Visible-light-driven four-component diacylation of styrenes with acyl azolium salts: carbonylative synthesis of 1,4-diketones

Publication type: Journal Article
Publication date: 2025-01-21
Springer Nature
scimago Q1
wos Q1
SJR: 2.377
CiteScore: 13.8
Impact factor: 9.7
ISSN: 16747291, 18691870
Abstract
A photochemically induced carbon monoxide-inclusive four-component carbonylation reaction has been delineated, facilitating the diacylation of styrenes with acyl azolium salts to synthesize valuable 1,4-diketone compounds with moderate to good yields. This process proceeds by generating acyl radicals from the Hantzsch esters and carbon monoxide, which subsequently add to the terminal position of styrenes. Then, under light irradiation, the newly generated carbon radical can further react with activated acyl azolium salts to finish the desired 1,4-diketone products.
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GOST Copy
Maolin Y. et al. Visible-light-driven four-component diacylation of styrenes with acyl azolium salts: carbonylative synthesis of 1,4-diketones // Science China Chemistry. 2025.
GOST all authors (up to 50) Copy
Maolin Y., Liu Y., Yang P., ZHAO Y., Wu X. Visible-light-driven four-component diacylation of styrenes with acyl azolium salts: carbonylative synthesis of 1,4-diketones // Science China Chemistry. 2025.
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RIS Copy
TY - JOUR
DO - 10.1007/s11426-024-2382-y
UR - https://link.springer.com/10.1007/s11426-024-2382-y
TI - Visible-light-driven four-component diacylation of styrenes with acyl azolium salts: carbonylative synthesis of 1,4-diketones
T2 - Science China Chemistry
AU - Maolin, Yang
AU - Liu, Yukun
AU - Yang, Peng
AU - ZHAO, YANHUA
AU - Wu, Xiao-Feng
PY - 2025
DA - 2025/01/21
PB - Springer Nature
SN - 1674-7291
SN - 1869-1870
ER -
BibTex
Cite this
BibTex (up to 50 authors) Copy
@article{2025_Maolin,
author = {Yang Maolin and Yukun Liu and Peng Yang and YANHUA ZHAO and Xiao-Feng Wu},
title = {Visible-light-driven four-component diacylation of styrenes with acyl azolium salts: carbonylative synthesis of 1,4-diketones},
journal = {Science China Chemistry},
year = {2025},
publisher = {Springer Nature},
month = {jan},
url = {https://link.springer.com/10.1007/s11426-024-2382-y},
doi = {10.1007/s11426-024-2382-y}
}