Laser and Photonics Reviews, volume 12, issue 1, pages 1700227

Metal-Dielectric Nanocavity for Real-Time Tracing Molecular Events with Temperature Feedback

Publication typeJournal Article
Publication date2017-11-15
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor11
ISSN18638880, 18638899
Electronic, Optical and Magnetic Materials
Atomic and Molecular Physics, and Optics
Condensed Matter Physics
Abstract
Plasmonic nanoparticles coupled with metallic films forming nanometer scale cavities have recently emerged as a powerful tool for enhancement of light-matter interaction. Despite high efficiency for sensing and light emission, such nanocavities exhibit harmful and uncontrolled optical heating which limits the ranges of light intensities and working temperature. In contrast to plasmonic nanoparticles, all-dielectric counterparts possess low Ohmic losses, high temperature stability along with a strong temperature-dependent Raman response. Here, we demonstrate that a silicon nanoparticle coupled with a thin gold film can serve as a multifunctional metal-dielectric (hybrid) nanocavity operating up to 1200 K. Resonant interaction of light with such nanocavity enables molecular sensing, heat-induced molecular events (protein unfolding), and their real-time tracing with a nanoscale thermometry through the monitoring enhanced Raman scattering both from the nanoparticle and analyzed molecules. We model numerically the thermo-optical properties of the hybrid nanocavity and reveal two alternative regimes of operation - with and without strong optical heating while other functionalities are preserved. We believe that the concept of the multifunctional hybrid nanocavities holds great potential for diverse photochemical and photophysical applications.

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Milichko V. A. et al. Metal-Dielectric Nanocavity for Real-Time Tracing Molecular Events with Temperature Feedback // Laser and Photonics Reviews. 2017. Vol. 12. No. 1. p. 1700227.
GOST all authors (up to 50) Copy
Milichko V. A., Zuev D., Krasnok A. E., Zograf G., Volodina K., Krasilin A., Mukhin I. S., Dmitriev P. A., Vinogradov V., Makarov S. V., Belov P. A. Metal-Dielectric Nanocavity for Real-Time Tracing Molecular Events with Temperature Feedback // Laser and Photonics Reviews. 2017. Vol. 12. No. 1. p. 1700227.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1002/lpor.201700227
UR - https://doi.org/10.1002%2Flpor.201700227
TI - Metal-Dielectric Nanocavity for Real-Time Tracing Molecular Events with Temperature Feedback
T2 - Laser and Photonics Reviews
AU - Dmitriev, Pavel A.
AU - Volodina, Katerina
AU - Milichko, Valentin A.
AU - Zuev, Dmitry
AU - Krasnok, A E
AU - Zograf, George
AU - Krasilin, Andrei
AU - Mukhin, Ivan S.
AU - Vinogradov, Vladimir
AU - Makarov, Sergey V.
AU - Belov, Pavel A.
PY - 2017
DA - 2017/11/15 00:00:00
PB - Wiley
SP - 1700227
IS - 1
VL - 12
SN - 1863-8880
SN - 1863-8899
ER -
BibTex |
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BibTex Copy
@article{2017_Milichko,
author = {Pavel A. Dmitriev and Katerina Volodina and Valentin A. Milichko and Dmitry Zuev and A E Krasnok and George Zograf and Andrei Krasilin and Ivan S. Mukhin and Vladimir Vinogradov and Sergey V. Makarov and Pavel A. Belov},
title = {Metal-Dielectric Nanocavity for Real-Time Tracing Molecular Events with Temperature Feedback},
journal = {Laser and Photonics Reviews},
year = {2017},
volume = {12},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002%2Flpor.201700227},
number = {1},
pages = {1700227},
doi = {10.1002/lpor.201700227}
}
MLA
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MLA Copy
Milichko, Valentin A., et al. “Metal-Dielectric Nanocavity for Real-Time Tracing Molecular Events with Temperature Feedback.” Laser and Photonics Reviews, vol. 12, no. 1, Nov. 2017, p. 1700227. https://doi.org/10.1002%2Flpor.201700227.
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