Metal‐Free Aminocarbonylation of p ‐Quinone Methides with Isocyanides: Synthesis of Sterically Hindered α‐Arylated Acetamides
2
Academy of Scientific and Innovative Research (AcSIR) Ghaziabad 201002 INDIA
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Publication type: Journal Article
Publication date: 2022-09-08
scimago Q2
wos Q2
SJR: 0.751
CiteScore: 5.9
Impact factor: 3.3
ISSN: 18614728, 1861471X
PubMed ID:
35986585
General Chemistry
Organic Chemistry
Biochemistry
Abstract
The synthesis of sterically hindered α-arylated acetamides generally requires a multistep reaction sequence and is also difficult to access due to steric constraints. This protocol allows the synthesis of sterically hindered α-arylated acetamides in moderate to high yields via 1,6-addition of isocyanides to p-quinone methides in the presence of BF3 .OEt2 . The present transformation features transition metal-free conditions, avoiding the use of toxic carbon monoxide, broad substrate scope, mild reaction conditions, and operational simplicity.
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Shirsath S. R. et al. Metal‐Free Aminocarbonylation of p ‐Quinone Methides with Isocyanides: Synthesis of Sterically Hindered α‐Arylated Acetamides // Chemistry - An Asian Journal. 2022. Vol. 17. No. 20.
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Shirsath S. R., More D. A., Muthukrishnan M. Metal‐Free Aminocarbonylation of p ‐Quinone Methides with Isocyanides: Synthesis of Sterically Hindered α‐Arylated Acetamides // Chemistry - An Asian Journal. 2022. Vol. 17. No. 20.
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TY - JOUR
DO - 10.1002/asia.202200642
UR - https://doi.org/10.1002/asia.202200642
TI - Metal‐Free Aminocarbonylation of p ‐Quinone Methides with Isocyanides: Synthesis of Sterically Hindered α‐Arylated Acetamides
T2 - Chemistry - An Asian Journal
AU - Shirsath, Sachin R
AU - More, Devidas A
AU - Muthukrishnan, M.
PY - 2022
DA - 2022/09/08
PB - Wiley
IS - 20
VL - 17
PMID - 35986585
SN - 1861-4728
SN - 1861-471X
ER -
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BibTex (up to 50 authors)
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@article{2022_Shirsath,
author = {Sachin R Shirsath and Devidas A More and M. Muthukrishnan},
title = {Metal‐Free Aminocarbonylation of p ‐Quinone Methides with Isocyanides: Synthesis of Sterically Hindered α‐Arylated Acetamides},
journal = {Chemistry - An Asian Journal},
year = {2022},
volume = {17},
publisher = {Wiley},
month = {sep},
url = {https://doi.org/10.1002/asia.202200642},
number = {20},
doi = {10.1002/asia.202200642}
}