Open Access
Advanced Energy Materials, volume 7, issue 17, pages 1700403
Manipulating Adsorption–Insertion Mechanisms in Nanostructured Carbon Materials for High‐Efficiency Sodium Ion Storage
Qiu Shen
1
,
Lifen Xiao
2, 3
,
Maria Sushko
3
,
Kee Sung Han
3
,
Yuyan Shao
3
,
Mengyu Yan
4
,
Xiuli Zhang
5
,
L. Q. Ma
4
,
Jiwen Feng
5
,
Yuliang Cao
1
,
Xinping Ai
1
,
Hanxi Yang
1
,
Jun Liu
3
5
State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics Wuhan Institute of Physics and Mathematics, Chinese Academy of Science Wuhan 430071 China
|
Publication type: Journal Article
Publication date: 2017-05-12
Journal:
Advanced Energy Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 27.8
ISSN: 16146832, 16146840
General Materials Science
Renewable Energy, Sustainability and the Environment
Abstract
Hard carbon is one of the most promising anode materials for sodium-ion batteries, but the low Coulombic efficiency is still a key barrier. In this paper, a series of nanostructured hard carbon materials with controlled architectures is synthesized. Using a combination of in situ X-ray diffraction mapping, ex situ nuclear magnetic resonance (NMR), electron paramagnetic resonance, electrochemical techniques, and simulations, an “adsorption–intercalation” mechanism is established for Na ion storage. During the initial stages of Na insertion, Na ions adsorb on the defect sites of hard carbon with a wide adsorption energy distribution, producing a sloping voltage profile. In the second stage, Na ions intercalate into graphitic layers with suitable spacing to form NaC x compounds similar to the Li ion intercalation process in graphite, producing a flat low voltage plateau. The cation intercalation with a flat voltage plateau should be enhanced and the sloping region should be avoided. Guided by this knowledge, nonporous hard carbon material has been developed which has achieved high reversible capacity and Coulombic efficiency to fulfill practical application.
Top-30
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Citations by publishers
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Elsevier
250 publications, 34.97%
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Wiley
194 publications, 27.13%
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American Chemical Society (ACS)
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Springer Nature
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2 publications, 0.28%
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Oxford University Press
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World Scientific
1 publication, 0.14%
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Shanghai Institute of Organic Chemistry
1 publication, 0.14%
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Frontiers Media S.A.
1 publication, 0.14%
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Cambridge University Press
1 publication, 0.14%
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Tianjin Daxue/Tianjin University
1 publication, 0.14%
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1 publication, 0.14%
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1 publication, 0.14%
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1 publication, 0.14%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.14%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Shen Q. et al. Manipulating Adsorption–Insertion Mechanisms in Nanostructured Carbon Materials for High‐Efficiency Sodium Ion Storage // Advanced Energy Materials. 2017. Vol. 7. No. 17. p. 1700403.
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Shen Q., Xiao L., Sushko M., Han K. S., Shao Y., Yan M., Zhang X., Ma L. Q., Feng J., Cao Y., Ai X., Yang H., Liu J. Manipulating Adsorption–Insertion Mechanisms in Nanostructured Carbon Materials for High‐Efficiency Sodium Ion Storage // Advanced Energy Materials. 2017. Vol. 7. No. 17. p. 1700403.
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TY - JOUR
DO - 10.1002/aenm.201700403
UR - https://doi.org/10.1002/aenm.201700403
TI - Manipulating Adsorption–Insertion Mechanisms in Nanostructured Carbon Materials for High‐Efficiency Sodium Ion Storage
T2 - Advanced Energy Materials
AU - Shen, Qiu
AU - Xiao, Lifen
AU - Feng, Jiwen
AU - Sushko, Maria
AU - Han, Kee Sung
AU - Shao, Yuyan
AU - Yan, Mengyu
AU - Zhang, Xiuli
AU - Ma, L. Q.
AU - Cao, Yuliang
AU - Ai, Xinping
AU - Yang, Hanxi
AU - Liu, Jun
PY - 2017
DA - 2017/05/12 00:00:00
PB - Wiley
SP - 1700403
IS - 17
VL - 7
SN - 1614-6832
SN - 1614-6840
ER -
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@article{2017_Shen,
author = {Qiu Shen and Lifen Xiao and Jiwen Feng and Maria Sushko and Kee Sung Han and Yuyan Shao and Mengyu Yan and Xiuli Zhang and L. Q. Ma and Yuliang Cao and Xinping Ai and Hanxi Yang and Jun Liu},
title = {Manipulating Adsorption–Insertion Mechanisms in Nanostructured Carbon Materials for High‐Efficiency Sodium Ion Storage},
journal = {Advanced Energy Materials},
year = {2017},
volume = {7},
publisher = {Wiley},
month = {may},
url = {https://doi.org/10.1002/aenm.201700403},
number = {17},
pages = {1700403},
doi = {10.1002/aenm.201700403}
}
Cite this
MLA
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Shen, Qiu, et al. “Manipulating Adsorption–Insertion Mechanisms in Nanostructured Carbon Materials for High‐Efficiency Sodium Ion Storage.” Advanced Energy Materials, vol. 7, no. 17, May. 2017, p. 1700403. https://doi.org/10.1002/aenm.201700403.