Open Access

Advanced Electronic Materials, volume 1, issue 7, pages 1500062

Ligand‐Induced Control of Photoconductive Gain and Doping in a Hybrid Graphene–Quantum Dot Transistor

Lyudmila Turyanska ¹

O.N. Makarovsky ¹

Simon A Svatek ¹

P.H. Beton ¹

C. J. Mellor ¹

A. Patane ¹

L J. Eaves ¹

N R Thomas ²

Michael Fay ³

Alexander J. Marsden ⁴

Neil Wilson ⁴

Hide authors affiliations Show authors affiliations: 4 affiliations

School of Physics and Astronomy The University of Nottingham Nottingham NG7 2RD UK |

Centre for Biomolecular Sciences School of Chemistry The University of Nottingham Nottingham NG7 2RD UK |

Nottingham Nanotechnology and Nanoscience Centre Nottingham NG7 2RD UK |

⁴

Department of Physics University of Warwick Coventry CV4 7AL UK |

Publication type: Journal Article

Publication date: 2015-06-05

Wiley

Journal: Advanced Electronic Materials

Quartile SCImago

Quartile WOS

Impact factor: 6.2

ISSN: 2199160X, 2199160X

DOI: 10.1002/aelm.201500062

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Electronic, Optical and Magnetic Materials

Abstract

Recent advances in graphene-based electronics range from the discovery of fundamental physical phenomena to the development of new high-performance photosensitive devices. [ 1–5 ] These applications exploit not only the unique electronic properties of graphene but also additional functionalities that can be achieved by capping the graphene layer with another material or nanostructure, e.g., atomically thin fi lms, [ 6,7 ] carbon nanotubes [ 8 ] or inorganic nanoparticles. [ 8–10 ] Colloidal semiconductor quantum dots (QDs) are of particular interest as their optical properties can be fi ne-tuned by varying their size and/or composition. [ 11 ] In addition, colloidal synthesis enables QDs to be functionalized by doping [ 12 ] and/or surface encapsulation. [ 13 ] Recently, a photoresponsivity of 10 7 A W −1 was achieved by depositing QDs on graphene and explained in terms of trapping of photoexcited carriers on the QDs and charge transfer between them and the graphene layer. [ 9,10 ] This mechanism should be strongly dependent on the interface between the QDs and graphene. Furthermore, the ligands that encapsulate the QDs may provide a means of modifying the transfer of electronic charges and enhancing the electronic properties of the graphene layer. Here, we investigate the properties of single layer graphene (SLG) functionalized with an overlayer of near-infrared PbS colloidal quantum dots capped with thioglycerol/dithioglycerol or polyethylene glycol (PEG500 and PEG2000). We demonstrate that the polarity of the conductivity and the carrier concentration can be modifi ed, and photoresponsivity of SLG can be signifi cantly enhanced by the choice of ligands. By reducing the length of capping ligands, hence the thickness of the dielectric barrier between the QDs and the SLG, and by preserving the integrity of the ligand layer, we achieve the effi - cient transfer of photogenerated carriers from the QDs to the graphene before recombining, resulting in enhanced photoresponsivities of up to ≈10 9 A W −1 .

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Citations by journals

	1 2 3
ACS Photonics	ACS Photonics, 3, 4.84% ACS Photonics 3 publications, 4.84%
ACS Applied Electronic Materials	ACS Applied Electronic Materials, 3, 4.84% ACS Applied Electronic Materials 3 publications, 4.84%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 4.84% Journal of Materials Chemistry C 3 publications, 4.84%
Journal of Chemical Physics	Journal of Chemical Physics, 2, 3.23% Journal of Chemical Physics 2 publications, 3.23%
Nanomaterials	Nanomaterials, 2, 3.23% Nanomaterials 2 publications, 3.23%
2D Materials	2D Materials, 2, 3.23% 2D Materials 2 publications, 3.23%
Japanese Journal of Applied Physics, Part 1: Regular Papers & Short Notes	Japanese Journal of Applied Physics, Part 1: Regular Papers & Short Notes, 2, 3.23% Japanese Journal of Applied Physics, Part 1: Regular Papers & Short Notes 2 publications, 3.23%
Advanced Functional Materials	Advanced Functional Materials, 2, 3.23% Advanced Functional Materials 2 publications, 3.23%
Small	Small, 2, 3.23% Small 2 publications, 3.23%
Small Methods	Small Methods, 2, 3.23% Small Methods 2 publications, 3.23%
Advanced Optical Materials	Advanced Optical Materials, 2, 3.23% Advanced Optical Materials 2 publications, 3.23%
Advanced Electronic Materials	Advanced Electronic Materials, 2, 3.23% Advanced Electronic Materials 2 publications, 3.23%
ACS Nano	ACS Nano, 2, 3.23% ACS Nano 2 publications, 3.23%
ACS applied materials & interfaces	ACS applied materials & interfaces, 2, 3.23% ACS applied materials & interfaces 2 publications, 3.23%
Nano	Nano, 1, 1.61% Nano 1 publication, 1.61%
Electronics (Switzerland)	Electronics (Switzerland), 1, 1.61% Electronics (Switzerland) 1 publication, 1.61%
Frontiers in Materials	Frontiers in Materials, 1, 1.61% Frontiers in Materials 1 publication, 1.61%
Nature Photonics	Nature Photonics, 1, 1.61% Nature Photonics 1 publication, 1.61%
Nature Communications	Nature Communications, 1, 1.61% Nature Communications 1 publication, 1.61%
Rare Metals	Rare Metals, 1, 1.61% Rare Metals 1 publication, 1.61%
Scientific Reports	Scientific Reports, 1, 1.61% Scientific Reports 1 publication, 1.61%
MRS Advances	MRS Advances, 1, 1.61% MRS Advances 1 publication, 1.61%
Applied Surface Science	Applied Surface Science, 1, 1.61% Applied Surface Science 1 publication, 1.61%
Journal of Physics: Conference Series	Journal of Physics: Conference Series, 1, 1.61% Journal of Physics: Conference Series 1 publication, 1.61%
Nanotechnology	Nanotechnology, 1, 1.61% Nanotechnology 1 publication, 1.61%
Chinese Physics B	Chinese Physics B, 1, 1.61% Chinese Physics B 1 publication, 1.61%
Nano Express	Nano Express, 1, 1.61% Nano Express 1 publication, 1.61%
Ceramics International	Ceramics International, 1, 1.61% Ceramics International 1 publication, 1.61%
Advanced Quantum Technologies	Advanced Quantum Technologies, 1, 1.61% Advanced Quantum Technologies 1 publication, 1.61%
	1 2 3

Citations by publishers

	2 4 6 8 10 12 14
Wiley	Wiley, 14, 22.58% Wiley 14 publications, 22.58%
American Chemical Society (ACS)	American Chemical Society (ACS), 13, 20.97% American Chemical Society (ACS) 13 publications, 20.97%
IOP Publishing	IOP Publishing, 7, 11.29% IOP Publishing 7 publications, 11.29%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 5, 8.06% Royal Society of Chemistry (RSC) 5 publications, 8.06%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 4.84% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 4.84%
Springer Nature	Springer Nature, 3, 4.84% Springer Nature 3 publications, 4.84%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 3.23% American Institute of Physics (AIP) 2 publications, 3.23%
Elsevier	Elsevier, 2, 3.23% Elsevier 2 publications, 3.23%
Japan Society of Applied Physics	Japan Society of Applied Physics, 2, 3.23% Japan Society of Applied Physics 2 publications, 3.23%
World Scientific	World Scientific, 1, 1.61% World Scientific 1 publication, 1.61%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.61% Frontiers Media S.A. 1 publication, 1.61%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 1.61% Nonferrous Metals Society of China 1 publication, 1.61%
Materials Research Society	Materials Research Society, 1, 1.61% Materials Research Society 1 publication, 1.61%
Pleiades Publishing	Pleiades Publishing, 1, 1.61% Pleiades Publishing 1 publication, 1.61%
Walter de Gruyter	Walter de Gruyter, 1, 1.61% Walter de Gruyter 1 publication, 1.61%
American Physical Society (APS)	American Physical Society (APS), 1, 1.61% American Physical Society (APS) 1 publication, 1.61%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.61% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.61%
	2 4 6 8 10 12 14

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GOST Copy

Turyanska L. et al. Ligand‐Induced Control of Photoconductive Gain and Doping in a Hybrid Graphene–Quantum Dot Transistor // Advanced Electronic Materials. 2015. Vol. 1. No. 7. p. 1500062.

GOST all authors (up to 50) Copy

Turyanska L., Makarovsky O., Svatek S. A., Beton P., Mellor C. J., Patane A., Eaves L. J., Thomas N. R., Fay M., Marsden A. J., Wilson N. Ligand‐Induced Control of Photoconductive Gain and Doping in a Hybrid Graphene–Quantum Dot Transistor // Advanced Electronic Materials. 2015. Vol. 1. No. 7. p. 1500062.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1002/aelm.201500062

UR - https://doi.org/10.1002/aelm.201500062

TI - Ligand‐Induced Control of Photoconductive Gain and Doping in a Hybrid Graphene–Quantum Dot Transistor

T2 - Advanced Electronic Materials

AU - Turyanska, Lyudmila

AU - Makarovsky, O.N.

AU - Svatek, Simon A

AU - Beton, P.H.

AU - Mellor, C. J.

AU - Patane, A.

AU - Eaves, L J.

AU - Thomas, N R

AU - Fay, Michael

AU - Marsden, Alexander J.

AU - Wilson, Neil

PY - 2015

DA - 2015/06/05 00:00:00

PB - Wiley

SP - 1500062

IS - 7

VL - 1

SN - 2199-160X

ER -

BibTex |

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BibTex Copy

@article{2015_Turyanska,

author = {Lyudmila Turyanska and O.N. Makarovsky and Simon A Svatek and P.H. Beton and C. J. Mellor and A. Patane and L J. Eaves and N R Thomas and Michael Fay and Alexander J. Marsden and Neil Wilson},

title = {Ligand‐Induced Control of Photoconductive Gain and Doping in a Hybrid Graphene–Quantum Dot Transistor},

journal = {Advanced Electronic Materials},

year = {2015},

volume = {1},

publisher = {Wiley},

month = {jun},

url = {https://doi.org/10.1002/aelm.201500062},

number = {7},

pages = {1500062},

doi = {10.1002/aelm.201500062}

}

MLA

Cite this

MLA Copy

Turyanska, Lyudmila, et al. “Ligand‐Induced Control of Photoconductive Gain and Doping in a Hybrid Graphene–Quantum Dot Transistor.” Advanced Electronic Materials, vol. 1, no. 7, Jun. 2015, p. 1500062. https://doi.org/10.1002/aelm.201500062.

Found error?

Publisher

Wiley

Journal

Advanced Electronic Materials

Quartile SCImago

Quartile WOS

Impact factor

6.2

ISSN

2199160X (Print)
2199160X (Electronic)