Synthesis of Diverse Allylsilanes Employing Brønsted Acid Catalyzed Reductive Functionalization
Elisabeth L. R. Leonard
1, 2
,
Geoffrey R. Akien
1
,
Thomas K Britten
3
,
Nahin Kazi
1, 2
,
Dean D Roberts
1, 2
,
M G Mclaughlin
2
Publication type: Journal Article
Publication date: 2023-11-06
scimago Q1
wos Q1
SJR: 0.930
CiteScore: 8.0
Impact factor: 4.0
ISSN: 16154150, 16154169
General Chemistry
Abstract
We present a rapid (0.25–1 h), method to produce functionalised allylsilanes from readily available vinylsilanes. Employing a Brønsted acid catalysed dehydration as the key step, allylsilanes are produced in good yields (22–98%) and, in most cases, as a single geometric isomer. Furthermore, a possible allylation‐Cope pathway was discovered for certain substrates and attempts to optimise this are described.
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Leonard E. L. R. et al. Synthesis of Diverse Allylsilanes Employing Brønsted Acid Catalyzed Reductive Functionalization // Advanced Synthesis and Catalysis. 2023. Vol. 365. No. 22. pp. 3872-3875.
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Leonard E. L. R., Akien G. R., Britten T. K., Kazi N., Roberts D. D., Mclaughlin M. G. Synthesis of Diverse Allylsilanes Employing Brønsted Acid Catalyzed Reductive Functionalization // Advanced Synthesis and Catalysis. 2023. Vol. 365. No. 22. pp. 3872-3875.
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TY - JOUR
DO - 10.1002/adsc.202300917
UR - https://doi.org/10.1002/adsc.202300917
TI - Synthesis of Diverse Allylsilanes Employing Brønsted Acid Catalyzed Reductive Functionalization
T2 - Advanced Synthesis and Catalysis
AU - Leonard, Elisabeth L. R.
AU - Akien, Geoffrey R.
AU - Britten, Thomas K
AU - Kazi, Nahin
AU - Roberts, Dean D
AU - Mclaughlin, M G
PY - 2023
DA - 2023/11/06
PB - Wiley
SP - 3872-3875
IS - 22
VL - 365
SN - 1615-4150
SN - 1615-4169
ER -
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@article{2023_Leonard,
author = {Elisabeth L. R. Leonard and Geoffrey R. Akien and Thomas K Britten and Nahin Kazi and Dean D Roberts and M G Mclaughlin},
title = {Synthesis of Diverse Allylsilanes Employing Brønsted Acid Catalyzed Reductive Functionalization},
journal = {Advanced Synthesis and Catalysis},
year = {2023},
volume = {365},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002/adsc.202300917},
number = {22},
pages = {3872--3875},
doi = {10.1002/adsc.202300917}
}
Cite this
MLA
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Leonard, Elisabeth L. R., et al. “Synthesis of Diverse Allylsilanes Employing Brønsted Acid Catalyzed Reductive Functionalization.” Advanced Synthesis and Catalysis, vol. 365, no. 22, Nov. 2023, pp. 3872-3875. https://doi.org/10.1002/adsc.202300917.