volume 2010 issue 9 pages 1772-1777

C2-Functionalization of 1-Substituted Imidazoles with Aldehydes and Electron-Deficient Acetylenes: A Novel Three-Component Reaction

Publication typeJournal Article
Publication date2010-03-01
scimago Q2
wos Q2
SJR0.558
CiteScore4.3
Impact factor2.7
ISSN1434193X, 10990690
Organic Chemistry
Physical and Theoretical Chemistry
Abstract
A novel three-component reaction between 1-substituted imidazoles, aldehydes, and electron-deficient acetylenes proceeds under mild conditions (20―25 °C, no catalyst, no solvent) to form an unknown family of C2-functionalized imidazoles in up to 74 % yield, the function constituting a push-pull combination of enol ether and acrylic moieties. In the case of cyanophenylacetylene, the function is built up stereospecifically to have the (Z) configuration. The interaction presumably occurs via zwitterion and carbene intermediates. The results contribute to basic imidazole and acetylene chemistry and open a shortcut to promising drug candidates.
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GOST |
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GOST Copy
Trofimov B. A. et al. C2-Functionalization of 1-Substituted Imidazoles with Aldehydes and Electron-Deficient Acetylenes: A Novel Three-Component Reaction // European Journal of Organic Chemistry. 2010. Vol. 2010. No. 9. pp. 1772-1777.
GOST all authors (up to 50) Copy
Trofimov B. A., Andriyankova L. V., Belyaeva K. V., Mal’kina A. G., Nikitina L. P., Afonin A., Ushakov I. C2-Functionalization of 1-Substituted Imidazoles with Aldehydes and Electron-Deficient Acetylenes: A Novel Three-Component Reaction // European Journal of Organic Chemistry. 2010. Vol. 2010. No. 9. pp. 1772-1777.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1002/ejoc.200901397
UR - https://doi.org/10.1002/ejoc.200901397
TI - C2-Functionalization of 1-Substituted Imidazoles with Aldehydes and Electron-Deficient Acetylenes: A Novel Three-Component Reaction
T2 - European Journal of Organic Chemistry
AU - Trofimov, B. A.
AU - Andriyankova, Ludmila V.
AU - Belyaeva, Kseniya V
AU - Mal’kina, Anastasiya G.
AU - Nikitina, Lina P.
AU - Afonin, A.V.
AU - Ushakov, Igor
PY - 2010
DA - 2010/03/01
PB - Wiley
SP - 1772-1777
IS - 9
VL - 2010
SN - 1434-193X
SN - 1099-0690
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2010_Trofimov,
author = {B. A. Trofimov and Ludmila V. Andriyankova and Kseniya V Belyaeva and Anastasiya G. Mal’kina and Lina P. Nikitina and A.V. Afonin and Igor Ushakov},
title = {C2-Functionalization of 1-Substituted Imidazoles with Aldehydes and Electron-Deficient Acetylenes: A Novel Three-Component Reaction},
journal = {European Journal of Organic Chemistry},
year = {2010},
volume = {2010},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/ejoc.200901397},
number = {9},
pages = {1772--1777},
doi = {10.1002/ejoc.200901397}
}
MLA
Cite this
MLA Copy
Trofimov, B. A., et al. “C2-Functionalization of 1-Substituted Imidazoles with Aldehydes and Electron-Deficient Acetylenes: A Novel Three-Component Reaction.” European Journal of Organic Chemistry, vol. 2010, no. 9, Mar. 2010, pp. 1772-1777. https://doi.org/10.1002/ejoc.200901397.