Open Access
Applied Physics A: Materials Science and Processing, volume 117, issue 2, pages 847-852
AC conductivity scaling behavior in grain and grain boundary response regime of fast lithium ionic conductors
Publication type: Journal Article
Publication date: 2014-05-01
Quartile SCImago
Q2
Quartile WOS
Q2
Impact factor: 2.7
ISSN: 09478396, 14320630
General Chemistry
General Materials Science
Abstract
AC conductivity spectra of Li-analogues NASICON-type Li1.5Al0.5Ge1.5P3O12 (LAGP), Li–Al–Ti–P–O (LATP) glass–ceramics and garnet-type Li7La2Ta2O13 (LLTO) ceramic are analyzed by universal power law and Summerfield scaling approaches. The activation energies and pre-exponential factors of total and grain conductivities are following the Meyer–Neldel (M-N) rule for NASICON-type materials. However, the garnet-type LLTO material deviates from the M-N rule line of NASICON-type materials. The frequency- and temperature-dependent conductivity spectra of LAGP and LLTO are superimposed by Summerfield scaling. The scaled conductivity curves of LATP are not superimposed at the grain boundary response region. The superimposed conductivity curves are observed at cross-over frequencies of grain boundary response region for LATP by incorporating the $$ \exp \left( {{{ - (E_{A}^{t} - E_{A}^{g} )} \mathord{\left/ {\vphantom {{ - (E_{A}^{t} - E_{A}^{g} )} {kT}}} \right. \kern-0pt} {kT}}} \right) $$ factor along with Summerfield scaling factors on the frequency axis, where $$ E_{A}^{t} $$ and $$ E_{A}^{g} $$ are the activation energies of total and grain conductivities, respectively.
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- We do not take into account publications without a DOI.
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- Statistics recalculated weekly.
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Mariappan C. R. AC conductivity scaling behavior in grain and grain boundary response regime of fast lithium ionic conductors // Applied Physics A: Materials Science and Processing. 2014. Vol. 117. No. 2. pp. 847-852.
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Mariappan C. R. AC conductivity scaling behavior in grain and grain boundary response regime of fast lithium ionic conductors // Applied Physics A: Materials Science and Processing. 2014. Vol. 117. No. 2. pp. 847-852.
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TY - JOUR
DO - 10.1007/s00339-014-8440-1
UR - https://doi.org/10.1007/s00339-014-8440-1
TI - AC conductivity scaling behavior in grain and grain boundary response regime of fast lithium ionic conductors
T2 - Applied Physics A: Materials Science and Processing
AU - Mariappan, C. R.
PY - 2014
DA - 2014/05/01 00:00:00
PB - Springer Nature
SP - 847-852
IS - 2
VL - 117
SN - 0947-8396
SN - 1432-0630
ER -
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@article{2014_Mariappan,
author = {C. R. Mariappan},
title = {AC conductivity scaling behavior in grain and grain boundary response regime of fast lithium ionic conductors},
journal = {Applied Physics A: Materials Science and Processing},
year = {2014},
volume = {117},
publisher = {Springer Nature},
month = {may},
url = {https://doi.org/10.1007/s00339-014-8440-1},
number = {2},
pages = {847--852},
doi = {10.1007/s00339-014-8440-1}
}
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Mariappan, C. R.. “AC conductivity scaling behavior in grain and grain boundary response regime of fast lithium ionic conductors.” Applied Physics A: Materials Science and Processing, vol. 117, no. 2, May. 2014, pp. 847-852. https://doi.org/10.1007/s00339-014-8440-1.