Hofmeister Salt Effects on the LCST Behavior of Poly(2-Oxazoline) Star Ionomers
Тип публикации: Journal Article
Дата публикации: 2012-08-22
scimago Q1
wos Q2
БС1
SJR: 1.078
CiteScore: 8.4
Impact factor: 4.3
ISSN: 10221336, 15213927
PubMed ID:
22911889
Materials Chemistry
Organic Chemistry
Polymers and Plastics
Краткое описание
Effects of pH, ionic strength, and type of salt (variation of anions) on the cloud-point temperature (T(CP)) of thermoresponsive poly(2-ethyl-2-oxazoline) star ionomers are investigated. T(CP) s can be varied in a wide range, from 10 to >95 °C, corresponding with the Hofmeister series and the ionization of the core. Addition of salt weakens the influence of pH. For star copolymer with an amine core similar trends are observed as for star copolymers with a carboxylic acid core, although the presence of a chaotropic salt affords an inversion of the effect of pH, that is, T(CP) s are lowest at pH 3, where the amine groups are fully protonated. This effect is likely due to the specific binding of chaotropic anions to the amine and ammonium groups, which is not observed for carboxylic acid groups.
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Ten Brummelhuis N., Secker C., Schlaad H. Hofmeister Salt Effects on the LCST Behavior of Poly(2-Oxazoline) Star Ionomers // Macromolecular Rapid Communications. 2012. Vol. 33. No. 19. pp. 1690-1694.
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Ten Brummelhuis N., Secker C., Schlaad H. Hofmeister Salt Effects on the LCST Behavior of Poly(2-Oxazoline) Star Ionomers // Macromolecular Rapid Communications. 2012. Vol. 33. No. 19. pp. 1690-1694.
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TY - JOUR
DO - 10.1002/marc.201200406
UR - https://doi.org/10.1002/marc.201200406
TI - Hofmeister Salt Effects on the LCST Behavior of Poly(2-Oxazoline) Star Ionomers
T2 - Macromolecular Rapid Communications
AU - Ten Brummelhuis, Niels
AU - Secker, Christian
AU - Schlaad, Helmut
PY - 2012
DA - 2012/08/22
PB - Wiley
SP - 1690-1694
IS - 19
VL - 33
PMID - 22911889
SN - 1022-1336
SN - 1521-3927
ER -
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@article{2012_Ten Brummelhuis,
author = {Niels Ten Brummelhuis and Christian Secker and Helmut Schlaad},
title = {Hofmeister Salt Effects on the LCST Behavior of Poly(2-Oxazoline) Star Ionomers},
journal = {Macromolecular Rapid Communications},
year = {2012},
volume = {33},
publisher = {Wiley},
month = {aug},
url = {https://doi.org/10.1002/marc.201200406},
number = {19},
pages = {1690--1694},
doi = {10.1002/marc.201200406}
}
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Ten Brummelhuis, Niels, et al. “Hofmeister Salt Effects on the LCST Behavior of Poly(2-Oxazoline) Star Ionomers.” Macromolecular Rapid Communications, vol. 33, no. 19, Aug. 2012, pp. 1690-1694. https://doi.org/10.1002/marc.201200406.