Hydrogen Peroxide Insular Dodecameric and Pentameric Clusters in Peroxosolvate Structures
Dmitry A Grishanov
1, 2
,
Mger A. Navasardyan
1, 2
,
Alexander G. Medvedev
1, 2
,
Ovadia Lev
3, 4
,
Petr V. Prikhodchenko
1, 2, 3, 4
,
Andrei V. Churakov
1, 2
Publication type: Journal Article
Publication date: 2017-10-19
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
28991407
General Chemistry
Catalysis
Abstract
Peroxosolvates of 2‐aminonicotinic acid (I) and lidocaine N‐oxide (II) including the largest insular hydrogen peroxide clusters were isolated and their crystal structures were determined by single‐crystal X‐ray diffraction. An unprecedented dodecameric hydrogen peroxide insular cluster was found in I. An unusual cross‐like pentameric cluster was observed in the structure of II. The topology of the (H2O2)12 assembly was never observed for small‐molecule clusters. In I and II new double and triple cross‐orientational disorders of H2O2 were found. Cluster II is the first example of a peroxosolvate crystal structure containing H2O2 molecules with a homoleptic hydrogen peroxide environment. In II, a hydrogen bond between an H2O2 molecule and a peptide group ‐CONH⋅⋅⋅O2H2 was observed for the first time.
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31
Total citations:
31
Citations from 2024:
10
(32%)
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GOST
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Grishanov D. A. et al. Hydrogen Peroxide Insular Dodecameric and Pentameric Clusters in Peroxosolvate Structures // Angewandte Chemie - International Edition. 2017. Vol. 56. No. 48. pp. 15241-15245.
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Grishanov D. A., Navasardyan M. A., Medvedev A. G., Lev O., Prikhodchenko P. V., Churakov A. V. Hydrogen Peroxide Insular Dodecameric and Pentameric Clusters in Peroxosolvate Structures // Angewandte Chemie - International Edition. 2017. Vol. 56. No. 48. pp. 15241-15245.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1002/anie.201709699
UR - https://onlinelibrary.wiley.com/doi/10.1002/anie.201709699
TI - Hydrogen Peroxide Insular Dodecameric and Pentameric Clusters in Peroxosolvate Structures
T2 - Angewandte Chemie - International Edition
AU - Grishanov, Dmitry A
AU - Navasardyan, Mger A.
AU - Medvedev, Alexander G.
AU - Lev, Ovadia
AU - Prikhodchenko, Petr V.
AU - Churakov, Andrei V.
PY - 2017
DA - 2017/10/19
PB - Wiley
SP - 15241-15245
IS - 48
VL - 56
PMID - 28991407
SN - 1433-7851
SN - 1521-3773
ER -
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BibTex (up to 50 authors)
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@article{2017_Grishanov,
author = {Dmitry A Grishanov and Mger A. Navasardyan and Alexander G. Medvedev and Ovadia Lev and Petr V. Prikhodchenko and Andrei V. Churakov},
title = {Hydrogen Peroxide Insular Dodecameric and Pentameric Clusters in Peroxosolvate Structures},
journal = {Angewandte Chemie - International Edition},
year = {2017},
volume = {56},
publisher = {Wiley},
month = {oct},
url = {https://onlinelibrary.wiley.com/doi/10.1002/anie.201709699},
number = {48},
pages = {15241--15245},
doi = {10.1002/anie.201709699}
}
Cite this
MLA
Copy
Grishanov, Dmitry A., et al. “Hydrogen Peroxide Insular Dodecameric and Pentameric Clusters in Peroxosolvate Structures.” Angewandte Chemie - International Edition, vol. 56, no. 48, Oct. 2017, pp. 15241-15245. https://onlinelibrary.wiley.com/doi/10.1002/anie.201709699.