volume 20, issue 11, pages 987-988
Cleavage of Water by Visible-Light Irradiation of Colloidal CdS Solutions; Inhibition of Photocorrosion by RuO2
1
Inslitut de Chimie Physique. Ecolc Polytechniquc Fédérale Ecublens CH‐1015 Lausanne (Switzerland)
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Publication type: Journal Article
Publication date: 1981-11-01
—
General Chemistry
Catalysis
Abstract
The conversion of light into chemical fuels in photochemical devices equipped with semiconductor electrodes (e.g. of n-CdS) is associated with a serious problem: “holes” produced in the valence band of the semidonductor upon irradiation migrate to the surface where photocorrosion occurs. In mi-croheterogenous CdS systems this is remedied by a thin layer of RuO2. A CdS sol prepared in the presence of maleic anhydride/styrene copolymer has now been loaded with RuO2 and Pt; these CdS microelectrodes are surprisingly active catalysts for cleavage of H2O and H2S.
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