Berichte der Bunsengesellschaft für physikalische Chemie, volume 86, issue 4, pages 301-305
Photo‐Degradation and Fluorescence of Colloidal‐Cadmium Sulfide in Aqueous Solution
Publication type: Journal Article
Publication date: 1982-04-01
Quartile SCImago
— Quartile WOS
—
Impact factor: —
ISSN: 00059021, 00059021
General Chemical Engineering
Abstract
Colloidal cadmium sulfide deposited on 13 nm silicon dioxide particles shows a weak fluorescence with a maximum at 620 – 660 nm (depending on the sample). Oxygen does not quench the fluorescence. All anions exert a quenching effect at concentrations below 10−3 M, S2-, Br−, and I− being the most effective ones. Tl+, Ag+, Pb2+, and Cu2+ strongly quench the fluorescence at concentrations below 10−4 M. Nitrobenzene quenches at higher concentrations in the 10−3 M range. Quenching is attributed to adsorbed ions or molecules. In the case of the anions, a mechanism is proposed in which positive hole-anion pairs are formed at the surface of the colloidal particles before neutralization by electrons takes place. In the case of the cations and of nitrobenzene, quenching is explained by electron capture. Colloidal CdS doped with less than 1% Cu2+ or Ag+ showed a much stronger fluorescence than undoped samples.—Colloidal cadmium sulfide is degraded by light only in the presence of oxygen the quantum yield in aerated solution being 0.04. The action of oxygen is mainly attributed to a reaction with intermediates of the sulfide oxidation by positive holes. In the presence of Tl+ or Pb2+ ions at some 10−5 M, the photo-degradation is drastically promoted up to a quantum yield of 0.24. Cu2+ and Ag+, however, retard the degradation. Both effects are understood in terms of electron scavenging by the adsorbed metal ions and reoxidation of the reduced metal by oxygen or by positive holes. Sodium sulfide protects cadmium sulfide from degradation. In the absence of air, small amounts of hydrogen are formed in Na2S containing solution.
Top-30
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Langmuir
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Citations by publishers
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Elsevier
63 publications, 25.2%
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Wiley
42 publications, 16.8%
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American Chemical Society (ACS)
38 publications, 15.2%
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Springer Nature
20 publications, 8%
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Royal Society of Chemistry (RSC)
15 publications, 6%
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American Institute of Physics (AIP)
7 publications, 2.8%
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The Chemical Society of Japan
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American Physical Society (APS)
4 publications, 1.6%
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Multidisciplinary Digital Publishing Institute (MDPI)
3 publications, 1.2%
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Materials Research Society
2 publications, 0.8%
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American Vacuum Society
1 publication, 0.4%
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CSIRO Publishing
1 publication, 0.4%
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The Electrochemical Society
1 publication, 0.4%
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Taylor & Francis
1 publication, 0.4%
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Walter de Gruyter
1 publication, 0.4%
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Optical Society of America
1 publication, 0.4%
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American Association for the Advancement of Science (AAAS)
1 publication, 0.4%
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Trans Tech Publications
1 publication, 0.4%
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Annual Reviews
1 publication, 0.4%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.4%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Henglein A. Photo‐Degradation and Fluorescence of Colloidal‐Cadmium Sulfide in Aqueous Solution // Berichte der Bunsengesellschaft für physikalische Chemie. 1982. Vol. 86. No. 4. pp. 301-305.
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Henglein A. Photo‐Degradation and Fluorescence of Colloidal‐Cadmium Sulfide in Aqueous Solution // Berichte der Bunsengesellschaft für physikalische Chemie. 1982. Vol. 86. No. 4. pp. 301-305.
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TY - JOUR
DO - 10.1002/bbpc.19820860409
UR - https://doi.org/10.1002/bbpc.19820860409
TI - Photo‐Degradation and Fluorescence of Colloidal‐Cadmium Sulfide in Aqueous Solution
T2 - Berichte der Bunsengesellschaft für physikalische Chemie
AU - Henglein, A.
PY - 1982
DA - 1982/04/01 01:00:00
PB - Wiley
SP - 301-305
IS - 4
VL - 86
SN - 0005-9021
SN - 0005-9021
ER -
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@article{1982_Henglein,
author = {A. Henglein},
title = {Photo‐Degradation and Fluorescence of Colloidal‐Cadmium Sulfide in Aqueous Solution},
journal = {Berichte der Bunsengesellschaft für physikalische Chemie},
year = {1982},
volume = {86},
publisher = {Wiley},
month = {apr},
url = {https://doi.org/10.1002/bbpc.19820860409},
number = {4},
pages = {301--305},
doi = {10.1002/bbpc.19820860409}
}
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MLA
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Henglein, A.. “Photo‐Degradation and Fluorescence of Colloidal‐Cadmium Sulfide in Aqueous Solution.” Berichte der Bunsengesellschaft für physikalische Chemie, vol. 86, no. 4, Apr. 1982, pp. 301-305. https://doi.org/10.1002/bbpc.19820860409.