Nature of Bonding in Donor-Acceptor Interactions Exemplified by Complexes of N-Heterocyclic Carbenes with 1,2,5-Telluradiazoles
Nikolay A. Pushkarevsky
1, 2, 3, 4
,
Pavel A. Petrov
1, 2, 3, 4
,
Denis S Grigoriev
1, 3
,
Anton I. Smolentsev
1, 2
,
Lucia M. Lee
5
,
Florian Kleemiss
6
,
Georgi E Salnikov
2, 7
,
Georgy E Salnikov
4, 8
,
Sergey N. Konchenko
1, 2, 3, 4
,
Ignacio Vargas-Baca
5, 9
,
Simon Grabowsky
6, 10
,
Jens Beckmann
6, 10
,
Andrey V. Zibarev
7, 8, 11, 12
6
9
Department of Chemistry and Chemical Biology McMaster University L8S 4M1 Ontario Canada
|
10
Publication type: Journal Article
Publication date: 2017-07-31
scimago Q1
wos Q2
SJR: 0.981
CiteScore: 6.7
Impact factor: 3.7
ISSN: 09476539, 15213765
PubMed ID:
28675774
General Chemistry
Catalysis
Organic Chemistry
Abstract
Comprehensive structural, spectroscopic, and quantum chemical analyses of new donor–acceptor complexes between N‐heterocyclic carbenes and 1,2,5‐telluradiazoles and a comparison with previously known complexes involving tellurenyl cations showed that the dative C−Te bonds cannot be solitarily described with only one Lewis formula. Canonical Lewis formulas that denote covalency and arrows emphasizing ionicity complement each other in varying extents. Evaluation of the relative weights of these resonance forms requires proper bonding description with a well‐balanced toolbox of analytical methods. If for conciseness only, one resonance form is used, it must be the most significant one according to the analytical evaluation. If unclear, all significant resonance forms should be displayed.
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Pushkarevsky N. A. et al. Nature of Bonding in Donor-Acceptor Interactions Exemplified by Complexes of N-Heterocyclic Carbenes with 1,2,5-Telluradiazoles // Chemistry - A European Journal. 2017. Vol. 23. No. 46. pp. 10987-10991.
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Pushkarevsky N. A., Petrov P. A., Grigoriev D. S., Smolentsev A. I., Lee L. M., Kleemiss F., Salnikov G. E., Salnikov G. E., Konchenko S. N., Vargas-Baca I., Grabowsky S., Beckmann J., Zibarev A. V. Nature of Bonding in Donor-Acceptor Interactions Exemplified by Complexes of N-Heterocyclic Carbenes with 1,2,5-Telluradiazoles // Chemistry - A European Journal. 2017. Vol. 23. No. 46. pp. 10987-10991.
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TY - JOUR
DO - 10.1002/chem.201703018
UR - https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201703018
TI - Nature of Bonding in Donor-Acceptor Interactions Exemplified by Complexes of N-Heterocyclic Carbenes with 1,2,5-Telluradiazoles
T2 - Chemistry - A European Journal
AU - Pushkarevsky, Nikolay A.
AU - Petrov, Pavel A.
AU - Grigoriev, Denis S
AU - Smolentsev, Anton I.
AU - Lee, Lucia M.
AU - Kleemiss, Florian
AU - Salnikov, Georgi E
AU - Salnikov, Georgy E
AU - Konchenko, Sergey N.
AU - Vargas-Baca, Ignacio
AU - Grabowsky, Simon
AU - Beckmann, Jens
AU - Zibarev, Andrey V.
PY - 2017
DA - 2017/07/31
PB - Wiley
SP - 10987-10991
IS - 46
VL - 23
PMID - 28675774
SN - 0947-6539
SN - 1521-3765
ER -
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BibTex (up to 50 authors)
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@article{2017_Pushkarevsky,
author = {Nikolay A. Pushkarevsky and Pavel A. Petrov and Denis S Grigoriev and Anton I. Smolentsev and Lucia M. Lee and Florian Kleemiss and Georgi E Salnikov and Georgy E Salnikov and Sergey N. Konchenko and Ignacio Vargas-Baca and Simon Grabowsky and Jens Beckmann and Andrey V. Zibarev},
title = {Nature of Bonding in Donor-Acceptor Interactions Exemplified by Complexes of N-Heterocyclic Carbenes with 1,2,5-Telluradiazoles},
journal = {Chemistry - A European Journal},
year = {2017},
volume = {23},
publisher = {Wiley},
month = {jul},
url = {https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201703018},
number = {46},
pages = {10987--10991},
doi = {10.1002/chem.201703018}
}
Cite this
MLA
Copy
Pushkarevsky, Nikolay A., et al. “Nature of Bonding in Donor-Acceptor Interactions Exemplified by Complexes of N-Heterocyclic Carbenes with 1,2,5-Telluradiazoles.” Chemistry - A European Journal, vol. 23, no. 46, Jul. 2017, pp. 10987-10991. https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201703018.