},
doi = {10.1002/adsc.201700649}
}
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MLA
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Wang, Hongyu, et al. “Asymmetric Intermolecular Rauhut−Currier Reaction for the Construction of 3,3-Disubstituted Oxindoles with Quaternary Stereogenic Centers.” Advanced Synthesis and Catalysis, vol. 359, no. 22, Sep. 2017, pp. 3934-3939. https://doi.org/10.1002/adsc.201700649.
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