Angewandte Chemie - International Edition, volume 61, issue 4
Highly Efficient Biobased Synthesis of Acrylic Acid
Publication type: Journal Article
Publication date: 2021-12-13
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
Petrochemical based polymers, paints and coatings are cornerstones of modern industry but our future sustainable society demands greener processes and renewable feedstock materials. A challenge is to access platform monomers from biomass resources while integrating the principles of green chemistry in their chemical synthesis. We present a synthesis route starting from biomass-derived furfural towards the commonly used monomers maleic anhydride and acrylic acid, implementing environmentally benign photooxygenation, aerobic oxidation and ethenolysis reactions. Maleic anhydride and acrylic acid, transformed into sodium acrylate, were isolated in yields of 85 % (2 steps) and 81 % (4 steps), respectively. With minimal waste and high atom efficiency, this biobased route provides a viable alternative to access key monomers.
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HERMENS J. M., Jensma A., Feringa B. L. Highly Efficient Biobased Synthesis of Acrylic Acid // Angewandte Chemie - International Edition. 2021. Vol. 61. No. 4.
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HERMENS J. M., Jensma A., Feringa B. L. Highly Efficient Biobased Synthesis of Acrylic Acid // Angewandte Chemie - International Edition. 2021. Vol. 61. No. 4.
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TY - JOUR
DO - 10.1002/anie.202112618
UR - https://doi.org/10.1002/anie.202112618
TI - Highly Efficient Biobased Synthesis of Acrylic Acid
T2 - Angewandte Chemie - International Edition
AU - Jensma, Andries
AU - Feringa, Ben L.
AU - HERMENS, JOHANNES M.
PY - 2021
DA - 2021/12/13
PB - Wiley
IS - 4
VL - 61
SN - 1433-7851
SN - 1521-3773
ER -
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@article{2021_HERMENS,
author = {Andries Jensma and Ben L. Feringa and JOHANNES M. HERMENS},
title = {Highly Efficient Biobased Synthesis of Acrylic Acid},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {61},
publisher = {Wiley},
month = {dec},
url = {https://doi.org/10.1002/anie.202112618},
number = {4},
doi = {10.1002/anie.202112618}
}