Open Access
Open access
Carbon Energy, volume 3, issue 6, pages 866-894

Progress and perspective of the cathode/electrolyte interface construction in all‐solid‐state lithium batteries

Publication typeJournal Article
Publication date2021-07-22
Journal: Carbon Energy
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor20.5
ISSN26379368, 26379368
Materials Chemistry
Materials Science (miscellaneous)
Renewable Energy, Sustainability and the Environment
Energy (miscellaneous)
Abstract
Security risks of flammability and explosion represent major problems with the use of conventional lithium rechargeable batteries using a liquid electrolyte. The application of solid-state electrolytes could effectively help to avoid these safety concerns. However, integrating the solid-state electrolytes into the all-solid-state lithium batteries is still a huge challenge mainly due to the high interfacial resistance present in the entire battery, especially at the interface between the cathode and the solid-state electrolyte pellet and the interfaces inside the cathode. Herein, recent progress made from investigations of cathode/solid-state electrolyte interfacial behaviors including the contact problem, the interlayer diffusion issue, the space-charge layer effect, and electrochemical compatibility is presented according to the classification of oxide-, sulfide-, and polymer-based solid-state electrolytes. We also propose strategies for the construction of ideal next-generation cathode/solid-state electrolyte interfaces with high room-temperature ionic conductivity, stable interfacial contact during long cycling, free formation of the space-charge region, and good compatibility with high-voltage cathodes.

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GOST |
Cite this
GOST Copy
Su S. et al. Progress and perspective of the cathode/electrolyte interface construction in all‐solid‐state lithium batteries // Carbon Energy. 2021. Vol. 3. No. 6. pp. 866-894.
GOST all authors (up to 50) Copy
Su S., Ma J., Zhao L., Lin K., Li Q., Lv S., Kang F., He Y. Progress and perspective of the cathode/electrolyte interface construction in all‐solid‐state lithium batteries // Carbon Energy. 2021. Vol. 3. No. 6. pp. 866-894.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1002/cey2.129
UR - https://doi.org/10.1002/cey2.129
TI - Progress and perspective of the cathode/electrolyte interface construction in all‐solid‐state lithium batteries
T2 - Carbon Energy
AU - Su, Shiming
AU - Ma, Jiabin
AU - Li, Qidong
AU - Kang, Feiyu
AU - He, Yan-bing
AU - Zhao, Liang
AU - Lin, Kui
AU - Lv, Shasha
PY - 2021
DA - 2021/07/22 00:00:00
PB - Wiley
SP - 866-894
IS - 6
VL - 3
SN - 2637-9368
SN - 2637-9368
ER -
BibTex |
Cite this
BibTex Copy
@article{2021_Su,
author = {Shiming Su and Jiabin Ma and Qidong Li and Feiyu Kang and Yan-bing He and Liang Zhao and Kui Lin and Shasha Lv},
title = {Progress and perspective of the cathode/electrolyte interface construction in all‐solid‐state lithium batteries},
journal = {Carbon Energy},
year = {2021},
volume = {3},
publisher = {Wiley},
month = {jul},
url = {https://doi.org/10.1002/cey2.129},
number = {6},
pages = {866--894},
doi = {10.1002/cey2.129}
}
MLA
Cite this
MLA Copy
Su, Shiming, et al. “Progress and perspective of the cathode/electrolyte interface construction in all‐solid‐state lithium batteries.” Carbon Energy, vol. 3, no. 6, Jul. 2021, pp. 866-894. https://doi.org/10.1002/cey2.129.
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