Porphyrinylphosphonate‐Based Metal–Organic Framework: Tuning Proton Conductivity by Ligand Design
Тип публикации: Journal Article
Дата публикации: 2020-12-23
scimago Q1
wos Q2
БС1
SJR: 0.981
CiteScore: 6.7
Impact factor: 3.7
ISSN: 09476539, 15213765
PubMed ID:
33017090
General Chemistry
Catalysis
Organic Chemistry
Краткое описание
A novel metal–organic framework [Zn3(Ni‐H2TPPP)(Ni‐H4TPPP)(Ni‐H5TPPP)⋅7(CH3)2NH2⋅DMF⋅7 H2O] (where Ni‐HxTPPP (x=2,4,5) are partially deprotonated [5,10,15,20‐tetrakis(3‐(phosphonatophenyl)‐porphyrinato(2‐))]nickel(II) species), IPCE‐2Ni, with outstanding proton conductivity (1.0×10−2 S cm−1 at 75 °C and 95 % relative humidity) has been obtained. The high concentration of free phosphonate groups and compensating dimethylammonium cations bound by hydrogen bonds in the unique crystal structure of IPCE‐2Ni is a key factor responsible for the observed high proton conductivity, which is one order of magnitude higher than for the corresponding MOF based on 5,10,15,20‐tetrakis(4‐(phosphonatophenyl)porphyrinato(2‐))]nickel(II) IPCE‐1Ni and comparable with that of leaders among MOFs.
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Enakieva Y. Y. et al. Porphyrinylphosphonate‐Based Metal–Organic Framework: Tuning Proton Conductivity by Ligand Design // Chemistry - A European Journal. 2020. Vol. 27. No. 5. pp. 1598-1602.
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Enakieva Y. Y., Sinelshchikova A., Grigoriev M. S., Chernyshev V. V., Kovalenko K. A., Stenina I. A., Yaroslavtsev A. B., Yaroslavtsev A. B., Gorbunova Y. G., Tsivadze A. Porphyrinylphosphonate‐Based Metal–Organic Framework: Tuning Proton Conductivity by Ligand Design // Chemistry - A European Journal. 2020. Vol. 27. No. 5. pp. 1598-1602.
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TY - JOUR
DO - 10.1002/chem.202003893
UR - https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.202003893
TI - Porphyrinylphosphonate‐Based Metal–Organic Framework: Tuning Proton Conductivity by Ligand Design
T2 - Chemistry - A European Journal
AU - Enakieva, Yulia Yu.
AU - Sinelshchikova, Anna
AU - Grigoriev, Mikhail S.
AU - Chernyshev, V. V.
AU - Kovalenko, Konstantin A.
AU - Stenina, Irina A
AU - Yaroslavtsev, A. B.
AU - Yaroslavtsev, Andrey B
AU - Gorbunova, Yulia G.
AU - Tsivadze, Aslan
PY - 2020
DA - 2020/12/23
PB - Wiley
SP - 1598-1602
IS - 5
VL - 27
PMID - 33017090
SN - 0947-6539
SN - 1521-3765
ER -
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@article{2020_Enakieva,
author = {Yulia Yu. Enakieva and Anna Sinelshchikova and Mikhail S. Grigoriev and V. V. Chernyshev and Konstantin A. Kovalenko and Irina A Stenina and A. B. Yaroslavtsev and Andrey B Yaroslavtsev and Yulia G. Gorbunova and Aslan Tsivadze},
title = {Porphyrinylphosphonate‐Based Metal–Organic Framework: Tuning Proton Conductivity by Ligand Design},
journal = {Chemistry - A European Journal},
year = {2020},
volume = {27},
publisher = {Wiley},
month = {dec},
url = {https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.202003893},
number = {5},
pages = {1598--1602},
doi = {10.1002/chem.202003893}
}
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MLA
Скопировать
Enakieva, Yulia Yu., et al. “Porphyrinylphosphonate‐Based Metal–Organic Framework: Tuning Proton Conductivity by Ligand Design.” Chemistry - A European Journal, vol. 27, no. 5, Dec. 2020, pp. 1598-1602. https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.202003893.
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