The Adsorption of Oxygen and Coadsorption of CO and Oxygen on Structurally Well-Defined PdAg Surface Alloys
Publication type: Journal Article
Publication date: 2012-08-07
scimago Q2
wos Q3
SJR: 0.553
CiteScore: 3.6
Impact factor: 2.2
ISSN: 14394235, 14397641
PubMed ID:
22887474
Physical and Theoretical Chemistry
Atomic and Molecular Physics, and Optics
Abstract
The dissociative interaction of oxygen with structurally well-defined monolayer Pd(x)Ag(1-x)/Pd(111) surface alloys of different compositions, with well-known distributions of the respective surface atoms (A. K. Engstfeld et al., Phys. Chem. Chem. Phys. 2012, 14, 10754-10761), and the coadsorption of/reaction with CO on oxygen pre-covered surfaces were studied by high-resolution electron energy loss spectroscopy (HREELS) and temperature-programmed desorption/reaction spectroscopy (TPD/TPR). The impact of geometric ensemble effects as well as electronic ligand and strain effects on the adsorption and reaction behaviour of the respective species on the bimetallic surfaces is elucidated and compared with related systems such as CO adsorption on similar surfaces and oxygen adsorption on a Pd(67)Ag(33)(111) bulk alloy surface. The data show a clear dominance of ensemble effects on the oxygen adsorption and CO coadsorption behaviour, with oxygen adsorption limited to threefold-hollow sites on Pd(3) sites, while the combined electronic effects, as evident from modifications in the adsorption and reaction characteristics on the Pd sites, are small.
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13
Total citations:
13
Citations from 2024:
4
(30.76%)
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GOST
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Farkas Á. et al. The Adsorption of Oxygen and Coadsorption of CO and Oxygen on Structurally Well-Defined PdAg Surface Alloys // ChemPhysChem. 2012. Vol. 13. No. 15. pp. 3516-3525.
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Farkas Á., Diemant T., Bansmann J., Behm R. J. The Adsorption of Oxygen and Coadsorption of CO and Oxygen on Structurally Well-Defined PdAg Surface Alloys // ChemPhysChem. 2012. Vol. 13. No. 15. pp. 3516-3525.
Cite this
RIS
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TY - JOUR
DO - 10.1002/cphc.201200477
UR - https://doi.org/10.1002/cphc.201200477
TI - The Adsorption of Oxygen and Coadsorption of CO and Oxygen on Structurally Well-Defined PdAg Surface Alloys
T2 - ChemPhysChem
AU - Farkas, Á.
AU - Diemant, Thomas
AU - Bansmann, Joachim
AU - Behm, R. J.
PY - 2012
DA - 2012/08/07
PB - Wiley
SP - 3516-3525
IS - 15
VL - 13
PMID - 22887474
SN - 1439-4235
SN - 1439-7641
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2012_Farkas,
author = {Á. Farkas and Thomas Diemant and Joachim Bansmann and R. J. Behm},
title = {The Adsorption of Oxygen and Coadsorption of CO and Oxygen on Structurally Well-Defined PdAg Surface Alloys},
journal = {ChemPhysChem},
year = {2012},
volume = {13},
publisher = {Wiley},
month = {aug},
url = {https://doi.org/10.1002/cphc.201200477},
number = {15},
pages = {3516--3525},
doi = {10.1002/cphc.201200477}
}
Cite this
MLA
Copy
Farkas, Á., et al. “The Adsorption of Oxygen and Coadsorption of CO and Oxygen on Structurally Well-Defined PdAg Surface Alloys.” ChemPhysChem, vol. 13, no. 15, Aug. 2012, pp. 3516-3525. https://doi.org/10.1002/cphc.201200477.