Chemistry of Heterocyclic Compounds

, том 57 , издание 3 , страницы 274-283

Electrocatalytic tandem assembly of aldehydes with 2-thiobarbituric acid into 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) and evaluation of their interaction with catalases

Тип публикации: Journal Article

Дата публикации: 2021-03-25

Springer Nature

Chemistry of Heterocyclic Compounds

SCImago Q3

WOS Q3

БС3

SJR: 0.281

CiteScore: 2.7

Impact factor: 1.2

ISSN: 00093122, 15738353

DOI: 10.1007/s10593-021-02904-8

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Organic Chemistry

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Electrocatalytic transformation of aldehydes with two equivalents of 1,3-diethyl-2-thiobarbituric acid has been carried out in alcohols in an undivided cell in the presence of sodium halides with the selective formation of the substituted 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) in 87–98% yields and with 870–980% current efficiency. This new one-pot electrochemically induced tandem Knoevenagel–Michael process is a simple and efficient approach to substituted 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) containing two 1,3-diethyl-2-thiobarbituric acid fragments separated by C-aryl-substituted spacer, which are promising compounds for different biomedical applications, including anticonvulsant, antiAIDS agents and anti-inflammatory remedies. Theoretical studies were carried out to investigate the interaction of the synthesized compounds with beef and human catalases.

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Elinson M. N. et al. Electrocatalytic tandem assembly of aldehydes with 2-thiobarbituric acid into 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) and evaluation of their interaction with catalases // Chemistry of Heterocyclic Compounds. 2021. Vol. 57. No. 3. pp. 274-283.

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Elinson M. N., Vereshchagin A. N., Ryzhkova Y. E., Karpenko K. A., Ryzhkov F. V., Egorov M. P. Electrocatalytic tandem assembly of aldehydes with 2-thiobarbituric acid into 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) and evaluation of their interaction with catalases // Chemistry of Heterocyclic Compounds. 2021. Vol. 57. No. 3. pp. 274-283.

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TY - JOUR

DO - 10.1007/s10593-021-02904-8

UR - https://doi.org/10.1007/s10593-021-02904-8

TI - Electrocatalytic tandem assembly of aldehydes with 2-thiobarbituric acid into 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) and evaluation of their interaction with catalases

T2 - Chemistry of Heterocyclic Compounds

AU - Elinson, Michail N

AU - Vereshchagin, Anatoly N.

AU - Ryzhkova, Yuliya E

AU - Karpenko, Kirill A

AU - Ryzhkov, Fedor V

AU - Egorov, Mikhail P.

PY - 2021

DA - 2021/03/25

PB - Springer Nature

SP - 274-283

IS - 3

VL - 57

SN - 0009-3122

SN - 1573-8353

ER -

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@article{2021_Elinson,

author = {Michail N Elinson and Anatoly N. Vereshchagin and Yuliya E Ryzhkova and Kirill A Karpenko and Fedor V Ryzhkov and Mikhail P. Egorov},

title = {Electrocatalytic tandem assembly of aldehydes with 2-thiobarbituric acid into 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) and evaluation of their interaction with catalases},

journal = {Chemistry of Heterocyclic Compounds},

year = {2021},

volume = {57},

publisher = {Springer Nature},

month = {mar},

url = {https://doi.org/10.1007/s10593-021-02904-8},

number = {3},

pages = {274--283},

doi = {10.1007/s10593-021-02904-8}

}

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Elinson, Michail N., et al. “Electrocatalytic tandem assembly of aldehydes with 2-thiobarbituric acid into 5,5'-(arylmethylene)bis(1,3-diethyl-2-thiobarbituric acids) and evaluation of their interaction with catalases.” Chemistry of Heterocyclic Compounds, vol. 57, no. 3, Mar. 2021, pp. 274-283. https://doi.org/10.1007/s10593-021-02904-8.

Издатель

Springer Nature

Журнал

Chemistry of Heterocyclic Compounds

SCImago Q3

WOS Q3

БС3

SJR

0.281

CiteScore

2.7

Impact factor