Mechanochemical Transformation of CF 3 Group: Synthesis of Amides and Schiff Bases
Satenik Mkrtchyan
1
,
Michał Jakubczyk
1, 2
,
Suneel Lanka
1, 3
,
Muhammad Yar
4
,
Khurshid Ayub
4
,
Mohanad Shkoor
5
,
Michael Pittelkow
6
,
Viktor O Iaroshenko
1, 7, 8
2
Publication type: Journal Article
Publication date: 2021-10-12
scimago Q1
wos Q1
SJR: 0.930
CiteScore: 8.0
Impact factor: 4.0
ISSN: 16154150, 16154169
General Chemistry
Abstract
We communicate two mild, solvent-free mechanochemical coupling transformations of CF3 group with nitro compounds into amides or Schiff bases employing Ytterbia as a catalyst. This process proceeds via C−F bond activation, accompanied with utilisation of Si-based reductants/oxygen scavengers – reductants of the nitro group. The scope and limitations of the disclosed methodologies are thoroughly studied. To the best of our knowledge, this work is the first example of mechanical energy promoted transformation of the inert CF3 group into other functionalities.
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Metrics
34
Total citations:
34
Citations from 2024:
18
(52.94%)
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MLA
Cite this
GOST
Copy
Mkrtchyan S. et al. Mechanochemical Transformation of CF 3 Group: Synthesis of Amides and Schiff Bases // Advanced Synthesis and Catalysis. 2021. Vol. 363. No. 24. pp. 5448-5460.
GOST all authors (up to 50)
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Mkrtchyan S., Jakubczyk M., Lanka S., Yar M., Ayub K., Shkoor M., Pittelkow M., Iaroshenko V. O. Mechanochemical Transformation of CF 3 Group: Synthesis of Amides and Schiff Bases // Advanced Synthesis and Catalysis. 2021. Vol. 363. No. 24. pp. 5448-5460.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/adsc.202100538
UR - https://doi.org/10.1002/adsc.202100538
TI - Mechanochemical Transformation of CF 3 Group: Synthesis of Amides and Schiff Bases
T2 - Advanced Synthesis and Catalysis
AU - Mkrtchyan, Satenik
AU - Jakubczyk, Michał
AU - Lanka, Suneel
AU - Yar, Muhammad
AU - Ayub, Khurshid
AU - Shkoor, Mohanad
AU - Pittelkow, Michael
AU - Iaroshenko, Viktor O
PY - 2021
DA - 2021/10/12
PB - Wiley
SP - 5448-5460
IS - 24
VL - 363
SN - 1615-4150
SN - 1615-4169
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2021_Mkrtchyan,
author = {Satenik Mkrtchyan and Michał Jakubczyk and Suneel Lanka and Muhammad Yar and Khurshid Ayub and Mohanad Shkoor and Michael Pittelkow and Viktor O Iaroshenko},
title = {Mechanochemical Transformation of CF 3 Group: Synthesis of Amides and Schiff Bases},
journal = {Advanced Synthesis and Catalysis},
year = {2021},
volume = {363},
publisher = {Wiley},
month = {oct},
url = {https://doi.org/10.1002/adsc.202100538},
number = {24},
pages = {5448--5460},
doi = {10.1002/adsc.202100538}
}
Cite this
MLA
Copy
Mkrtchyan, Satenik, et al. “Mechanochemical Transformation of CF 3 Group: Synthesis of Amides and Schiff Bases.” Advanced Synthesis and Catalysis, vol. 363, no. 24, Oct. 2021, pp. 5448-5460. https://doi.org/10.1002/adsc.202100538.